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Low-cost O3 sensor in remote Alpine environment

Dallo, Frederico; Zannoni, Daniele; Gabrieli, Jacopo; Cristofanelli, Paolo; Calzolari, Francescopiero; Blasi, Fabrizio de; Spolaor, Andrea; Battistel, Dario; Lodi, Rachele; Cairns, Warren R. L.; Fjæraa, Ann Mari; Bonasoni, Paolo; Barbante, Carlo

2021

Mercury observations in EMEP

Tørseth, Kjetil; Pfaffhuber, Katrine Aspmo; Aas, Wenche; Rud, Richard Olav

2021

En vellykket miljømessig bærekraftig sirkulær økonomi – Utfordringer og muligheter fra et forskningsperspektiv

Bouman, Evert Alwin; Abbasi, Golnoush; Rostkowski, Pawel Marian; Dusinska, Maria; Guerreiro, Cristina

2021

Black carbon in Siberian Arctic: gas flaring and wildfires impacts

Popovicheva, Olga; Kobelev, Vasily O.; Chichaeva, M. A.; Evangeliou, Nikolaos; Eleftheriadis, K.; Kasimov, Nikolai S.

2021

Skogens helsetilstand i Norge. Resultater fra skogskadeovervåkingen i 2020.

Timmermann, Volkmar; Beachell, Andreas Myki; Brurberg, May Bente; Børja, Isabella; Clarke, Nicholas; Fløistad, Inger; Hietala, Ari Mikko; Hylen, Gro; Jepsen, Jane Uhd; Nordbakken, Jørn-Frode; Pettersson, Martin; Solberg, Sverre; Solheim, Halvor; Talgø, Venche; Vindstad, Ole Petter Laksforsmo; Økland, Bjørn; Aas, Wenche

Skogens helsetilstand påvirkes i stor grad av klima og værforhold, enten direkte ved tørke, frost og vind, eller indirekte ved at klimaet påvirker omfanget av soppsykdommer og insektangrep. Klimaendringene og den forventede økningen i klimarelaterte skogskader gir store utfordringer for forvaltningen av framtidas skogressurser. Det samme gjør invaderende skadegjørere, både allerede etablerte arter og nye som kan komme til Norge i nær framtid. I denne rapporten presenteres resultater fra skogskadeovervåkingen i Norge i 2020 og trender over tid.
I den landsrepresentative skogovervåkingen har kronetettheten hos gran og furu holdt seg stabil i 2020 sammenlignet med tidligere år. Det ble registrert lite misfarging hos bartrærne.
Skadenivået hos både bartrær, bjørk og andre løvtrær var lavere enn i 2019. Abiotiske faktorer med snø, vind og tørke som de viktigste årsakene dominerte skadebildet hos alle treslag.
Kjemiske analyser av luft og nedbør i den intensive skogovervåkingen viser at det fortsatt er høyest verdier av antropogene svovel- og nitrogenforbindelser på den sørligste overvåkingsflata i Birkenes grunnet langtransportert forurensing. Den høyeste konsentrasjonen av nitrogendioksid i luft ble målt på stasjonen i Hurdal i 2020, noe som skyldes utslipp fra veitrafikken i regionen. Det var lave nivåer av bakkenært ozon i Norge i 2020 og ingen overskridelser av UNECEs grenseverdi på 5000 ppb-timer for skog. Vegetasjonsanalysene fra Hurdal har påvist en endring i bunn-vegetasjonens artssammensetning grunnet økt lystilgang og mye barnålstrø. Både hogst utenfor overvåkingsflata og flere skrantende, råteangrepne og døde grantrær i flata har bidratt til økt lystilgang og til større strømengde på bakken. Mange grantrær på flata i Hurdal er sterkt preget av råte med lav kronetetthet og mye misfarging. Flere trær på flata har dødd de seinere årene som følge av råteskader, ofte i kombinasjon med andre faktorer som vindfelling og skader etter tørken i 2018 med påfølgende barkbilleangrep.
Overvåking av bjørkemålere har vist at fjellbjørkeskogen både i Nord-Norge og fjellregionene i sørlige halvdel av landet har vært utsatt for betydelige utbrudd av bjørkemålere i løpet av perioden 2012–2018. Overvåkingsdata fra 2019 og 2020 tyder imidlertid på at målerbestandene nå er lave eller i sterk tilbakegang i det meste av landet. I Troms har målerbestandene allerede nådd et bunnpunkt, og bestandene er nedadgående også i fjellet i Sør-Norge. Vi forventer derfor at skogen i mesteparten av Norge vil bli mindre utsatt for angrep av bjørkemålere de neste par årene.
De fleste fylkene hadde en økning i fangstverdiene i barkbilleovervåkingen i 2020-sesongen. Alle fangstverdiene var imidlertid under 10 000 biller per felle, mens de høyeste verdiene ved slutten av utbruddet på 1970-tallet var rundt 25 000 biller per felle. Fylkene rundt Oslofjorden hadde noen lokale tilfeller av tørke- og barkbilleskader. Det ble ikke funnet noen tydelig økning av fellefangstene i tiden for en annen generasjon, men modellberegninger viser at stor granbarkbille har nok døgngrader til å gjennomføre to generasjoner før overvintring.
I august 2020 ble soppen Diplodia sapinea funnet på sterkt skadet vrifuru i Ås kommune. Tidligere har det blitt gjort noen få funn av soppen på andre bartrearter i det samme området. D. sapinea er vanlig i varmere strøk på flere kontinenter, spesielt på furuarter. De pågående klima-endringene har trolig bidratt til at soppen har kunnet spre og etablere seg mot nord, men vi kan heller ikke utelukke innførsel av soppen via plantemateriale til bruk i grøntanlegg eller skog. D. sapinea er trolig bare i etableringsfasen i Norge, og har til dags dato gjort liten skade på våre stedegne bartrær.....

