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Fate of Springtime Atmospheric Reactive Mercury: Concentrations and Deposition at Zeppelin, Svalbard

Osterwalder, Stefan; Dunham-Cheatham, Sarrah M.; Araujo, Beatriz Ferreira; Magand, Olivier; Thomas, Jennie L.; Baladima, Foteini; Pfaffhuber, Katrine Aspmo; Berg, Torunn; Zhang, Lei; Huang, Jiaoyan; Dommergue, Aurélien; Sonke, Jeroen E.; Gustin, Mae Sexauer

Mid-latitude atmospheric elemental mercury (Hg) emissions undergo extensive oxidation to reactive Hg (RM) compounds during Arctic polar sunrise, resulting in enhanced atmospheric deposition that impacts Arctic marine wildlife and humans. It has been difficult to estimate RM dry deposition, because RM concentrations, compounds, and their deposition velocities are ill-defined. Here, we investigate RM concentrations sampled with membrane-based methods and find these to exceed denuder-based RM detection by 5 times at the Zeppelin Observatory on Svalbard (March 26–July 24, 2019). Measured dry deposition of gaseous oxidized Hg was about half of the modeled RM deposition, demonstrating that particulate-bound Hg was an important component of dry deposition. Using thermal membrane desorption, RM chemistry was found to be dominated by Hg–Cl/Br (51%) and Hg–N (45%) compounds. Back-trajectory analysis indicated that Hg–Br/Cl compounds were predominantly advected from within the marine boundary layer (sea ice exposure), while Hg–N originated from the free troposphere. Weekly average RM compound-specific dry deposition velocities ranged from 0.12 to 0.49 cm s–1, with a net RM dry deposition of 1.9 μg m–2 (1.5–2.5 μg m–2; 95% confidence interval) that exceeds the mean annual Hg wet deposition flux in Svalbard. Overall, we find that springtime atmospheric RM deposition has been underestimated in the Arctic marine environment.

2021

Evaluation of high-resolution air pollution modelling for the continental Nordic countries

Frohn, Lise Marie; Brandt, Jørgen; Andersson, Camilla; Anderssen, Christopher; Bennet, Cecilia; Christensen, Jesper H.; Im, Ulas; Karvosenoja, Niko; Kukkonen, Jaakko; Lopez-Aparicio, Susana; Nielsen, Ole-Kenneth; Palamarchuk, Yuliia; Paunu, Ville-Veikko; Pleljdrup, Marlene Smith; Segersson, David; Sofiev, Mikhail; Geels, Camilla

2021

Occurrence and dissipation mechanism of organic pollutants during the composting of sewage sludge: A critical review

Lü, Huixiong; Chen, Xiao-Hong; Mo, Che-Hui; Huang, Yu-Hong; He, Min-Ying; Li, Yan-Wen; Feng, Nai-Xian; Katsoyiannis, Athanasios A.; Cai, Quan-Ying

2021

En vellykket miljømessig bærekraftig sirkulær økonomi – Utfordringer og muligheter fra et forskningsperspektiv

Bouman, Evert Alwin; Abbasi, Golnoush; Rostkowski, Pawel Marian; Dusinska, Maria; Guerreiro, Cristina

2021

Black carbon in Siberian Arctic: gas flaring and wildfires impacts

Popovicheva, Olga; Kobelev, Vasily O.; Chichaeva, M. A.; Evangeliou, Nikolaos; Eleftheriadis, K.; Kasimov, Nikolai S.

2021

PAH measurements at Lista. January 2020 – December 2020.

Hak, Claudia

On behalf of Aluminiumindustriens Miljøsekretariat (AMS) and Alcoa Lista, NILU – Norwegian institute for air research has
conducted a sampling campaign in the surroundings of the Alcoa Lista aluminium smelter in order to update the knowledge on PAH-concentrations around the smelter today. Samples were taken in the period January – December 2020 and
analysed for particle bound PAHs. As a consequence of reduced emissions compared to earlier measurements, the ambient
concentrations of benzo(a)pyrene (BaP) were reduced. BaP had an annual average concentration below the target value at
both sampling sites. At Huseby, the lower assessment threshold was exceeded. PAH-levels in the area were similar to those observed in Norwegian cities.

