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Indian Land Carbon Sink Estimated from Surface and GOSAT Observations

Nayagam, Lorna Raja; Maksyutov, Shamil; Janardanan, Rajesh; Oda, Tomohiro; Tiwari, Yogesh K.; Sreenivas, Gaddamidi; Datye, Amey; Jain, Chaithanya D.; Ratnam, Madineni Venkat; Sinha, Vinayak; Hakkim, Haseeb; Terao, Yukio; Naja, Manish; Ahmed, Md. Kawser; Mukai, Hitoshi; Zeng, Jiye; Kaiser, Johannes; Someya, Yu; Yoshida, Yukio

The carbon sink over land plays a key role in the mitigation of climate change by removing carbon dioxide (CO2) from the atmosphere. Accurately assessing the land sink capacity across regions should contribute to better future climate projections and help guide the mitigation of global emissions towards the Paris Agreement. This study estimates terrestrial CO2 fluxes over India using a high-resolution global inverse model that assimilates surface observations from the global observation network and the Indian subcontinent, airborne sampling from Brazil, and data from the Greenhouse gas Observing SATellite (GOSAT) satellite. The inverse model optimizes terrestrial biosphere fluxes and ocean-atmosphere CO2 exchanges independently, and it obtains CO2 fluxes over large land and ocean regions that are comparable to a multi-model estimate from a previous model intercomparison study. The sensitivity of optimized fluxes to the weights of the GOSAT satellite data and regional surface station data in the inverse calculations is also examined. It was found that the carbon sink over the South Asian region is reduced when the weight of the GOSAT data is reduced along with a stricter data filtering. Over India, our result shows a carbon sink of 0.040 ± 0.133 PgC yr−1 using both GOSAT and global surface data, while the sink increases to 0.147 ± 0.094 PgC yr−1 by adding data from the Indian subcontinent. This demonstrates that surface observations from the Indian subcontinent provide a significant additional constraint on the flux estimates, suggesting an increased sink over the region. Thus, this study highlights the importance of Indian sub-continental measurements in estimating the terrestrial CO2 fluxes over India. Additionally, the findings suggest that obtaining robust estimates solely using the GOSAT satellite data could be challenging since the GOSAT satellite data yield significantly varies over seasons, particularly with increased rain and cloud frequency.

MDPI

2025

Increasing Trends of Legacy and Emerging Organic Contaminants in a Dated Sediment Core From East-Africa

Nipen, Maja; Vogt, Rolf David; Bohlin-Nizzetto, Pernilla; Borgå, Katrine; Mwakalapa, Eliezer Brown; Borgen, Anders Røsrud; Schlabach, Martin; Christensen, Guttorm; Mmochi, Aviti John; Breivik, Knut

Temporal trends of industrial organic contaminants can show how environmental burdens respond to changes in production, regulation, and other anthropogenic and environmental factors. Numerous studies have documented such trends from the Northern Hemisphere, while there is very limited data in the literature from sub-Saharan Africa. We hypothesized that the temporal trends of legacy and contemporary industrial contaminants in sub-Saharan Africa could greatly differ from the regions in which many of these chemicals were initially produced and more extensively used. For this purpose, a dated sediment core covering six decades from a floodplain system in urban Dar es Salaam, Tanzania, was analysed. The samples were analysed for selected legacy persistent organic pollutants (POPs) [polychlorinated biphenyls (PCBs) and polybrominated biphenyl ethers (PBDEs)] and chemicals of emerging concern (CECs) [alternative brominated flame retardants (aBFRs), chlorinated paraffins (CPs), and dechloranes]. All groups of chemicals showed a steep increase in concentrations towards the uppermost sediment layers reflecting the more recent years. Concentrations of the individual compound groups in surface sediment were found in the order CPs >> aBFRs ∼ ∑25PBDEs > dechloranes ∼ ∑32PCBs. Time trends for the individual compounds and compound groups differed, with ∑32PCBs showing presence in sediments since at least the early 1960s, while some CECs first occurred in sediments corresponding to the last decade. Investigations into potential drivers for the observed trends showed that socioeconomic factors related to growth in population, economy, and waste generation have contributed to increasing concentrations of PBDEs, aBFRs, CPs, and Dechlorane Plus. Further monitoring of temporal trends of industrial organic contaminants in urban areas in the Global South is recommended.

Frontiers Media S.A.

2022

Increasing Trends of Legacy and Emerging Organic Contaminants in a Dated Sediment Core From East-Africa

Nipen, Maja; Vogt, Rolf David; Bohlin-Nizzetto, Pernilla; Borgå, Katrine; Mwakalapa, Eliezer; Borgen, Anders; Schlabach, Martin; Christensen, Guttorm; Mmochi, Aviti; Breivik, Knut

2022

Increasing springtime ozone mixing ratios in the free troposphere over western North America.

Cooper, O.R.; Parrish, D.D.; Stohl, A.; Trainer, M.; Nédeléc, P.; Thouret, V.; Cammas, J.P.; Oltmans, S.J.; Johnson, B.J.; Tarasick, D.; Leblanc, T.; McDermid, I.S.; Jaffe, D.; Gao, R.; Stith, J.; Ryerson, T.; Aikin, K.; Campos, T.; Weinheimer, A.; Avery, M.A.