NIBIO

2021

Main sources controlling atmospheric burdens of persistent organic pollutants on a national scale

Halvorsen, Helene Lunder; Bohlin-Nizzetto, Pernilla; Eckhardt, Sabine; Gusev, Alexey; Krogseth, Ingjerd Sunde; Möckel, Claudia; Shatalov, Victor; Skogeng, Lovise Pedersen; Breivik, Knut

National long-term monitoring programs on persistent organic pollutants (POPs) in background air have traditionally relied on active air sampling techniques. Due to limited spatial coverage of active air samplers, questions remain (i) whether active air sampler monitoring sites are representative for atmospheric burdens within the larger geographical area targeted by the monitoring programs, and thus (ii) if the main sources affecting POPs in background air across a nation are understood. The main objective of this study was to explore the utility of spatial and temporal trends in concert with multiple modelling approaches to understand the main sources affecting polychlorinated biphenyls (PCBs) and organochlorine pesticides (OCPs) in background air across a nation. For this purpose, a comprehensive campaign was carried out in summer 2016, measuring POPs in background air across Norway using passive air sampling. Results were compared to a similar campaign in 2006 to assess possible changes over one decade. We furthermore used the Global EMEP Multi-media Modeling System (GLEMOS) and the Flexible Particle dispersion model (FLEXPART) to predict and evaluate the relative importance of primary emissions, secondary emissions, long-range atmospheric transport (LRAT) and national emissions in controlling atmospheric burdens of PCB-153 on a national scale. The concentrations in air of both PCBs and most of the targeted OCPs were generally low, with the exception of hexachlorobenzene (HCB). A limited spatial variability for all POPs in this study, together with predictions by both models, suggest that LRAT dominates atmospheric burdens across Norway. Model predictions by the GLEMOS model, as well as measured isomeric ratios, further suggest that LRAT of some POPs are dictated by secondary emissions. Our results illustrate the utility of combining observations and mechanistic modelling approaches to help identify the main factors affecting atmospheric burdens of POPs across a nation, which, in turn, may be used to inform both national monitoring and control strategies.

