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Observed recent change in climate and potential for decay of Norwegian wood structures

Grøntoft, Terje

The wood rot decay of structures and buildings in Norway represents high costs. This paper reports the observed trends for the potential rot decay of Norwegian wood structures in the cities of Oslo and Bergen over the recent 55 years, calculated as the “wood rot climate index” developed by Scheffer, and compares the reports with previous reported values based on climate change modelling. The observed change in the wood rot climate index was close to the modelling result. Bergen is exposed directly to the westerly Atlantic winds and has among the highest rain amounts in Norway, whereas Oslo is shielded by the Scandinavian mountain chain and has much less rain. The change in the wood rot climate index since 1961 was about 20% in both cities, but the trend in the index (climate index change per year) was about 80% stronger in Bergen. The absolute index changes were largest in the summer; then spring (50 to 60% of the summer increase); and small, zero, or even negative (autumn in Oslo) in the remaining seasons. The relative changes were higher in the spring than summer and very high in Bergen in the winter from a low value. The change to positive index values in the spring and winter indicates temperature and humidity conditions favoring the growth of wood rot and, thus, extended the rot duration through the year. The expected increase in the future wood rot decay potential in Norway shows the need for increased focus on adaption measures to reduce the related damages and costs.

2019

Individual variability in contaminants and physiological status in a resident Arctic seabird species

Eckbo, Norith; Bohec, Céline Le; Planas-Bielsa, Victor; Warner, Nicholas Alexander; Schull, Quentin; Herzke, Dorte; Zahn, Sandrine; Haarr, Ane; Gabrielsen, Geir W.; Borgå, Katrine

2019

Using life cycle assessment to inform municipal climate mitigation planning

Thorne, Rebecca Jayne; Bouman, Evert; Guerreiro, Cristina D.b.b.; Majchrzak, Anna; Calus, Sylwia

Local governments can play a key role in reducing emissions associated with local energy use. 17 Polish municipalities provided data on energy use and CO2 emissions for 2015. Life Cycle Assessment (LCA) was used to calculate lifecycle impact indicators for greenhouse gases, particulate matter, acidification and eutrophication associated with the annual energy demand in each municipality. Results showed that impacts from energy use increase almost proportionally with total energy used in the participating municipalities due to the heavy reliance on fossil fuels. Analysis of two municipalities of similar size showed that impacts can be attributed to different usage sectors. For one municipality, energy plans should focus on reducing emissions from private transport and associated fuel use. For the other, energy plans should focus on reducing energy demand from residential buildings. This means that a ‘one-size-fits-all’ energy plan, which may be developed at a national level, would not fit all municipalities. The application of LCA allows for identifying and informing energy planning with impact reduction potential for multiple environmental pressures. Analysis of the provided energy use and CO2 data showed large uncertainties in CO2 emission intensities and allowing for sufficient time and guidance in the energy and emissions accounting is recommended.

2019

Abating N in Nordic agriculture - Policy, measures and way forward

Hellsten, Sofie; Dalgaard, Tommy; Rankinen, Katri; Tørseth, Kjetil; Bakken, Lars; Bechmann, Marianne; Kulmala, Airi; Moldan, Filip; Olofsson, Stina; Piil, Kristoffer; Pira, Kajsa; Turtola, Eila

During the past twenty years, the Nordic countries (Denmark, Sweden, Finland and Norway) have introduced a range of measures to reduce losses of nitrogen (N) to air and to aquatic environment by leaching and runoff. However, the agricultural sector is still an important N source to the environment, and projections indicate relatively small emission reductions in the coming years.

The four Nordic countries have different priorities and strategies regarding agricultural N flows and mitigation measures, and therefore they are facing different challenges and barriers. In Norway farm subsidies are used to encourage measures, but these are mainly focused on phosphorus (P). In contrast, Denmark targets N and uses control regulations to reduce losses. In Sweden and Finland, both voluntary actions combined with subsidies help to mitigate both N and P.

The aim of this study was to compare the present situation pertaining to agricultural N in the Nordic countries as well as to provide recommendations for policy instruments to achieve cost effective abatement of reactive N from agriculture in the Nordic countries, and to provide guidance to other countries.

To further reduce N losses from agriculture, the four countries will have to continue to take different routes. In particular, some countries will need new actions if 2020 and 2030 National Emissions Ceilings Directive (NECD) targets are to be met. Many options are possible, including voluntary action, regulation, taxation and subsidies, but the difficulty is finding the right balance between these policy options for each country.