NILU

2021

Appropriate Assimilation Methods for Air Quality Prediction and Pollutant Emission Inversion. An Urban Data Assimilation Systems Report.

Hamer, Paul David; Walker, Sam-Erik; Schneider, Philipp

This report presents a review of data assimilation methods applicable to air quality. In the introduction, we first describe a brief history of data assimilation method development in the context of numerical weather prediction (NWP), and then we highlight key differences when applying data assimilation methods to air quality prediction from NWP applications. Based on these differences, we outline a set of key requirements for data assimilation when applied to air quality. Following this, we review the available data assimilation algorithms and attempt to identify suitable data assimilation methods that could be applied with air quality models. This review and its findings form the basis of the developments to be carried out in the Urban Data Assimilation Systems project.

NILU

2021

Status report of air quality in Europe for year 2019, using validated data

Targa, Jaume; Ripoll, Anna; Banyuls, Lorena; Ortiz, Alberto González; Guerreiro, Cristina

This report presents summarized information on the status of air quality in Europe in 2019, based on validated air quality monitoring data officially reported by the member and cooperating countries of the EEA. It aims at informing on the status of ambient air quality in Europe in 2019 and on the progress towards meeting the European air quality standards for the protection of health, as well as the WHO air quality guidelines. The report also compares the air quality status in 2019 with the previous three years. The pollutants covered in this report are particulate matter (PM10 and PM2.5), O3, NO2, benzo(a)pyrene (BaP), SO2, CO, benzene and toxic metals (As, Cd, Ni, Pb). Measured concentrations above the European air quality standards for PM10, PM2.5, O3, NO2 were reported by 21, 7, 24, and 22 European countries for 2019, respectively. Exceedances of the air quality standards for BaP, SO2, CO, and benzene were measured in, respectively, 14, 6, 3, and two European countries in 2019. Exceedances of European standards for toxic metals were reported by one country for Cd and Pb and by three countries for As and Ni.

ETC/ATNI

2021

European air quality interim mapping under ETC/ATNI. Evaluation of AQ mapping using UTD measurement and CAMS forecast modelling data: an approach for more timely European AQ annual maps.

Horálek, Jan; Hamer, Paul David; Schreiberova, Marketa; Schneider, Philipp

Air quality European-wide annual maps based on the Air Quality (AQ) e-Reporting validated (E1a) measurement data, the EMEP modelling data and other supplementary data have been regularly produced, using the Regression – Interpolation – Merging Mapping (RIMM) methodology. However, due to the time schedule of production of the validated AQ measurement and the EMEP modelling data, the RIMM air quality maps of a year Y have typically not been available until May of year Y+2. In this report, we examine the AQ interim mapping, based on the preliminary (E2a) measurement and the CAMS Ensemble Forecast modelling data. Such interim maps could be prepared one year earlier than the validated maps. In order to overcome an obstacle of data gaps of E2a data in several areas, so-called pseudo stations data in areas with no E2a data are estimated, based on regression relation between E2a data from year Y and validated E1a data from year Y-1, together with the ratio of the modelling results from years Y and Y-1. The analysis have been performed for the PM10 annual average, the NO2 annual average and the ozone indicator SOMO35, based on the 2017 data. We evaluate these maps using the validated E1a data. Based on the results, we recommend the regular production of the interim AQ maps for the examined indicators, in addition to the regular AQ maps.

ETC/ATNI

2021

Towards FAIR nanosafety data

Jeliazkova, Nina; Apostolova, Margarita D.; Andreoli, Cristina; Barone, Flavia; Barrick, Andrew; Battistelli, Chiara L.; Bossa, Cecilia; Botea-Petcu, Alina; Chatel, Amelie; Angelis, Isabella De; Dusinska, Maria; Yamani, Naouale El; Gheorghe, Daniela; Giusti, Anna; Gómez-Fernández, Paloma; Grafström, Roland; Gromelski, Maciej; Jacobsen, Nicklas Raun; Jeliazkov, Vedrin; Jensen, Keld Alstrup; Kochev, Nikolay; Kohonen, Pekka; Manier, Nicolas; Mariussen, Espen; Mech, Agnieszka; Navas, José María; Paskaleva, Vesselina; Precupas, Aurica; Puzyn, Tomasz; Rasmussen, Kirsten; Ritchie, Peter; Llopis, Isabel Rodriguez; Rundén-Pran, Elise; Sandu, Romica; Shandilya, Neeraj; Tanasescu, Sperenta; Haase, Andrea; Nymark, Penny