2021

The SCCS scientific advice on the safety of nanomaterials in cosmetics

Bernauer, Ulrike; Bodin, Laurent; Chaudhry, Qasim; Coenraads, Pieter Jan; Dusinska, Maria; Gaffet, Eric; Panteri, Eirini; Rogiers, Vera; Rousselle, Christophe; Stepnik, Maciej; Vanhaecke, Tamara; Wijnhoven, Susan; Goetz, Natalie von; Jong, Wim H. de

2021

Using the 3D MOCAGE CTM to simulate the chemistry of halogens in the volcanic plume of Etna's eruption in December 2018 at the regional scale

Narivelo, Herizo; Marécal, Virginie; Hamer, Paul David; Surl, Luke; Roberts, Tjarda; Bacles, Mickaël; Varnach, Simon; Wagner, Thomas

2021

Global NH3 emissions from livestock management: Implementation of a dynamical module within a land surface model and impact on atmospheric chemistry

Beaudor, M.; Vuichard, Nicolas; Lathiere, J.; Damme, M Van; Coheur, PF; Clarisse, L.; Evangeliou, Nikolaos; Hauglustaine, D

2021

Impacts of Short-lived Climate Forcers on Arctic Climate, Air Quality, and Human Health

Kupiainen, Kaarle; Eckhardt, Sabine; Flanner, Mark G. (eds.)

Arctic Monitoring and Assessment Programme (AMAP)

2021

Understanding Air Quality Trends in Europe. Focus on the relative contribution of changes in emission of activity sectors, natural fraction and meteorological variability.

Colette, Augustin; Solberg, Sverre; Aas, Wenche; Walker, Sam-Erik

Emission changes are the main driver of all air pollutant trends. For NO2 and PM10, both the GAM and the CTM results indicate that emission changes contribute to at least 90% of the 2000-2017 trend. For ozone peaks (as 4MDA8), meteorology can be important. The GAM model estimates that it contributes to an increase counteracting mitigation effort up to a magnitude of 20 to 80% (compared to the effect of emission and background changes) in Austria, Belgium, Czech Republic, France, and Italy. Given the good skill of the GAM model to capture meteorological effect, this estimate can be considered quite robust.

The relative contribution of agriculture and industry to the total PM10 mass has been reduced by around 30% for both sectors, but the similarity of evolution is not directly linked to the emission trends in the respective sectors. The relationship between emissions and concentrations is nonlinear and depends on availability of precursor gases to form ammonium sulphate and ammonium nitrate. The relative contribution of traffic sources to PM10 has been reduced with around 20%, while the trend attributed to residential heating is marginal. The heating sector has become a relatively more important contributor to the aerosol pollution and needs more attention. The model also indicates that the natural contributions (such as sea salt and dust) has had little impact on the long-term changes in PM10.

The analysis includes observational data only from stations with data available for at least 14 years in the period 2000-2017. This drastically reduces the number of monitoring sites included in the analysis and the spatial representativity of the assessment, with bias towards countries benefiting from a long-term monitoring network.

Further improvements of models as well as observational basis are needed to reduce the uncertainties. Understanding organic aerosols from the residential heating sector should be a priority.

ETC/ATNI

2021

Health risk assessments of air pollution. Estimations of the 2019 HRA, benefit analysis of reaching specific air quality standards and more.

Ortiz, Alberto González; Guerreiro, Cristina; Soares, Joana; Horálek, Jan

The health risk related to exposure to air pollution (fine particulate matter - PM2.5, ozone - O3, and nitrogen dioxide - NO2) in 2019 was estimated in terms of number of premature deaths and years of life lost related to exposure to for 41 European countries, including the 27 EU Member States. In 2019, air pollution continued to drive a significant burden of premature death and disease in the 41 countries reporting to EEA: 373,000 premature deaths were attributed to chronic exposure to PM2.5; 47,700 premature deaths were attributed to chronic NO2 exposure; 19,070 premature deaths were attributed to acute O3 exposure. The analysis on the EU’s progress to reach the 2030 target established in the Zero Pollution Action Plan shows a steady decrease in the number of premature deaths along the years, and if it continues to fall at a comparable rate in the future, then the target would be achieved by 2032. Had the new WHO air quality guideline level for PM2.5 of 5 µg/m3 been attained already in 2019 everywhere in Europe, the number of estimated premature deaths would have been at least 58 % lower. On the other hand, the attainment of the EU limit value for PM2.5 of 25 µg/m3 would have left the estimated number of premature deaths unchanged in EU-27.