The governments in the Nordic countries should put more attention to the NECD and consult with relevant stakeholders, researchers and farmer's associations on which measures to prioritize to achieve these goals on time. It is important to pick remaining low hanging fruits through use of the most cost effective mitigation measures. We suggest that N application rate and its timing should be in accordance with the crop need and carrying capacity of environmental recipients. Also, the choice of application technology can further reduce the risk of N losses into air and waters. This may require more region-specific solutions and knowledge-based support with tailored information in combination with further targeted subsidies or regulations.

2019

Very Strong Atmospheric Methane Growth in the 4 Years 2014-2017: Implications for the Paris Agreement

Nisbet, E. G.; Manning, M. R.; Dlugokencky, E. J.; Fisher, R. E.; Lowry, D.; Michel, S. E.; Myhre, Cathrine Lund; Platt, Stephen Matthew; Allen, G.; Bousquet, P.; Brownlow, R.; Cain, M.; France, J. L.; Hermansen, Ove; Hossaini, R.; Jones, A. E.; Levin, I.; Manning, A. C.; Myhre, Gunnar; Pyle, J. A.; Vaughn, B.; Warwick, N. J.; White, James W. C.

Atmospheric methane grew very rapidly in 2014 (12.7 ± 0.5 ppb/year), 2015 (10.1 ± 0.7 ppb/year), 2016 (7.0 ± 0.7 ppb/year), and 2017 (7.7 ± 0.7 ppb/year), at rates not observed since the 1980s. The increase in the methane burden began in 2007, with the mean global mole fraction in remote surface background air rising from about 1,775 ppb in 2006 to 1,850 ppb in 2017. Simultaneously the 13C/12C isotopic ratio (expressed as δ13CCH4) has shifted, has shifted, now trending negative for more than a decade. The causes of methane's recent mole fraction increase are therefore either a change in the relative proportions (and totals) of emissions from biogenic and thermogenic and pyrogenic sources, especially in the tropics and subtropics, or a decline in the atmospheric sink of methane, or both. Unfortunately, with limited measurement data sets, it is not currently possible to be more definitive. The climate warming impact of the observed methane increase over the past decade, if continued at >5 ppb/year in the coming decades, is sufficient to challenge the Paris Agreement, which requires sharp cuts in the atmospheric methane burden. However, anthropogenic methane emissions are relatively very large and thus offer attractive targets for rapid reduction, which are essential if the Paris Agreement aims are to be attained.
PLAIN LANGUAGE SUMMARY: The rise in atmospheric methane (CH4), which began in 2007, accelerated in the past 4 years. The growth has been worldwide, especially in the tropics and northern midlatitudes. With the rise has come a shift in the carbon isotope ratio of the methane. The causes of the rise are not fully understood, and may include increased emissions and perhaps a decline in the destruction of methane in the air. Methane's increase since 2007 was not expected in future greenhouse gas scenarios compliant with the targets of the Paris Agreement, and if the increase continues at the same rates it may become very difficult to meet the Paris goals. There is now urgent need to reduce methane emissions, especially from the fossil fuel industry.

2019

Time trends of persistent organic pollutants in 30 year olds sampled in 1986, 1994, 2001 and 2007 in Northern Norway: measurements, mechanistic modeling and a comparison of study designs

Nøst, Therese Haugdahl; Berg, Vivian; Hanssen, Linda; Rylander, Charlotta; Gaudreau, Eric; Dumas, Pierre; Breivik, Knut; Sandanger, Torkjel M

