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The influence of vegetation drought stress on formaldehyde and ozone distributions over a central European city

Trimmel, Heidelinde; Hamer, Paul David; Mayer, Monika; Schreier, Stefan F.; Weihs, Philipp; Eitzinger, Josef; Sandén, Hans; Fitzky, Anne Charlott; Richter, Andreas; Calvet, Jean-Christophe; Bonan, Bertrand; Meurey, Catherine; Vallejo, Islen; Eckhardt, Sabine; Sousa Santos, Gabriela; Oumami, Safae; Arteta, Joaquim; Marécal, Virginie; Tarrasón, Leonor; Karl, Thomas; Rieder, Harald E.

To estimate the effect of vegetation stress and changes in biogenic volatile organic compound (BVOC) emissions on urban ozone (O3) levels we perform a systematic, observation-based analysis of the relationship between formaldehyde (HCHO) mixing ratios, meteorological parameters, measurement-based drought indicators and O3 over the central European city of Vienna, Austria. In addition, numerical models SURface EXternalisée (SURFEX), Model of Emissions of Gases and Aerosols from Nature (MEGAN) Vers.2.1 and 3 and MOdèle de Chimie A Grande Echelle (MOCAGE) are combined to estimate the soil moisture, the spatial distribution and drought response of isoprene emissions, and the resulting distribution of HCHO in the atmosphere. To analyse the effect of drought during spring and summer we contrast observations during dry and reference years. Our results show that the observed HCHO can be explained using the simulated isoprene emissions as well as observed and simulated vegetation drought responses. HCHO mixing ratios differ strongly between dry and reference seasons. Spring-time precipitation deficits facilitate reduced HCHO mixing ratios due to delayed and weakened plant growth. In consequence also O3 burdens are lowered due to reduced BVOC precursor emissions. These reductions occur despite radiation levels being higher than during the reference year, illustrating the strong potential of spring-time BVOC emissions to modulate urban O3 burdens. Conversely, during summer elevated O3 levels occur during local drought conditions. These are driven by advected isoprene originating from nearby forest areas, which are not affected by drought. Our results regarding elevated summer-time O3 burdens under vegetation heat and drought stress are in good agreement with previous work.

Elsevier

2023

The Integrated Carbon Observation System in Europe

Heiskanen, Jouni; Brümmer, Christian; Buchmann, Nina; Calfapietra, Carlo; Chen, Huilin; Gielen, Bert; Gkritzalis, Thanos; Hammer, Samuel; Hartman, Susan; Herbst, Mathias; Janssens, Ivan A.; Jordan, Armin; Juurola, Eija; Karstens, Ute; Kasurinen, Ville; Kruijt, Bart; Lankreijer, Harry; Levin, Ingeborg; Linderson, Maj-Lena; Loustau, Denis; Merbold, Lutz; Myhre, Cathrine Lund; Papale, Dario; Pavelka, Marian; Pilegaard, Kim; Ramonet, Michel; Rebmann, Corinna; Rinne, Janne; Rivier, Leonard; Saltikoff, Elena; Sanders, Richard; Steinbacher, Martin; Steinhoff, Tobias; Watson, Andrew; Vermeulen, Alex T.; Vesala, Timo; Vitkova, Gabriela; Kutsch, Werner

Since 1750, land use change and fossil fuel combustion has led to a 46 % increase in the atmospheric carbon dioxide (CO2) concentrations, causing global warming with substantial societal consequences. The Paris Agreement aims to limiting global temperature increases to well below 2°C above pre-industrial levels. Increasing levels of CO2 and other greenhouse gases (GHGs), such as methane (CH4) and nitrous oxide (N2O), in the atmosphere are the primary cause of climate change. Approximately half of the carbon emissions to the atmosphere is sequestered by ocean and land sinks, leading to ocean acidification but also slowing the rate of global warming. However, there are significant uncertainties in the future global warming scenarios due to uncertainties in the size, nature and stability of these sinks. Quantifying and monitoring the size and timing of natural sinks and the impact of climate change on ecosystems are important information to guide policy-makers’ decisions and strategies on reductions in emissions. Continuous, long-term observations are required to quantify GHG emissions, sinks, and their impacts on Earth systems. The Integrated Carbon Observation System (ICOS) was designed as the European in situ observation and information system to support science and society in their efforts to mitigate climate change. It provides standardized and open data currently from over 140 measurement stations across 12 European countries. The stations observe GHG concentrations in the atmosphere and carbon and GHG fluxes between the atmosphere, land surface and the oceans. This article describes how ICOS fulfills its mission to harmonize these observations, ensure the related long-term financial commitments, provide easy access to well-documented and reproducible high-quality data and related protocols and tools for scientific studies, and deliver information and GHG-related products to stakeholders in society and policy.

American Meteorological Society

2021

The Kongsfjorden system - a flagship programme for Ny-Ålesund. A concluding document from Workshop 28-31 March, 2008. Kortrapport 11/2009

Gabrielsen, G.W.; Hop, H.; Hübner, C.; Kallenborn, R.; Weslawski, J.M.; Wiencke, C. (eds.)

2009

The Kyoto Protocol: climate change.

Reimann, S.; Stordal, F. with contrib. from Ciais, P.; Goede, A.; Lazaridis, M.; Mazière, M. De, Zander, R.

2004

The Lagrangian particle dispersion model FLEXPART version 10.