ETC/ATNI

2021

Erratum: Fate of Springtime Atmospheric Reactive Mercury: Concentrations and Deposition at Zeppelin, Svalbard (ACS Earth Space Chem. (2021) 5:11 (3234−3246) DOI: 10.1021/acsearthspacechem.1c00299)

Osterwalder, Stefan; Dunham-Cheatham, Sarrah M.; Araujo, Beatriz Ferreira; Magand, Olivier; Thomas, Jennie L.; Baladima, Foteini; Pfaffhuber, Katrine Aspmo; Berg, Torunn; Zhang, Lei; Huang, Jiaoyan; Zieger, Paul; Dommergue, Aurélien; Sonke, Jeroen E.; Gustin, Mae Sexauer

2021

Cloud-scale modelling of the impact of deep convection on the fate of oceanic bromoform in the troposphere: a case study over the west coast of Borneo

Hamer, Paul David; Marécal, Virginie; Hossaini, Ryan; Pirre, Michel; Krysztofiak, Gisele; Ziska, Franziska; Engel, Andreas; Sala, Stephan; Keber, Timo; Bönisch, Harald; Atlas, Elliot; Krüger, Kirstin; Chipperfield, Martyn; Catoire, Valery; Samah, Azizan A.; Dorf, Marcel; Moi, Phang Siew; Schlager, Hans; Pfeilsticker, Klaus

This paper presents a modelling study on the fate of CHBr3 and its product gases in the troposphere within the context of tropical deep convection. A cloud-scale case study was conducted along the west coast of Borneo, where several deep convective systems were triggered on the afternoon and early evening of 19 November 2011. These systems were sampled by the Falcon aircraft during the field campaign of the SHIVA project and analysed using a simulation with the cloud-resolving meteorological model C-CATT-BRAMS at 2×2 km resolution that represents the emissions, transport by large-scale flow, convection, photochemistry, and washout of CHBr3 and its product gases (PGs). We find that simulated CHBr3 mixing ratios and the observed values in the boundary layer and the outflow of the convective systems agree. However, the model underestimates the background CHBr3 mixing ratios in the upper troposphere, which suggests a missing source at the regional scale. An analysis of the simulated chemical speciation of bromine within and around each simulated convective system during the mature convective stage reveals that >85 % of the bromine derived from CHBr3 and its PGs is transported vertically to the point of convective detrainment in the form of CHBr3 and that the remaining small fraction is in the form of organic PGs, principally insoluble brominated carbonyls produced from the photo-oxidation of CHBr3. The model simulates that within the boundary layer and free troposphere, the inorganic PGs are only present in soluble forms, i.e. HBr, HOBr, and BrONO2, and, consequently, within the convective clouds, the inorganic PGs are almost entirely removed by wet scavenging. We find that HBr is the most abundant PG in background lower-tropospheric air and that this prevalence of HBr is a result of the relatively low background tropospheric ozone levels at the regional scale. Contrary to a previous study in a different environment, for the conditions in the simulation, the insoluble Br2 species is hardly formed within the convective systems and therefore plays no significant role in the vertical transport of bromine. This likely results from the relatively small quantities of simulated inorganic bromine involved, the presence of HBr in large excess compared to HOBr and BrO, and the relatively efficient removal of soluble compounds within the convective column.

2021

Hydrolysis of FTOH precursors, a simple method to account for some of the unknown PFAS

Nikiforov, Vladimir

There is a growing concern over a suspected presense of unknown perfluoroaliphatic substances (PFAS) in consumer goods and in the environment. Such unknown substances, possibly with high molecular weight, might be precursors of hazardous or controlled known PFAS. Recent studies confirmed that total organic fluorine (TOF) content often can not be explained by the measured target PFAS. One of the suspected classes of such unknowns are polymers with fluorotelomer alcohol (FTOH) residues in a side chain. In this report we suggest hydrolysis of precursors, as a complementary method to account for the unknown PFAS. It was shown here that hydrolysis allows to preserve structural information on the perlfuorinated parts of the precursors, which can be an advantage for the purpose of accurate risk assessment or source identification. A convenient procedure for hydrolysis with 4% sodium hydroxide inwater-methanol mixture (1:9) at 60 C for 16 h was shown to convert model substances - FTOH acrylate, methacrylate and isobutyrate esters as well as FTOH phenylcarbamate to free FTOHs. Analysis of extracts of textile samples with preliminary hydrolysis and without it showed up to 1300-fold higher level of “hidden” FTOHs.