2010

Increases in global and East Asian nitrogen trifluoride (NF3) emissions inferred from atmospheric observations and GEOS-Chem

Liu, Yu; Sheng, Jianxiong; Rigby, Matthew; Ganesan, Anita L.; Kim, Jooil; Western, Luke M.; Muhle, Jens; Park, Sunyoung; Park, Hyeri; Weiss, Ray F. ; Salameh, Peter K.; O'Doherty, Simon; Young, Dickon; Krummel, Paul B.; Vollmer, Martin K.; Reimann, Stefan; Lunder, Chris Rene; Prinn, Ronald G.

2024

Increases in Global and East Asian Nitrogen Trifluoride (NF3) Emissions Inferred from Atmospheric Observations

Liu, Yu; Sheng, Jianxiong; Rigby, Matthew; Ganesan, Anita L.; Kim, Jooil; Western, Luke M.; Mühle, Jens; Park, Sunyoung; Park, Hyeri; Weiss, Ray F. ; Salameh, Peter K.; O'Doherty, Simon; Young, Dickon; Krummel, Paul B. ; Vollmer, Martin K.; Reimann, Stefan; Lunder, Chris Rene; Prinn, Ronald G.

Nitrogen trifluoride (NF3) is a potent and long-lived greenhouse gas that is widely used in the manufacture of semiconductors, photovoltaic cells, and flat panel displays. Using atmospheric observations from eight monitoring stations from the Advanced Global Atmospheric Gases Experiment (AGAGE) and inverse modeling with a global 3-D atmospheric chemical transport model (GEOS-Chem), we quantify global and regional NF3 emission from 2015 to 2021. We find that global emissions have grown from 1.93 ± 0.58 Gg yr–1 (± one standard deviation) in 2015 to 3.38 ± 0.61 Gg yr–1 in 2021, with an average annual increase of 10% yr–1. The available observations allow us to attribute significant emissions to China (0.93 ± 0.15 Gg yr–1 in 2015 and 1.53 ± 0.20 Gg yr–1 in 2021) and South Korea (0.38 ± 0.07 Gg yr–1 to 0.65 ± 0.10 Gg yr–1). East Asia contributes around 73% of the global NF3 emission increase from 2015 to 2021: approximately 41% of the increase is from emissions from China (with Taiwan included), 19% from South Korea, and 13% from Japan. For Japan, which is the only one of these three countries to submit annual NF3 emissions to UNFCCC, our bottom-up and top-down estimates are higher than reported. With increasing demand for electronics, especially flat panel displays, emissions are expected to further increase in the future.

2024

Increased soil N2O emissions from the Arctic-Boreal region: A non-negligible non-carbon climate feedback

Pan, Naiqing; Tian, Hanqin; Pan, Shufen; Shi, Hao; Canadell, Josep G; Chang, Jinfeng; Ciais, Philippe; Davidson, Eric A.; Hugelius, Gustaf; Ito, Akihiko; Jackson, Robert B.; Joos, Fortunat; Millet, Dylan B.; Olin, Stefan; Patra, Prabir K.; Thompson, Rona Louise; Wells, Kelley C.; Wilson, Chris J.; Zaehle, Sönke

2021

Increased nitrous oxide emissions in East Asia as estimated by bottom-up and top-down approaches

Pan, Naiqing; Xu, Rongting; Pan, Shufen; Thompson, Rona Louise; Canadell, Josep G.; Jackson, Robert B.; Winiwarter, Wilfried; Zhou, Feng

2019

Increased contribution of biomass burning to haze events in Shanghai since China’s clean air actions

Fang, Wenzheng; Evangeliou, Nikolaos; Eckhardt, Sabine; Xing, Ju; Zhang, Hailong; Xiao, Hang; Zhao, Meixun; Kim, Sang-Woo

High levels of East Asian black carbon (BC) aerosols affect ecological and environmental sustainability and contribute to climate warming. Nevertheless, the BC sources in China, after implementing clean air actions from 2013‒2017, are currently elusive due to a lack of observational constraints. Here we combine dual-isotope-constrained observations and chemical-transport modelling to quantify BC’s sources and geographical origins in Shanghai. Modelled BC concentrations capture the overall source trend from continental China and the outflow to the Pacific. Fossil sources dominate (~70%) BC in relatively clean summer. However, a striking increase in biomass burning (15‒30% higher in a fraction of biomass burning compared to summer and 2013/2014 winter), primarily attributable to residential emissions, largely contributes to wintertime BC (~45%) pollution. It highlights the increasing importance of residential biomass burning in the recent winter haze associated with >65% emissions from China’s central-east corridor. Our results suggest clearing the haze problem in China’s megacities and mitigating climate impact requires substantial reductions in regional residential emissions, besides reducing urban traffic and industry emissions.

Springer Nature

2023

Increase in HFC-134a emissions in response to the success of the Montreal Protocol.