<p><i>Background</i>: Human biomonitoring studies have demonstrated decreasing concentrations of many persistent organic pollutants (POPs) in years after emission peaks.</p> <p><i>Objectives</i>: To describe time trends of POPs in blood using four cross-sectional samples of 30 year olds from Tromsø, Norway across 1986–2007, and to compare the measured concentrations of polychlorinated biphenyl 153 (PCB-153) to model-estimated values. A second objective was to compare the repeated cross-sectional time trends with those observed in our previous longitudinal study using repeated individual measurements in older men from the same surveys.</p> <p><i>Methods</i>: Serum from 45 persons aged 30 years in each of the following years: 1986, 1994, 2001, and 2007 was analyzed for 14 POPs. Further, predicted concentrations of PCB-153 in each sampling year were derived using the emission-based CoZMoMAN model.</p> <p><i>Results</i>: The median decreases in summed serum POP concentrations (lipid-adjusted) in 1994, 2001, and 2007 relative to 1986 were − 71%, − 81%, and − 86% for women and − 65%, − 77%, and − 87% for men, respectively. The overall time trend in predicted PCB-153 concentrations demonstrated agreement with the observed trend although model predictions were higher than the measured concentrations at all time points. Compared to our previous longitudinal study of repeated individual measurements in older men, similar although more prominent declines were observed in the younger cross-sectional samples.</p> <p><i>Discussion</i>: Observed declines in serum concentrations from 1986 to 2007 were substantial for legacy POPs in men and women at reproductive ages in Northern Norway and are generally consistent with previous longitudinal biomonitoring efforts in the study population. The measured concentrations and observed declines likely reflect a combination of recent and historic exposures. Small differences in time trends observed between the studies could be attributed to different study designs (i.e. the chosen age group or sex and cross-sectional versus repeated individual measurement sampling).</p>

2019

The strength in numbers: comprehensive characterization of house dust using complementary mass spectrometric techniques

Rostkowski, Pawel; Haglund, Peter; Aalizadeh, Reza; Alygizakis, Nikiforos; Thomaidis, Nikolaos; Arandes, Joaquin Beltran; Bohlin-Nizzetto, Pernilla; Booij, Petra; Budzinski, Hélène; Brunswick, Pamela; Covaci, Adrian; Gallampois, Christine; Grosse, Sylvia; Hindle, Ralph; Ipolyi, Ildiko; Jobst, Karl; Kaserzon, Sarit; Leonards, Pim; Lestremau, Francois; Letzel, Thomas; Magnér, Jörgen; Matsukami, Hidenori; Moschet, Christoph; Oswald, Peter; Plassmann, Merle; Slobodnik, Jaroslav; Yang, Chun

Untargeted analysis of a composite house dust sample has been performed as part of a collaborative effort to evaluate the progress in the field of suspect and nontarget screening and build an extensive database of organic indoor environment contaminants. Twenty-one participants reported results that were curated by the organizers of the collaborative trial. In total, nearly 2350 compounds were identified (18%) or tentatively identified (25% at confidence level 2 and 58% at confidence level 3), making the collaborative trial a success. However, a relatively small share (37%) of all compounds were reported by more than one participant, which shows that there is plenty of room for improvement in the field of suspect and nontarget screening. An even a smaller share (5%) of the total number of compounds were detected using both liquid chromatography–mass spectrometry (LC-MS) and gas chromatography–mass spectrometry (GC-MS). Thus, the two MS techniques are highly complementary. Most of the compounds were detected using LC with electrospray ionization (ESI) MS and comprehensive 2D GC (GC×GC) with atmospheric pressure chemical ionization (APCI) and electron ionization (EI), respectively. Collectively, the three techniques accounted for more than 75% of the reported compounds. Glycols, pharmaceuticals, pesticides, and various biogenic compounds dominated among the compounds reported by LC-MS participants, while hydrocarbons, hydrocarbon derivatives, and chlorinated paraffins and chlorinated biphenyls were primarily reported by GC-MS participants. Plastics additives, flavor and fragrances, and personal care products were reported by both LC-MS and GC-MS participants. It was concluded that the use of multiple analytical techniques was required for a comprehensive characterization of house dust contaminants. Further, several recommendations are given for improved suspect and nontarget screening of house dust and other indoor environment samples, including the use of open-source data processing tools. One of the tools allowed provisional identification of almost 500 compounds that had not been reported by participants.

2019

Source apportionment of circum-Arctic atmospheric black carbon from isotopes and modeling

Winiger, P.; Barrett, T. E.; Sheesley, R. J.; Huang, L.; Sharma, S.; Barrie, L. A.; Yttri, Karl Espen; Evangeliou, Nikolaos; Eckhardt, Sabine; Stohl, Andreas; Klimont, Z.; Heyes, C.; Semiletov, I. P.; Dudarev, O. V.; Charkin, A.; Shakhova, N.; Holmstrand, H.; Andersson, A.; Gustafsson, Ö.