2021

Impacts of UV irradiance and medium-energy electron precipitation on the North Atlantic oscillation during the 11-year solar cycle

Guttu, Sigmund; Orsolini, Yvan; Stordal, Frode; Otterå, Odd Helge; Omrani, Nour-Eddine; Tartaglione, Nazario; Verronen, Pekka T.; Rodger, Craig J.; Clilverd, Mark A.

Observational studies suggest that part of the North Atlantic Oscillation (NAO) variability may be attributed to the spectral ultra-violet (UV) irradiance variations associated to the 11-year solar cycle. The observed maximum surface pressure response in the North Atlantic occurs 2–4 years after solar maximum, and some model studies have identified that atmosphere–ocean feedbacks explain the multi-year lag. Alternatively, medium-to-high energy electron (MEE) precipitation, which peaks in the declining phase of the solar cycle, has been suggested as a potential cause of this lag. We use a coupled (ocean–atmosphere) climate prediction model and a state-of-the-art MEE forcing to explore the respective roles of irradiance and MEE precipitation on the NAO variability. Three decadal ensemble experiments were conducted over solar cycle 23 in an idealized setting. We found a weak ensemble-mean positive NAO response to the irradiance. The simulated signal-to-noise ratio remained very small, indicating the predominance of internal NAO variability. The lack of multi-annual lag in the NAO response was likely due to lagged solar signals imprinted in temperatures below the oceanic mixed-layer re-emerging equatorward of the oceanic frontal zones, which anchor ocean–atmosphere feedbacks. While there is a clear, yet weak, signature from UV irradiance in the atmosphere and upper ocean over the North Atlantic, enhanced MEE precipitation on the other hand does not lead to any systematic changes in the stratospheric circulation, despite its marked chemical signatures.

2021

Evaluation of interannual variability of Arctic and Antarctic ozone loss since 198

Goutail, Florence; Pazmino, Andrea; Pommereau, Jean-Pierre; Lefevre, Franck; Godin-Beekmann, Sophie; Hauchecorne, Alain; Lecouffe, Audrey; Clerbaux, Cathy; Boynard, Anne; Hadji-Lazaro, Juliette; Chipperfield, Martyn P.; Feng, Wuhu; Roozendael, Michel Van; Jepsen, Nis; Hansen, Georg Heinrich; Kivi, Rigel; Bognar, Kristof; Strong, Kimberly; Walker, Kaley A.; Colwell, Steve

2021

The hCOMET project: International database comparison of results with the comet assay in human biomonitoring. Baseline frequency of DNA damage and effect of main confounders