2021

Time trends of persistent organic pollutants (POPs) and Chemicals of Emerging Arctic Concern (CEAC) in Arctic air from 25 years of monitoring

Wong, Fiona; Hung, Hayley; Dryfhout-Clark, Helena; Aas, Wenche; Bohlin-Nizzetto, Pernilla; Breivik, Knut; Mastromonaco, Michelle N.; Brorström-Lundén, Eva; Ólafsdóttir, Kristín; Sigurdsson, Arni; Vorkamp, Katrin; Bossi, Rossana; Skov, Henrik; Hakola, Hannele; Barresi, Enzo; Sverko, Ed; Fellin, Phil; Li, Henrik; Vlasenko, Alexander; Zapevalov, Mikhail; Samsonov, Dmitry; Wilson, Simon

The long-term time trends of atmospheric pollutants at eight Arctic monitoring stations are reported. The work was conducted under the Arctic Monitoring and Assessment Programme (AMAP) of the Arctic Council. The monitoring stations were: Alert, Canada; Zeppelin, Svalbard; Stórhöfði, Iceland; Pallas, Finland; Andøya, Norway; Villum Research Station, Greenland; Tiksi and Amderma, Russia. Persistent organic pollutants (POPs) such as α- and γ-hexachlorocyclohexane (HCH), polychlorinated biphenyls (PCBs), α-endosulfan, chlordane, dichlorodiphenyltrichloroethane (DDT) and polybrominated diphenyl ethers (PBDEs) showed declining trends in air at all stations. However, hexachlorobenzene (HCB), one of the initial twelve POPs listed in the Stockholm Convention in 2004, showed either increasing or non-changing trends at the stations. Many POPs demonstrated seasonality but the patterns were not consistent among the chemicals and stations. Some chemicals showed winter minimum and summer maximum concentrations at one station but not another, and vice versa. The ratios of chlordane isomers and DDT species showed that they were aged residues. Time trends of perfluorooctanoic acid (PFOA) and perfluorooctane sulfonic acid (PFOS) were showing decreasing concentrations at Alert, Zeppelin and Andøya. The Chemicals of Emerging Arctic Concern (CEAC) were either showing stable or increasing trends. These include methoxychlor, perfluorohexane sulfonic acid (PFHxS), 6:2 fluorotelomer alcohol, and C9-C11 perfluorocarboxylic acids (PFCAs). We have demonstrated the importance of monitoring CEAC before they are being regulated because model calculations to predict their transport mechanisms and fate cannot be made due to the lack of emission inventories. We should maintain long-term monitoring programmes with consistent data quality in order to evaluate the effectiveness of chemical control efforts taken by countries worldwide.

2021

Transformative Potential and Learning Outcomes of Air Quality Citizen Science Projects in High Schools Using Low-Cost Sensors

Grossberndt, Sonja; Passani, Antonella; Lisio, Giulia Di; Janssen, Anneli; Castell, Nuria

The rise of advanced ICT technologies has made it possible to apply low-cost sensor systems for measuring air quality in citizen science projects, including education. High school students in Norway used these sensor systems in a citizen science project to design, carry out, and evaluate their own research projects on air quality. An impact assessment framework was designed to assess the impact of these activities, considering five areas of impact: scientific, social, economic, political, and environmental. In addition, the framework also considers the transformative potential of the citizen science pilot, i.e., the degree to which the pilot can help to change, alter, or replace current systems, and the business-as-usual in one or more fields such as knowledge production or environmental protection. Data for this assessment were gathered in the form of questionnaires that the students had to complete before starting and after finalizing the pilot activities. The results showed positive impacts on learning, a pro-environmental world view, and an increase in pro-science attitudes and interest in scientific and environmental-related topics at the end of the pilot activities. Only weak impacts were measured for behavioral change. The activities showed transformative potential, which makes the student activities an example of good practice for citizen science activities on air quality with low-cost sensors.