Black carbon (BC) contributes to Arctic climate warming, yet source attributions are inaccurate due to lacking observational constraints and uncertainties in emission inventories. Year-round, isotope-constrained observations reveal strong seasonal variations in BC sources with a consistent and synchronous pattern at all Arctic sites. These sources were dominated by emissions from fossil fuel combustion in the winter and by biomass burning in the summer. The annual mean source of BC to the circum-Arctic was 39 ± 10% from biomass burning. Comparison of transport-model predictions with the observations showed good agreement for BC concentrations, with larger discrepancies for (fossil/biomass burning) sources. The accuracy of simulated BC concentration, but not of origin, points to misallocations of emissions in the emission inventories. The consistency in seasonal source contributions of BC throughout the Arctic provides strong justification for targeted emission reductions to limit the impact of BC on climate warming in the Arctic and beyond.

2019

Snow buntings (Plectrophenax nivealis) as bio-indicators for exposure differences to legacy and emerging persistent organic pollutants from the Arctic terrestrial environment on Svalbard

Warner, Nicholas Alexander; Sagerup, Kjetil; Kristoffersen, Siv; Herzke, Dorte; Gabrielsen, Geir W.; Jenssen, Bjørn Munro

Eggs of snow buntings (Plectrophenax nivealis) were applied as a bio-indicator to examine differences in exposure to legacy persistent organic pollutants (POPs) and perflouroalkyl subtances (PFAS) from the terrestrial environment surrounding the settlements of Longyearbyen, Barentsburg and Pyramiden on Svalbard, Norway. Significantly higher concentrations of summed polychlorinated biphenyls (sumPCB7) in eggs collected from Barentsburg (2980 ng/g lipid weight (lw)) and Pyramiden (3860 ng/g lw) compared to Longyearbyen (96 ng/g lw) are attributed to local sources of PCBs within these settlements. Similar findings were observed for p,p′-dichlorodiphenyldichloroethylene (p,p′-DDE) where higher median concentrations observed in Pyramiden (173 ng/g lw) and Barentsburg (75 ng/g lw) compared to Longyearbyen (48 ng/g lw) may be influenced by guano inputs from breeding seabird populations, although other point sources cannot be ruled out. Concentrations of perfluorooctane sulphonate (PFOS) and several perfluorinated carboxylic acids (PFCAs) in snow bunting eggs were found to be statistically higher in the populated settlements of Longyearbyen and Barentsburg compared to the abandoned Pyramiden. Narrow foraging ranges of snow buntings during breeding season was useful in assessing point sources of exposure for PCBs and PFAS at particular sites with extreme differences observed between nest locations. SumPCB7 concentrations ranged from 2 μg/g ww to below detection limits between nest sites located less than a kilometer from each other in Pyramiden. Similar findings were observed in Longyearbyen, where several PFCAs ranged from 2 to 55 times higher between nest sites with similar spatial distances. These findings indicate that snow buntings can be a useful bio-indicator offering high spatial resolution for contaminant source apportionment in terrestrial environments on Svalbard.

2019

Open fires in Greenland in summer 2017: transport, deposition and radiative effects of BC, OC and BrC emissions

Evangeliou, Nikolaos; Kylling, Arve; Eckhardt, Sabine; Myroniuk, Viktor; Stebel, Kerstin; Paugam, Ronan; Zibtsev, Sergiy; Stohl, Andreas

Highly unusual open fires burned in western Greenland between 31 July and 21 August 2017, after a period of warm, dry and sunny weather. The fires burned on peatlands that became vulnerable to fires by permafrost thawing. We used several satellite data sets to estimate that the total area burned was about 2345 ha. Based on assumptions of typical burn depths and emission factors for peat fires, we estimate that the fires consumed a fuel amount of about 117 kt C and emitted about 23.5 t of black carbon (BC) and 731 t of organic carbon (OC), including 141 t of brown carbon (BrC). We used a Lagrangian particle dispersion model to simulate the atmospheric transport and deposition of these species. We find that the smoke plumes were often pushed towards the Greenland ice sheet by westerly winds, and thus a large fraction of the emissions (30 %) was deposited on snow- or ice-covered surfaces. The calculated deposition was small compared to the deposition from global sources, but not entirely negligible. Analysis of aerosol optical depth data from three sites in western Greenland in August 2017 showed strong influence of forest fire plumes from Canada, but little impact of the Greenland fires. Nevertheless, CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) lidar data showed that our model captured the presence and structure of the plume from the Greenland fires. The albedo changes and instantaneous surface radiative forcing in Greenland due to the fire emissions were estimated with the SNICAR model and the uvspec model from the libRadtran radiative transfer software package. We estimate that the maximum albedo change due to the BC and BrC deposition was about 0.007, too small to be measured. The average instantaneous surface radiative forcing over Greenland at noon on 31 August was 0.03–0.04 W m−2, with locally occurring maxima of 0.63–0.77 W m−2 (depending on the studied scenario). The average value is up to an order of magnitude smaller than the radiative forcing from other sources. Overall, the fires burning in Greenland in the summer of 2017 had little impact on the Greenland ice sheet, causing a small extra radiative forcing. This was due to the – in a global context – still rather small size of the fires. However, the very large fraction of the emissions deposited on the Greenland ice sheet from these fires could contribute to accelerated melting of the Greenland ice sheet if these fires become several orders of magnitude larger under future climate.

