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2000
2021
Fluorinated polymers in a low carbon, circular and toxic-free economy. Technical report.
Fluorinated polymers are used in a variety of applications providing benefits to the society, but at the same time also causing risks of irreversible pollution and impacts on the environment and human health in different stages of the lifecycle. The main aim of the study was to provide information on impacts of fluorinated polymers along their lifecycles in a low carbon, circular and toxic-free economy, which could be relevant to consider in future assessments. An important part of the work was also to discuss options for risk governance and to identify knowledge gaps. The work was based on a literature survey of recently published reports and selected peer-reviewed articles on the topic.
The report presents the results of the work carried out by the ETC/WMGE and ETC/CME.
ETC/WMGE
2021
Of the thousands of per- and polyfluoroalkyl substances (PFAS) known to exist, only a small fraction (≤1%) are commonly monitored in humans. This discrepancy has led to concerns that human exposure may be underestimated. Here, we address this problem by applying a comprehensive fluorine mass balance (FMB) approach, including total fluorine (TF), extractable organic fluorine (EOF), total oxidizable precursors (TOP), and selected target PFAS, to human serum samples collected over a period of 28 years (1986, 2007, and 2015) in Tromsø, Norway. While concentrations of TF did not change between sampling years, EOF was significantly higher in 1986 compared to 2007 and 2015. The ∑12PFAS concentrations were highest in 2007 compared to 1986 and 2015, and unidentified EOF (UEOF) decreased from 1986 (46%) to 2007 (10%) and then increased in 2015 (37%). While TF and EOF were not influenced by sex, women had higher UEOF compared to men, opposite to target PFAS. This is the first FMB in human serum to include TOP, and it suggests that precursors with >4 perfluorinated carbon atoms make a minor contribution to EOF (0–4%). Additional tools are therefore needed to identify substances contributing to the UEOF in human serum.
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