2021

SIOS’s Earth Observation (EO), Remote Sensing (RS), and operational activities in response to COVID-19

Jawak, Shridhar D.; Andersen, Bo Nyborg; Pohjola, Veijo A; Godøy, Øystein; Hübner, Christiane; Jennings, Inger; Ignatiuk, Dariusz; Holmen, Kim; Sivertsen, Agnar; Hann, Richard; Tømmervik, Hans; Kääb, Andreas; Błaszczyk, Małgorzata; Salzano, Roberto; Luks, Bartłomiej; Høgda, Kjell Arild; Storvold, Rune; Nilsen, Lennart; Salvatori, Rosamaria; Krishnan, Kottekkatu Padinchati; Chatterjee, Sourav; Lorentzen, Dag A; Erlandsson, Rasmus; Lauknes, Tom Rune; Malnes, Eirik; Karlsen, Stein Rune; Enomoto, Hiroyuki; Fjæraa, Ann Mari; Zhang, Jie; Marty, Sabine; Nygård, Knut; Lihavainen, Heikki

Svalbard Integrated Arctic Earth Observing System (SIOS) is an international partnership of research institutions studying the environment and climate in and around Svalbard. SIOS is developing an efficient observing system, where researchers share technology, experience, and data, work together to close knowledge gaps, and decrease the environmental footprint of science. SIOS maintains and facilitates various scientific activities such as the State of the Environmental Science in Svalbard (SESS) report, international access to research infrastructure in Svalbard, Earth observation and remote sensing services, training courses for the Arctic science community, and open access to data. This perspective paper highlights the activities of SIOS Knowledge Centre, the central hub of SIOS, and the SIOS Remote Sensing Working Group (RSWG) in response to the unprecedented situation imposed by the global pandemic coronavirus (SARS-CoV-2) disease 2019 (COVID-19). The pandemic has affected Svalbard research in several ways. When Norway declared a nationwide lockdown to decrease the rate of spread of the COVID-19 in the community, even more strict measures were taken to protect the Svalbard community from the potential spread of the disease. Due to the lockdown, travel restrictions, and quarantine regulations declared by many nations, most physical meetings, training courses, conferences, and workshops worldwide were cancelled by the first week of March 2020. The resumption of physical scientific meetings is still uncertain in the foreseeable future. Additionally, field campaigns to polar regions, including Svalbard, were and remain severely affected. In response to this changing situation, SIOS initiated several operational activities suitable to mitigate the new challenges resulting from the pandemic. This article provides an extensive overview of SIOS’s Earth observation (EO), remote sensing (RS) and other operational activities strengthened and developed in response to COVID-19 to support the Svalbard scientific community in times of cancelled/postponed field campaigns in Svalbard. These include (1) an initiative to patch up field data (in situ) with RS observations, (2) a logistics sharing notice board for effective coordinating field activities in the pandemic times, (3) a monthly webinar series and panel discussion on EO talks, (4) an online conference on EO and RS, (5) the SIOS’s special issue in the Remote Sensing (MDPI) journal, (6) the conversion of a terrestrial remote sensing training course into an online edition, and (7) the announcement of opportunity (AO) in airborne remote sensing for filling the data gaps using aerial imagery and hyperspectral data. As SIOS is a consortium of 24 research institutions from 9 nations, this paper also presents an extensive overview of the activities from a few research institutes in pandemic times and highlights our upcoming activities for the next year 2021. Finally, we provide a critical perspective on our overall response, possible broader impacts, relevance to other observing systems, and future directions. We hope that our practical services, experiences, and activities implemented in these difficult times will motivate other similar monitoring programs and observing systems when responding to future challenging situations. With a broad scientific audience in mind, we present our perspective paper on activities in Svalbard as a case study.
Earth observation; Remote sensing; COVID-19; Svalbard; Earth System Science; SIOS

2021

Synergistic and Competing Influences of Air Pollutants on Air Quality and Arctic Climate

Salzen, Knut von; Anenberg, Susan C.; Arnold, Steve; Eckhardt, Sabine; Ekman, Annica; Flanner, Mark G.; Gauss, Michael; Im, Ulas; Klimont, Zbigniew; Krishnan, Srinath; Kupiainen, Kaarle; Mahmood, Rashed; Oliviè, Dirk Jan Leo; Oshima, Naga; Pozzoli, Luca; Rao, Shilpa; Sand, Maria; Sigmond, Michael; Tsigaridis, Kostas; Tsyro, Svetlana; Turnock, Steven T; Dingenen, Rita Van; Whaley, Cynthia; Winter, Barbara