2019

Global and regional trends of atmospheric sulfur

Aas, Wenche; Mortier, Augustin; Bowersox, Van C.; Cherian, Ribu; Faluvegi, Greg; Fagerli, Hilde; Hand, Jenny; Klimont, Zbigniew; Galy-Lacaux, Corinne; Lehmann, Christopher M.B.; Myhre, Cathrine Lund; Myhre, Gunnar; Oliviè, Dirk Jan Leo; Sato, Keiichi; Quaas, Johannes; Rao, Pasumarthi Surya Prakasa; Schulz, Michael; Shindell, Drew; Skeie, Ragnhild Bieltvedt; Stein, Ariel; Takemura, Toshihiko; Tsyro, Svetlana; Vet, Robert; Xu, Xiaobin

The profound changes in global SO2 emissions over the last decades have affected atmospheric composition on a regional and global scale with large impact on air quality, atmospheric deposition and the radiative forcing of sulfate aerosols. Reproduction of historical atmospheric pollution levels based on global aerosol models and emission changes is crucial to prove that such models are able to predict future scenarios. Here, we analyze consistency of trends in observations of sulfur components in air and precipitation from major regional networks and estimates from six different global aerosol models from 1990 until 2015. There are large interregional differences in the sulfur trends consistently captured by the models and observations, especially for North America and Europe. Europe had the largest reductions in sulfur emissions in the first part of the period while the highest reduction came later in North America and East Asia. The uncertainties in both the emissions and the representativity of the observations are larger in Asia. However, emissions from East Asia clearly increased from 2000 to 2005 followed by a decrease, while in India a steady increase over the whole period has been observed and modelled. The agreement between a bottom-up approach, which uses emissions and process-based chemical transport models, with independent observations gives an improved confidence in the understanding of the atmospheric sulfur budget.

2019

Global soil nitrous oxide emissions since the preindustrial era estimated by an ensemble of terrestrial biosphere models: Magnitude, attribution, and uncertainty

Tian, Hanqin; Yang, Jia; Xu, Rongting; Lu, Chaoqun; Canadell, Josep G.; Davidson, Eric A.; Jackson, Robert B.; Arneth, Almut; Chang, Jinfeng; Ciais, Philippe; Gerber, Stefan; Ito, Akihiko; Joos, Fortunat; Lienert, Sebastian; Messina, Palmira; Olin, Stefan; Pan, Shufen; Peng, Changhui; Saikawa, Eri; Thompson, Rona Louise; Vuichard, Nicolas; Winiwarter, Wilfried; Zaehle, Sönke; Zhang, Bowen

2019

Measurements of Oxidative Potential of Particulate Matter at Belgrade Tunnel; Comparison of BPEAnit, DTT and DCFH Assay

Jovanovic, Maja; Savic, Jasmina; Salimi, Farhad; Stevanovic, Svetlana; Brown, Reece A.; Jovasevic-Stojanovic, Milena; Manojlovic, Dragan; Bartonova, Alena; Bottle, Steven; Ristovski, Zoran

