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Precise estimation of atmospheric pollutant releases is crucial for assessing the impact of environmental accidents. Atmospheric inversion typically relies on a linear model with a source–receptor sensitivity (SRS) matrix, which may contain significant errors or even completely fail to capture the real magnitude of the event. We propose a correction of the SRS matrix formulated as slight shifts in the observation locations, effectively warping the sensitivity field. To constrain these shifts and ensure data-driven corrections, we model them using a Gaussian process prior. This prior not only enforces smoothness and sparsity, but also enables posterior prediction of shifts at previously unseen locations. This key feature provides a mechanism for hyper-parameter tuning: the predicted shift field can be visualized on a map and assessed by an expert. We present a user-friendly framework that combines a Bayesian inversion model with correction and a tuning algorithm based on L-curve-like plots and the maps of predicted shifts. The proposed method is demonstrated on three case studies: the ETEX-I experiment, the 137Cs emissions during the 2020 Chernobyl wildfires, and the 106Ru release in 2017.
2026
Understanding new particle formation (NPF) and the fate of nanoparticles is crucial because of their close links to air quality, cloud formation, and climate. These effects vary spatially and temporally owing to diverse aerosol sources and their relatively short atmospheric lifetime. Here, we present a comprehensive analysis of long-term trends in NPF-associated nucleation-mode particles and cloud condensation nuclei (CCN) concentrations across diverse observation environments using quality-controlled particle number size distribution (PNSD) and CCN data from 37 sites, primarily from Global Atmosphere Watch (GAW) stations. We identify declining decadal trends in both NPF occurrences and nucleated particle concentrations across most site types, with the strongest declines in urban areas. We observe simultaneous reductions in both CCN concentrations and nucleation-mode particles, suggesting that newly formed particles are a potential source of CCN. This, in turn, suggests that cloud microphysical properties and radiative effects can be indirectly influenced through aerosol–cloud interactions that modify cloud droplet formation. These findings indicate that decreasing anthropogenic emissions could influence the climate forcing potential of aerosol–cloud interactions, with important implications for future climate projections.
2026
ML-based data fusion of model, satellite, and ground observations for 1-km PM2.5 mapping over Europe
2026
Arctic Amplification is not well understood. It is the result of a complicated interplay between remote and local forcing and feedback processes. Therefore, it is crucial to enhance our understanding of the transport of energy and moisture from lower latitudes. The amount of aerosol in the Arctic is also an important quantity as their role in Arctic Amplification, via direct radiative forcing and aerosol-cloud interactions, remain poorly quantified.In this work, we aim to better quantify how aerosols, energy, and moisture are transported to and distributed within the Arctic. We investigate observations at Arctic stations, including, Villum and Zeppelin, and perform backward-in-time simulations with the Lagrangian atmospheric transport model FLEXPART (Pisso et al., 2019; Bakels et al., 2024) to derive so-called emission sensitivities and use these sensitivities to better quantify source regions of aerosols, energy, and moisture.In general, we aim to better describe the spatial and temporal atmospheric transport characteristics into the Arctic and how these characteristics have changed in recent years. We focus on the transport during warm-air intrusions, since almost 30% of the total poleward transport of moisture (during winter) occurs during such events (Woods et al., 2013). Warm-air intrusions are often associated with large-scale atmospheric blocking patterns forcing a change in transport direction from east to more poleward, bringing warm, moist, and cloudy air into the Arctic. Warm-air intrusions can also be favourable for an enhanced transport of aerosols (e.g., Dada et al., 2022).Since climate models show large biases in moisture flux during these events (Woods et al., 2017), there is clearly a need to better quantify the transport of moisture, energy, and aerosols during these events. This will also help to provide better forcing for climate simulations.Bakels et al. (2024): 10.5194/gmd-17-7595-2024; Dada et al. (2022): 10.1038/s41467-022-32872-2; Lapere et al. (2024): 10.1029/2023JD039606; Pisso et al. (2019): 10.5194/gmd-12-4955-2019; Woods et al. (2013): 10.1002/grl.50912; Woods et al. (2017): 10.1175/JCLI-D-16-0710.
2026
2026
2026