2021

Low-cost O3 sensor in remote Alpine environment

Dallo, Frederico; Zannoni, Daniele; Gabrieli, Jacopo; Cristofanelli, Paolo; Calzolari, Francescopiero; Blasi, Fabrizio de; Spolaor, Andrea; Battistel, Dario; Lodi, Rachele; Cairns, Warren R. L.; Fjæraa, Ann Mari; Bonasoni, Paolo; Barbante, Carlo

2021

Mercury observations in EMEP

Tørseth, Kjetil; Pfaffhuber, Katrine Aspmo; Aas, Wenche; Rud, Richard Olav

2021

Skogens helsetilstand i Norge. Resultater fra skogskadeovervåkingen i 2020.

Timmermann, Volkmar; Beachell, Andreas Myki; Brurberg, May Bente; Børja, Isabella; Clarke, Nicholas; Fløistad, Inger; Hietala, Ari Mikko; Hylen, Gro; Jepsen, Jane Uhd; Nordbakken, Jørn-Frode; Pettersson, Martin; Solberg, Sverre; Solheim, Halvor; Talgø, Venche; Vindstad, Ole Petter Laksforsmo; Økland, Bjørn; Aas, Wenche

Skogens helsetilstand påvirkes i stor grad av klima og værforhold, enten direkte ved tørke, frost og vind, eller indirekte ved at klimaet påvirker omfanget av soppsykdommer og insektangrep. Klimaendringene og den forventede økningen i klimarelaterte skogskader gir store utfordringer for forvaltningen av framtidas skogressurser. Det samme gjør invaderende skadegjørere, både allerede etablerte arter og nye som kan komme til Norge i nær framtid. I denne rapporten presenteres resultater fra skogskadeovervåkingen i Norge i 2020 og trender over tid.
I den landsrepresentative skogovervåkingen har kronetettheten hos gran og furu holdt seg stabil i 2020 sammenlignet med tidligere år. Det ble registrert lite misfarging hos bartrærne.
Skadenivået hos både bartrær, bjørk og andre løvtrær var lavere enn i 2019. Abiotiske faktorer med snø, vind og tørke som de viktigste årsakene dominerte skadebildet hos alle treslag.
Kjemiske analyser av luft og nedbør i den intensive skogovervåkingen viser at det fortsatt er høyest verdier av antropogene svovel- og nitrogenforbindelser på den sørligste overvåkingsflata i Birkenes grunnet langtransportert forurensing. Den høyeste konsentrasjonen av nitrogendioksid i luft ble målt på stasjonen i Hurdal i 2020, noe som skyldes utslipp fra veitrafikken i regionen. Det var lave nivåer av bakkenært ozon i Norge i 2020 og ingen overskridelser av UNECEs grenseverdi på 5000 ppb-timer for skog. Vegetasjonsanalysene fra Hurdal har påvist en endring i bunn-vegetasjonens artssammensetning grunnet økt lystilgang og mye barnålstrø. Både hogst utenfor overvåkingsflata og flere skrantende, råteangrepne og døde grantrær i flata har bidratt til økt lystilgang og til større strømengde på bakken. Mange grantrær på flata i Hurdal er sterkt preget av råte med lav kronetetthet og mye misfarging. Flere trær på flata har dødd de seinere årene som følge av råteskader, ofte i kombinasjon med andre faktorer som vindfelling og skader etter tørken i 2018 med påfølgende barkbilleangrep.
Overvåking av bjørkemålere har vist at fjellbjørkeskogen både i Nord-Norge og fjellregionene i sørlige halvdel av landet har vært utsatt for betydelige utbrudd av bjørkemålere i løpet av perioden 2012–2018. Overvåkingsdata fra 2019 og 2020 tyder imidlertid på at målerbestandene nå er lave eller i sterk tilbakegang i det meste av landet. I Troms har målerbestandene allerede nådd et bunnpunkt, og bestandene er nedadgående også i fjellet i Sør-Norge. Vi forventer derfor at skogen i mesteparten av Norge vil bli mindre utsatt for angrep av bjørkemålere de neste par årene.
De fleste fylkene hadde en økning i fangstverdiene i barkbilleovervåkingen i 2020-sesongen. Alle fangstverdiene var imidlertid under 10 000 biller per felle, mens de høyeste verdiene ved slutten av utbruddet på 1970-tallet var rundt 25 000 biller per felle. Fylkene rundt Oslofjorden hadde noen lokale tilfeller av tørke- og barkbilleskader. Det ble ikke funnet noen tydelig økning av fellefangstene i tiden for en annen generasjon, men modellberegninger viser at stor granbarkbille har nok døgngrader til å gjennomføre to generasjoner før overvintring.
I august 2020 ble soppen Diplodia sapinea funnet på sterkt skadet vrifuru i Ås kommune. Tidligere har det blitt gjort noen få funn av soppen på andre bartrearter i det samme området. D. sapinea er vanlig i varmere strøk på flere kontinenter, spesielt på furuarter. De pågående klima-endringene har trolig bidratt til at soppen har kunnet spre og etablere seg mot nord, men vi kan heller ikke utelukke innførsel av soppen via plantemateriale til bruk i grøntanlegg eller skog. D. sapinea er trolig bare i etableringsfasen i Norge, og har til dags dato gjort liten skade på våre stedegne bartrær.....