Milić, Mirta; Ceppi, Marcello; Bruzzone, Marco; Azqueta, Amaya; Brunborg, Gunnar; Godschalk, Roger; Koppen, Gudrun; Langie, Sabine; Møller, Peter; Teixeira, João Paulo; Alija, Avdulla; Anderson, Diana; Andrade, Vanessa; Andreoli, Cristina; Asllani, Fisnik; Bangkoglu, Ezgi Eyluel; Barancokova, Magdalena; Basaran, Nursen; Boutet-Robinet, Elisa; Buschini, Annamaria; Cavallo, Delia; Pererira, Cristina Costa; Costa, Carla; Costa, Solange; Silva, Juliana Da; Bo’, Cristian Del; Sreckovic, Vesna Dimitrijevic; Djelic, Ninoslav; Dobrzynska, Malgorzata; Duracková, Zdenka; Dvorakova, Monika; Gajski, Goran; Galati, Serena; Lima, Omar García; Giovannelli, Lisa; Goroshinskaya, Irina A.; Grindel, Annemarie; Gützkow, Kristine Bjerve; Hernández, Alba; Hernandez, Carlos; Holven, Kirsten Bjørklund; Ibero-Baraibar, Idoia; Ottestad, Inger Olaug; Kadioglu, Ela; Kazimirova, Alena; Kuznetsova, Elena; Ladeira, Carina; Laffon, Blanca; Lamonaca, Palma; Lebailly, Pierre; Louro, Henriqueta; Cardoso, Tania Mandina; Marcon, Francesca; Marcos, Ricard; Moretti, Massimo; Moretti, Silvia; Najafzadeh, Mojgan; Nemeth, Zsuzsanna; Neri, Monica; Novotna, Bozena; Orlow, Irene; Paduchova, Zuzana; Pastor, Susana; Perdry, Hervé; Spremo-Potparević, Biljana; Ramadhani, Dwi; Riso, Patrizia; Rohr, Paula; Rojas, Emilio; Rossner, Pavel; Safar, Anna; Sardas, Semra; Silva, Maria João; Sirota, Nikolay; Smolkova, Bozena; Staruchova, Marta; Stetina, Rudolf; Stopper, Helga; Surikova, Ekaterina I.; Ulven, Stine Marie; Ursini, Cinzia Lucia; Valdiglesias, Vanessa; Valverde, Mahara; Vodička, Pavel; Volkovova, Katarina; Wagner, Karl-Heinz; Zivkovic, Lada; Dusinska, Maria; Collins, Andrew Richard; Bonassi, Stefano

The alkaline comet assay, or single cell gel electrophoresis, is one of the most popular methods for assessing DNA damage in human population. One of the open issues concerning this assay is the identification of those factors that can explain the large inter-individual and inter-laboratory variation. International collaborative initiatives such as the hCOMET project - a COST Action launched in 2016 - represent a valuable tool to meet this challenge. The aims of hCOMET were to establish reference values for the level of DNA damage in humans, to investigate the effect of host factors, lifestyle and exposure to genotoxic agents, and to compare different sources of assay variability. A database of 19,320 subjects was generated, pooling data from 105 studies run by 44 laboratories in 26 countries between 1999 and 2019. A mixed random effect log-linear model, in parallel with a classic meta-analysis, was applied to take into account the extensive heterogeneity of data, due to descriptor, specimen and protocol variability. As a result of this analysis interquartile intervals of DNA strand breaks (which includes alkali-labile sites) were reported for tail intensity, tail length, and tail moment (comet assay descriptors). A small variation by age was reported in some datasets, suggesting higher DNA damage in oldest age-classes, while no effect could be shown for sex or smoking habit, although the lack of data on heavy smokers has still to be considered. Finally, highly significant differences in DNA damage were found for most exposures investigated in specific studies. In conclusion, these data, which confirm that DNA damage measured by the comet assay is an excellent biomarker of exposure in several conditions, may contribute to improving the quality of study design and to the standardization of results of the comet assay in human populations.

2021

Nedstenging lite å si for utslipp

Platt, Stephen Matthew (intervjuobjekt); Grønning, Trygve (journalist)

2021

Ett år uten et av Norges største miljøproblem: – Mer insekter, null svovelstank

Berglen, Tore Flatlandsmo; Aspholm, Paul Eric (intervjuobjekter); Andreassen, Erik; Kalinina, Kristina (journalister)

2021

Grenseområdene Norge-Russland. Luft- og nedbørkvalitet 2020.

Berglen, Tore Flatlandsmo; Nilsen, Anne-Cathrine; Våler, Rita Larsen; Vadset, Marit; Uggerud, Hilde Thelle; Hak, Claudia; Andresen, Erik

Smelteverkene i nordvest-Russland slapp ut store mengder svoveldioksid (SO2) og tungmetaller. Utslippene påvirket luft- og nedbørkvalitet i grenseområdene. Miljøovervåkingen viser at grenseverdier for SO2 er overholdt i kalenderåret 2020, samt for vinter 2019/20. Smelteverket i Nikel stengte ned 23. desember 2020 og dette er ventet å gi stor nedgang i
forurensningen i grenseområdene. Målsettingsverdier for Ni, As og Cd er overholdt.

NILU

2021

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