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Air pollution emission inventory using national high-resolution spatial parameters for the Nordic countries and analysis of PM2.5 spatial distribution for road transport and machinery and off-road sectors

Paunu, Ville-Veikko; Karvosenoja, Niko; Segersson, David; Lopez-Aparicio, Susana; Nielsen, Ole-Kenneth; Plejdrup, Marlene S.; Thorsteinsson, Throstur; Vo, Dam Thanh; Kuenen, Jeroen; Gon, Hugo Denier van der; Jalkanen, Jukka-Pekka; Brandt, Jørgen; Geels, Camilla

Air pollution is an important cause of adverse health effects, even in the Nordic countries, which have relatively good air quality. Modelling-based air quality assessment of the health impacts relies on reliable model estimates of ambient air pollution concentrations, which furthermore rely on good-quality spatially resolved emission data. While quantitative emission estimates are the cornerstone of good emission data, description of the spatial distribution of the emissions is especially important for local air quality modelling at high resolution. In this paper we present a new air pollution emission inventory for the Nordic countries with high-resolution spatial allocation (1 km × 1 km) covering the years 1990, 1995, 2000, 2005, 2010, 2012, and 2014. The inventory is available at https://doi.org/10.5281/zenodo.10571094 (Paunu et al., 2023). To study the impact of applying national data and methods to the spatial distribution of the emissions, we compared road transport and machinery and off-road sectors to CAMS-REGv4.2, which used a consistent spatial distribution method throughout Europe for each sector. Road transport is a sector with well-established proxies for spatial distribution, while for the machinery and off-road sector, the choice of proxies is not as straightforward as it includes a variety of different type of vehicles and machines operating in various environments. We found that CAMS-REGv4.2 was able to produce similar spatial patterns to our Nordic inventory for the selected sectors. However, the resolution of our Nordic inventory allows for more detailed impact assessment than CAMS-REGv4.2, which had a resolution of 0.1° × 0.05° (longitude–latitude, roughly 5.5 km × 3.5–6.5 km in the Nordic countries). The EMEP/EEA Guidebook chapter on spatial mapping of emissions has recommendations for the sectoral proxies. Based on our analysis we argue that the guidebook should have separate recommendations for proxies for several sub-categories of the machinery and off-road sectors, instead of including them within broader sectors. We suggest that land use data are the best starting point for proxies for many of the subsectors, and they can be combined with other suitable data to enhance the spatial distribution. For road transport, measured traffic flow data should be utilized where possible, to support modelled data in the proxies.

2024

Air Pollution by Ozone Across Europe. The Handbook of Environmental Chemistry, vol. 26

Derwent, R.G.; Hjellbrekke, A.-G.

2013

Air pollution

Krogseth, Ingjerd Sunde

2019

Air policy

King, Peter; Armah, Frederick Ato; Dickerson, Phillip; Guerreiro, Cristina; Keating, Terry; Lucon, Oswaldo dos Santos; Miyazaki, Asami; Patel, Amit; Reis, Stefan

2019

Air monitoring at the Trollhaugen Observatory in Antarctica

Aas, Wenche; Eckhardt, Sabine; Evangeliou, Nikolaos; Fiebig, Markus; Halse, Anne Karine; Hansen, Georg H.; Lunder, Chris Rene; Myhre, Cathrine Lund; Bohlin-Nizzetto, Pernilla; Pfaffhuber, Katrine Aspmo; Platt, Stephen Matthew; Schmidbauer, Norbert; Solberg, Sverre; Svendby, Tove Marit; Yttri, Karl Espen

2020

Air measurements of linear and cyclic volatile methyl siloxanes along a transect between Portugal and Norway.

Cincinelli, A.; Pieri, F.; Martellini, T.; Ratola, N.; Katsoyiannis, A.; Del Vento, S.; Schuster, J.K.; Jones, K.C.

2012

Air implementation pilot: Workshop on measures, Copenhagen, February 27th 2013. ETC/ACM Technical Paper, 2013/5

Viana, M.; Castell, N.; Doering, U.; de Leeuw, F.; Malherbe, L.; Nagl, C.; Rouil, L.; Guerreiro, C.; Ruyssenaars, P.; Ortiz, A.G.