Fortems-Cheiney, A.; Saunois, M.; Pison, I.; Chevallier, F.; Bousquet, P.; Cressot, C.; Montzka, S.A.; Fraser, P.J.; Vollmer, M.K.; Simmonds, P.G.; Young, D,. O'Doherty, S.; Weiss, R.F.; Artuso, F.; Barletta, B.; Blake, D.R.; Li, S.; Lunder, C.; Miller, B.R.; Park, S.; Prinn, R.; Saito, T.; Steele, L P.; Yokouchi, Y.

2015

Inclusion of land cover and traffic data in NO2 mapping methodology. ETC/ACM Technical Paper, 2016/12

Horálek, J.; de Smet, P.; Schneider, P.; Kurfürst, P.; de Leeuw, F.

2017

Inception report. Support in development and implementation of air quality e-Reporting in West Balkan. NILU report

Ødegård, R. Å.; Kobernus, M. J.

The Norwegian Institute for Air Research (NILU), 4sfera Innova SLU (4sfera) and EKONERG have been commissioned to develop a solution for Air Quality e-Reporting for the West Balkan countries.

2016

iNANOD liposomes. Cyto- and genotoxicity testing.

Rundén-Pran, Elise; Hudecova, Alexandra Misci; Mariussen, Espen; Dusinska, Maria

NILU

2018

In-situ, satellite measurement and model evidence for the dominant regional contribution to fine particulate matter levels in the Paris Megacity.

Beekmann, M.; Prévôt, A. S. H.; Drewnick, F.; Sciare, J.; Pandis, S. N.; Denier van der Gon, H. A. C.; Crippa, M.; Freutel, F.; Poulain, L.; Ghersi, V.; Rodriguez, E.; Beirle, S.; Zotter, P.; von der Weiden-Reinmüller, S.-L.; Bressi, M.; Fountoukis, C.; Petetin, H.; Szidat, S.; Schneider, J.; Rosso, A.; El Haddad, I.; Megaritis, A.; Zhang, Q. J.; Michoud, V.; Slowik, J. G.; Moukhtar, S.; Kolmonen, P.; Stohl, A.; Eckhardt, S.; Borbon, A.; Gros, V.; Marchand, N.; Jaffrezo, J. L.; Schwarzenboeck, A.; Colomb, A.; Wiedensohler, A.; Borrmann, S.; Lawrence, M.; Baklanov, A.; Baltensperger, U.

2015

In-situ observation of Asian pollution transported into the Arctic lowermost stratosphere.

Roiger, A.; Schlager, H.; Schäfler, A.; Huntrieser, H.; Scheibe, M.; Aufmhoff, H.; Cooper, O. R.; Sodemann, H.; Stohl, A.; Burkhart, J.; Lazzara, M.; Schiller, C.; Law, K. S.; Arnold, F.

2011

In vivo Mammalian Alkaline Comet Assay: Method Adapted for Genotoxicity Assessment of Nanomaterials

Cardoso, Renato; Dusinska, Maria; Collins, Andrew Richard; Manjanatha, Mugamane; Pfuhler, Stefan; Registre, Marilyn; Elespuru, Rosalie K.

The in vivo Comet assay measures the generation of DNA strand breaks under conditions in which the DNA will unwind and migrate to the anode in an electrophoresis assay, producing comet-like figures. Measurements are on single cells, which allows the sampling of a diversity of cells and tissues for DNA damaging effects. The Comet assay is the most common in vivo method for genotoxicity assessment of nanomaterials (NM). The Method outlined here includes a recommended step-by-step approach, consistent with OECD 489, taking into consideration the issues impacting assessment of NM, including choice of cells or systems, handling of NM test articles, dose determination, assay methods and data assessment. This method is designed to be used along with the accompanying “Common Considerations” paper, which discusses issues common to any genotoxicity assay using NM as a test article.

Frontiers Media S.A.

2022

In vitro evaluation of the genotoxicity of poly(anhydride) nanoparticles designed for oral drug delivery.

Iglesias, T.; Dusinska, M.; El Yamani, N.; Irache, J. M.; Azqueta, A.; López de Cerain, A.

2017

In vitro cyto- and genotoxicity of CeO2, TiO2 and Ag nanoforms: the role of physical properties

Longhin, Eleonora Marta; Rios Mondragon, Ivan; Mariussen, Espen; Congying, Z.; Busquets, M.; Hofshagen, Ole-Bendik; Franco Puntes, V.; Cimpan, Mihaela-Roxana; Shaposhnikov, S.; Dusinska, Maria; Rundén-Pran, Elise

2023

In vitro approaches for assessing the genotoxicity of nanomaterials

Dusinska, Maria; Mariussen, Espen; Rundén-Pran, Elise; Hudecova, Alexandra Misci; Elje, Elisabeth; Kazimirova, Alena; El Yamani, Naouale; Dommershausen, Nils; Tharmann, Julian; Fieblinger, Dagmar; Herzberg, Frank; Luch, Andreas; Haase, Andrea

2019

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