To estimate the oxidative potential (OP) of particulate matter (PM), two commonly used cell-free, molecular probes were applied: dithiothreitol (DTT) and dichloro-dihydro-fluorescein diacetate (DCFH-DA), and their performance was compared with 9,10-bis (phenylethynyl) anthracene-nitroxide (BPEAnit). To the best of our knowledge, this is the first study in which the performance of the DTT and DCFH has been compared with the BPEAnit probe. The average concentrations of PM, organic carbon (OC) and elemental carbon (EC) for fine (PM2.5) and coarse (PM10) particles were determined. The results were 44.8 ± 13.7, 9.8 ± 5.1 and 9.3 ± 4.8 µg·m−3 for PM2.5 and 75.5 ± 25.1, 16.3 ± 8.7 and 11.8 ± 5.3 µg·m−3 for PM10, respectively, for PM, OC and EC. The water-soluble organic carbon (WSOC) fraction accounted for 42 ± 14% and 28 ± 9% of organic carbon in PM2.5 and PM10, respectively. The average volume normalized OP values for the three assays depended on both the sampling periods and the PM fractions. The OPBPEAnit had its peak at 2 p.m.; in the afternoon, it was three times higher compared to the morning and late afternoon values. The DCFH and BPEAnit results were correlated (r = 0.64), while there was no good agreement between the BPEAnit and the DTT (r = 0.14). The total organic content of PM does not necessarily represent oxidative capacity and it shows varying correlation with the OP. With respect to the two PM fractions studied, the OP was mostly associated with smaller particles.

2019

Polycyclic Aromatic Hydrocarbons Not Declining in Arctic Air Despite Global Emission Reduction

Yu, Yong; Katsoyiannis, Athanasios A.; Bohlin-Nizzetto, Pernilla; Brorström-Lundén, Eva; Ma, Jianmin; Zhao, Yuan; Wu, Zhiyong; Tych, Wlodzimierz; Mindham, David; Sverko, Ed; Barresi, Enzo; Dryfhout-Clark, Helena; Fellin, Phil; Hung, Hayley

Two decades of atmospheric measurements of polycyclic aromatic hydrocarbons (PAHs) were conducted at three Arctic sites, i.e., Alert, Canada; Zeppelin, Svalbard; and Pallas, Finland. PAH concentrations decrease with increasing latitude in the order of Pallas > Zeppelin > Alert. Forest fire was identified as an important contributing source. Three representative PAHs, phenanthrene (PHE), pyrene (PYR), and benzo[a]pyrene (BaP) were selected for the assessment of their long-term trends. Significant decline of these PAHs was not observed contradicting the expected decline due to PAH emission reductions. A global 3-D transport model was employed to simulate the concentrations of these three PAHs at the three sites. The model predicted that warming in the Arctic would cause the air concentrations of PHE and PYR to increase in the Arctic atmosphere, while that of BaP, which tends to be particle-bound, is less affected by temperature. The expected decline due to the reduction of global PAH emissions is offset by the increment of volatilization caused by warming. This work shows that this phenomenon may affect the environmental occurrence of other anthropogenic substances, such as more volatile flame retardants and pesticides.

2019

Monitoring Soil Moisture Drought over Northern High Latitudes from Space

Blyverket, Jostein; Hamer, Paul David; Schneider, Philipp; Albergel, Clement; Lahoz, William A.

Mapping drought from space using, e.g., surface soil moisture (SSM), has become viable in the last decade. However, state of the art SSM retrieval products suffer from very poor coverage over northern latitudes. In this study, we propose an innovative drought indicator with a wider spatial and temporal coverage than that obtained from satellite SSM retrievals. We evaluate passive microwave brightness temperature observations from the Soil Moisture and Ocean Salinity (SMOS) satellite as a surrogate drought metric, and introduce a Standardized Brightness Temperature Index (STBI). We compute the STBI by fitting a Gaussian distribution using monthly brightness temperature data from SMOS; the normal assumption is tested using the Shapior-Wilk test. Our results indicate that the assumption of normally distributed brightness temperature data is valid at the 0.05 significance level. The STBI is validated against drought indices from a land surface data assimilation system (LDAS-Monde), two satellite derived SSM indices, one from SMOS and one from the ESA CCI soil moisture project and a standardized precipitation index based on in situ data from the European Climate Assessment & Dataset (ECA&D) project. When comparing the temporal dynamics of the STBI to the LDAS-Monde drought index we find that it has equal correlation skill to that of the ESA CCI soil moisture product ( 0.71 ). However, in addition the STBI provides improved spatial coverage because no masking has been applied over regions with dense boreal forest. Finally, we evaluate the STBI in a case study of the 2018 Nordic drought. The STBI is found to provide improved spatial and temporal coverage when compared to the drought index created from satellite derived SSM over the Nordic region. Our results indicate that when compared to drought indices from precipitation data and a land data assimilation system, the STBI is qualitatively able to capture the 2018 drought onset, severity and spatial extent. We did see that the STBI was unable to detect the 2018 drought recovery for some areas in the Nordic countries. This false drought detection is likely linked to the recovery of vegetation after the drought, which causes an increase in the passive microwave brightness temperature, hence the STBI shows a dry anomaly instead of normal conditions, as seen for the other drought indices. We argue that the STBI could provide additional information for drought monitoring in regions where the SSM retrieval problem is not well defined. However, it then needs to be accompanied by a vegetation index to account for the recovery of the vegetation which could cause false drought detection.