Pisso, I.; Sollum, E.; Grythe, H.; Kristiansen, N.; Cassiani, M.; Eckhardt, S.; Thompson, R.; Zwaaftnik, C. G.; Evangeliou, N.; Hamburger, T.; Sodemann, H.; Haimberger, L.; Henne, S.; Brunner, D.; Burkhart, J.; Fouilloux, A.; Fang, X.; Phillip, A.; Seibert, P.; Stohl, A.

2017

The Lagrangian particle dispersion model FLEXPART version 10.4

Pisso, Ignacio; Sollum, Espen; Grythe, Henrik; Kristiansen, Nina Iren; Cassiani, Massimo; Eckhardt, Sabine; Arnold, Delia; Morton, Don; Thompson, Rona Louise; Zwaaftink, Christine Groot; Evangeliou, Nikolaos; Sodemann, Harald; Haimberger, Leopold; Henne, Stephan; Brunner, Dominik; Burkhart, John; Fouilloux, Anne Claire; Brioude, Jerome; Philipp, Anne; Seibert, Petra; Stohl, Andreas

2019

The Lagrangian particle dispersion model FLEXPART version 10.4

Pisso, Ignacio; Sollum, Espen; Grythe, Henrik; Kristiansen, Nina Iren; Cassiani, Massimo; Eckhardt, Sabine; Arnold, Delia; Morton, Don; Thompson, Rona Louise; Zwaaftink, Christine Groot; Evangeliou, Nikolaos; Sodemann, Harald; Haimberger, Leopold; Henne, Stephan; Brunner, Dominik; Burkhart, John; Fouilloux, Anne Claire; Brioude, Jerome; Philipp, Anne; Seibert, Petra; Stohl, Andreas

2020

The Lagrangian particle dispersion model FLEXPART-WRF version 3.1.

Brioude, J.; Arnold, D.; Stohl, A.; Cassiani, M.; Morton, D.; Seibert, P.; Angevine, W.; Evan, S.; Dingwell, A.; Fast, J. D.; Easter, R. C.; Pisso, I.; Burkhart, J.; Wotawa, G.

2013

The libRadtran software package for radiative transfer calculations (version 2.0.1).

Emde, C.; Buras-Schnell, R.; Kylling, A.; Mayer, B.; Gasteiger, J.; Hamann, U.; Kylling, J.; Richter, B.; Pause, C.; Dowling, T.; Bugliaro, L.

2016

The link between springtime total ozone and summer UV radiation in Northern Hemisphere extratropics.

Karpechko, A.Yu.; Backman, L.; Thölix, L.; Ialongo, I.; Andersson, M.; Fioletov, V.; Heikkilä, A.; Johnsen, B.; Koskela, T.; Kyrölä, E.; Lakkala, K.; Myhre, C.L.; Rex, M.; Sofieva, V.F.; Tamminen, J.; Wohltmann, I.

2013

The magnitude, trend and drivers of the global nitrous oxide budget: a new assessment

Tian, Hanqin; Thompson, Rona Louise; Xu, Rongting; Canadell, Josep G.; Davidson, Eric A.; Ciais, Philippe; Jackson, Robert B.; Winiwarter, Wilfried; Suntharalingam, Parvadha; Regnier, Pierre; Zhou, Feng; Janssens-Maenhout, Greet; Arneth, Almut; Li, Wei; Pan, Naiqing; Pan, Shufen; Prather, Michael J.; Raymond, Peter A.; Shi, Hao; GCP/INI Synthesis Team, *

2019

The mass flow and proposed management of bisphenol A in selected Norwegian waste streams.

Arp, H. P. H.; Morin, N. A. O.; Hale, S. E.; Okkenhaug, G.; Breivik, K.; Sparrevik, M.

2017

The MEMORI dosimeter - a user friendly tool for evaluation of indoor air quality for cultural heritage. NILU F

Grøntoft, T.; Wittstadt, K.; Bellendorf, P.; Dahlin, E.; Håland, S.; Bernardo, C.; Ødegård, R.; Røen, H.V.; Heltne, T.

2012

The MEMORI dosimeter - a user friendly tool for evaluation of indoor air quality for cultural heritage. NILU OR

Grøntoft, T.; Wittstadt, K.; Bellendorf, P.; Dahlin, E.; Håland, S.; Bernardo, C.; Ødegård, R.; Røen, H.V.; Heltne, T.

2012

The MEMORI dosimeter for indoor environment.

Dahlin, E.; Grøntoft, T.; Lopez-Aparicio, S.; Bellendorf, P.; Wittstadt, Schieweck, A.; Drda-Kühn, K.; Perla Colombini, M.; Bonaduce, I.; Vandenabeele, P.; Larsen, R.; Poulsen Sommer, D.V.; Potthast, A.; Marincas, O.; Thickett, D.; Andrade, G.; Tabuenca, A.; Odlyha, M.; Hackney, S.; Laurenson, P.; McDonagh, C.; Ackerman, J.J.

2012

The MEMORI dosimeter for indoor environment. NILU PP

Dahlin, E.; Grøntoft, T.; Lopez-Aparicio, S.; Bellendorf, P.; Wittstadt, Schieweck, A.; Drda-Kühn, K.; Perla Colombini, M.; Bonaduce, I.; Vandenabeele, P.; Larsen, R.; Poulsen Sommer, D.V.; Potthast, A.; Marincas, O.; Thickett, D.; Andrade, G.; Tabuenca, A.; Odlyha, M.; Hackney, S.; Laurenson, P.; McDonagh, C.; Ackerman, J.J.

2012

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