NIBIO

2021

Main sources controlling atmospheric burdens of persistent organic pollutants on a national scale

Halvorsen, Helene Lunder; Bohlin-Nizzetto, Pernilla; Eckhardt, Sabine; Gusev, Alexey; Krogseth, Ingjerd Sunde; Möckel, Claudia; Shatalov, Victor; Skogeng, Lovise Pedersen; Breivik, Knut

National long-term monitoring programs on persistent organic pollutants (POPs) in background air have traditionally relied on active air sampling techniques. Due to limited spatial coverage of active air samplers, questions remain (i) whether active air sampler monitoring sites are representative for atmospheric burdens within the larger geographical area targeted by the monitoring programs, and thus (ii) if the main sources affecting POPs in background air across a nation are understood. The main objective of this study was to explore the utility of spatial and temporal trends in concert with multiple modelling approaches to understand the main sources affecting polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in background air across a nation. For this purpose, a comprehensive campaign was carried out in summer 2016, measuring POPs in background air across Norway using passive air sampling. Results were compared to a similar campaign in 2006 to assess possible changes over one decade. We furthermore used the Global EMEP Multi-media Modeling System (GLEMOS) and the Flexible Particle dispersion model (FLEXPART) to predict and evaluate the relative importance of primary emissions, secondary emissions, long-range atmospheric transport (LRAT) and national emissions in controlling atmospheric burdens of PCB-153 on a national scale. The concentrations in air of both PCBs and most of the targeted OCPs were generally low, with the exception of hexachlorobenzene (HCB). A limited spatial variability for all POPs in this study, together with predictions by both models, suggest that LRAT dominates atmospheric burdens across Norway. Model predictions by the GLEMOS model, as well as measured isomeric ratios, further suggest that LRAT of some POPs are dictated by secondary emissions. Our results illustrate the utility of combining observations and mechanistic modelling approaches to help identify the main factors affecting atmospheric burdens of POPs across a nation, which, in turn, may be used to inform both national monitoring and control strategies.

2021

The SCCS scientific advice on the safety of nanomaterials in cosmetics

Bernauer, Ulrike; Bodin, Laurent; Chaudhry, Qasim; Coenraads, Pieter Jan; Dusinska, Maria; Gaffet, Eric; Panteri, Eirini; Rogiers, Vera; Rousselle, Christophe; Stepnik, Maciej; Vanhaecke, Tamara; Wijnhoven, Susan; Goetz, Natalie von; Jong, Wim H. de

2021

Using the 3D MOCAGE CTM to simulate the chemistry of halogens in the volcanic plume of Etna's eruption in December 2018 at the regional scale

Narivelo, Herizo; Marécal, Virginie; Hamer, Paul David; Surl, Luke; Roberts, Tjarda; Bacles, Mickaël; Varnach, Simon; Wagner, Thomas

2021

Global NH3 emissions from livestock management: Implementation of a dynamical module within a land surface model and impact on atmospheric chemistry

Beaudor, M.; Vuichard, Nicolas; Lathiere, J.; Damme, M Van; Coheur, PF; Clarisse, L.; Evangeliou, Nikolaos; Hauglustaine, D

2021

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