2019

Year-Round In Situ Measurements of Arctic Low-Level Clouds: Microphysical Properties and Their Relationships With Aerosols

Koike, Makoto; Ukita, Jinro; Ström, Johan; Tunved, Peter; Shiobara, Masataka; Vitale, Vito; Lupi, Angelo; Baumgardner, D.; Ritter, Christoph; Hermansen, Ove; Yamada, K.; Pedersen, Christina Alsvik

Two years of continuous in situ measurements of Arctic low‐level clouds have been made at the Mount Zeppelin Observatory (78°56′N, 11°53′E), in Ny‐Ålesund, Spitsbergen. The monthly median value of the cloud particle number concentration (Nc) showed a clear seasonal variation: Its maximum appeared in May–July (65 ± 8 cm−3), and it remained low between October and March (8 ± 7 cm−3). At temperatures warmer than 0 °C, a clear correlation was found between the hourly Nc values and the number concentrations of aerosols with dry diameters larger than 70 nm (N70), which are proxies for cloud condensation nuclei (CCN). When clouds were detected at temperatures colder than 0 °C, some of the data followed the summertime Nc to N70 relationship, while other data showed systematically lower Nc values. The lidar‐derived depolarization ratios suggested that the former (CCN‐controlled) and latter (CCN‐uncontrolled) data generally corresponded to clouds consisting of supercooled water droplets and those containing ice particles, respectively. The CCN‐controlled data persistently appeared throughout the year at Zeppelin. The aerosol‐cloud interaction index (ACI = dlnNc/(3dlnN70)) for the CCN‐controlled data showed high sensitivities to aerosols both in the summer (clean air) and winter–spring (Arctic haze) seasons (0.22 ± 0.03 and 0.25 ± 0.02, respectively). The air parcel model calculations generally reproduced these values. The threshold diameters of aerosol activation (Dact), which account for the Nc of the CCN‐controlled data, were as low as 30–50 nm when N70 was less than 30 cm−3, suggesting that new particle formation can affect Arctic cloud microphysics.

2019

The comet assay applied to HepG2 liver spheroids

Elje, Elisabeth; Hesler, Michelle; Rundén-Pran, Elise; Mann, Pascal; Mariussen, Espen; Wagner, Sylvia; Dusinska, Maria; Kohl, Yvonne

In accordance with the 3 Rs to reduce in vivo testing, more advanced in vitro models, moving from 2D monolayer to 3D cultures, should be developed for prediction of human toxicity of industrial chemicals and environmental pollutants. In this study we compared cytotoxic and genotoxic responses induced by chemicals in 2D and 3D spheroidal cultures of the human liver cancer cell line HepG2.

HepG2 spheroids were prepared by hanging drop technology. Both 3D spheroids and 2D monolayer cultures were exposed to different chemicals (colchicine, chlorpromazine hydrochloride or methyl methanesulfonate) for geno- and cytotoxicity studies. Cytotoxicity was investigated by alamarBlue assay, flow cytometry and confocal imaging. DNA damage was investigated by the comet assay with and without Fpg enzyme for detection of DNA strand breaks and oxidized or alkylated base lesions.

The results from the cyto- and genotoxicity tests showed differences in sensitivity comparing the 2D and 3D HepG2 models. This study shows that human 3D spheroidal hepatocellular cultures can be successfully applied for genotoxicity testing by the comet assay and represent a promising advanced in vitro model for toxicity testing.