2013

Air implementation pilot: Management practices (update 2013). ETC/ACM Technical Paper, 2013/7

Castell, N.; Guerreiro, C.

2013

Air implementation pilot: Assessing the modelling activities. ETC/ACM Technical Paper, 2013/4

Castell, N.; Denby, B.R.; Guerreiro, C.

2013

Air implementation pilot- Lessons learnt from the implementation of air quality legislation at urban level. EEA report, 7/2013

González Ortiz, A.; Mourelatou, A.; Schilling J.; Verheye, T.; Brockett, S.; Buzica, D.; Arduino G.; de Wilt W.; Castell, N.; Nagl, C.; Malherbe, L.; de Leeuw, F.; Targa, J.; Viana, M.; Döring, U.; Rouïl, L.; Guerreiro, C.; Tarrasón, L.

2013

Air exposures: Making children aware. Two Norwegian campaigns. NILU PP

Innset, B.; Endregard, G.; Tønnesen, D.; Bartonova, A.; Sandås, A.; Lauvanger, E.G.

2005

Air concentrations and wet deposition of major inorganic ions at five non-urban sites in China, 2001-2003.

Aas, W.; Shao, M.; Jin, L.; Larssen, T.; Zhao, D.; Xiang, R.; Zhang, J.; Xiao, J.; Duan, L.

2007

Air concentrations and wet deposition of major inorganic ions at five non-urban sites in China, 2001-2003 (part I). NILU PP

Aas, W.; Shao, M.; Jin, L.; Larssen, T.; Zhao, D.; Xiang, R.; Zhang, J.; Xiao, J.

2005

Air

Dickinson, Philip; Guerreiro, Cristina; Keating, Terry; Nzioka, John M.; Chung, Serena H.; Reis, Stefan

2019

AI-driven spatiotemporal quantification and prediction of soil salinity at European scale using the LUCAS database

Zarif, Mohammad Aziz; Hassani, Amirhossein; Panagos, Panos; Lebron, Inma; Robinson, David A.; Shokri, Nima

2024

AI-driven insights into soil health and soil degradation in Europe in the face of climate and anthropogenic challenges

Afshar, Mehdi H.; Hassani, Amirhossein; Aminzadeh, Milad; borrelli, Pasquale; Panagos, Panos; Robinson, David A.; Shokri, Nima

2024

Aging of Tire Particles in Deep-Sea Conditions: Interactions between Hydrostatic Pressure, Prokaryotic Growth and Chemical Leaching

Schmidt, Natascha; Foscari, Aurelio; Herzke, Dorte; Garel, Marc; Tamburini, Christian; Seiwert, Bettina; Reemtsma, Thorsten; Sempéré, Richard

Tire particles can enter the marine environment e.g. through direct discharge of road runoff, sewage systems or riverine inputs. Their fate in marine waters remains largely unknown, though the deep sea could be a final sink as for other marine litter. To simulate these conditions, we investigated in laboratory-controlled conditions the effects of high-hydrostatic pressure [20 MPa] vs atmospheric pressure [0.1 MPa] on the leaching of 17 organic compounds from cryo-milled tire tread particles (μm sized) and crumb rubber particles (mm sized) into natural seawater. We monitored the abundance of heterotrophic prokaryotes in the leachates over the 14 day exposure period under biotic conditions. Abiotic controls were employed to delineate the influence of prokaryotes on the fate of leached chemicals. Our results showed leaching of dissolved organic carbon and target chemicals under all experimental conditions, with higher concentrations of certain target chemicals under high-hydrostatic pressure conditions (e.g., 1,3-diphenylguanidine [DPG]: max. 703 (20 MPa) vs 119 μg/L (0.1 MPa) from cryo-milled tire tread particles under biotic conditions). Under abiotic conditions leaching was weaker for DPG and other chemicals, with contrasting trends for chemicals prone to biotransformation. In crumb rubber leachates chemical concentrations increased with time, but showed no significant differences between biotic/abiotic or high-hydrostatic/atmospheric pressure conditions. Prokaryotic abundance increased in all samples containing tire particles compared to seawater controls, indicating the use of the rubber and/or leached chemicals as an energy source.

2025

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