2019

Cleaning costs for European sheltered white painted steel and modern glass surfaces due to air pollution since the year 2000

Grøntoft, Terje; Verney-Carron, Aurelie; Tidblad, Johan

This paper reports estimated maintenance-cleaning costs, cost savings and cleaning interval increases for structural surfaces and windows in Europe obtainable by reducing the air pollution. Methodology and data from the ICP-materials project were used. The average present (2018) cleaning costs for sheltered white painted steel surfaces and modern glass due to air pollution over background, was estimated to be ~2.5 Euro/m2∙year. Hypothetical 50% reduction in the air pollution was found to give savings in these cleaning costs of ~1.5 Euro/m2∙year. Observed reduction in the air pollution, from 2002–2005 until 2011–2014, have probably increased the cleaning interval for white painted steel with ~100% (from 12 to 24 years), representing reductions in the single intervention cleaning costs from 7 to 4%/year (= % of one cleaning investment, per year during the cleaning interval) and for the modern glass with ~65% (from 0.85 to 1.3 years), representing reductions in the cleaning cost from 124 to 95%/year. The cleaning cost reductions, obtainable by 50% reduction in air pollution, would have been ~3 %/year for white painted steel and ~60%/year for the modern glass, representing ~100 and 50% additional cleaning interval increases. These potential cleaning cost savings are significantly higher than previously reported for the weathering of Portland limestone ornament and zinc monuments.

2019

Dose calculations in aircrafts after Fukushima nuclear power plant accident – Preliminary study for aviation operations

Vargas, Arturo; Arnold, Delia; Duch, M.-A.; Evangeliou, Nikolaos; Sievers, Klaus; Maurer, C

There is little information to decision support in air traffic management in case of nuclear releases into the atmosphere. In this paper, the dose estimation due to both, external exposure (i.e. cloud immersion, deposition inside and outside the aircraft), and due to internal exposure (i.e, inhalation of radionuclides inside the aircraft) to passengers and crew is calculated for a worst-case emergency scenario. The doses are calculated for different radionuclides and activities. Calculations are mainly considered according to International Commission on Radiological Protection (ICRP) recommendations and Monte Carlo simulations. In addition, a discussion on potential detectors installed inside the aircraft for monitoring the aerosol concentration and the ambient dose equivalent rate, H*(10), for during-flight monitoring and early warning is provided together with the evaluation of a response of a generic detector. The results show that the probability that a catastrophic nuclear accident would produce significant radiological doses to the passengers and crew of an aircraft is very low. In the worst-case scenarios studied, the maximum estimated effective dose was about 1 mSv during take-off or landing operations, which is the recommended yearly threshold for the public. However, in order to follow the ALARA (As Low As Reasonably Achievable) criteria and to avoid aircraft contamination, the installation of radiological detectors is considered. This would, on one hand help the pilot or corresponding decision maker to decide about the potential change of the route and, on the other, allow for gathering of 4D data for future studies.

2019

PM10 levels at urban, suburban, and background locations in the eastern Mediterranean: local versus regional sources with emphasis on African dust

Chatoutsidou, Sofia Eirini; Kopanakis, Ilias; Lagouvardos, Konstantinos; Mihalopoulos, Nikolaos; Tørseth, Kjetil; Lazaridis, Mihalis

2019

Acceleration of global N2O emissions seen from two decades of atmospheric inversion

Thompson, Rona Louise; Lassaletta, Luis; Patra, Prabir K.; Wilson, Chris; Wells, Kelley C.; Gressent, Alicia; Koffi, Ernest N.; Chipperfield, Martyn P.; Winiwarter, Wilfried; Davidson, Eric A.; Tian, Hanqin; Canadell, Josep G.

2019

Frequency of extreme precipitation increases extensively with event rareness under global warming

Myhre, Gunnar; Alterskjær, Kari; Stjern, Camilla Weum; Hodnebrog, Øivind; Marelle, Louis; Samset, Bjørn Hallvard; Sillmann, Jana; Schaller, Nathalie; Fischer, Erich; Schulz, Michael; Stohl, Andreas

The intensity of the heaviest extreme precipitation events is known to increase with global warming. How often such events occur in a warmer world is however less well established, and the combined effect of changes in frequency and intensity on the total amount of rain falling as extreme precipitation is much less explored, in spite of potentially large societal impacts. Here, we employ observations and climate model simulations to document strong increases in the frequencies of extreme precipitation events occurring on decadal timescales. Based on observations we find that the total precipitation from these intense events almost doubles per degree of warming, mainly due to changes in frequency, while the intensity changes are relatively weak, in accordance to previous studies. This shift towards stronger total precipitation from extreme events is seen in observations and climate models, and increases with the strength – and hence the rareness – of the event. Based on these results, we project that if historical trends continue, the most intense precipitation events observed today are likely to almost double in occurrence for each degree of further global warming. Changes to extreme precipitation of this magnitude are dramatically stronger than the more widely communicated changes to global mean precipitation.

2019

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