Fant 9758 publikasjoner. Viser side 125 av 391:
The report evaluates current mapping methodology with respect to city- and NUTS3-levels mapping across Europe. It states that the current mapping can be used at the city and the NUTS3 levels, despite a mild smoothing effect at locations of the measurement stations. However, it suggests a post-processing correction based on the mapping residuals.
A potential new approach for the city ranking have been examined, namely the population-weighted concentration based on the mapping results. While the averaged measurement data from the background stations (as used in the current city ranking) provides a superior information for the whole city in general, the population-weighted concentration also well represents the whole city and gives a consistent information for all cities, including those without station measurements.
Next to this, alternative treatments of rural and urban stations has been evaluated. If the urban traffic areas should be better represented in the final maps, an increased map resolution is recommended.
Several possibilities of future development towards the European-wide city level mapping in a fine resolution have been suggested, namely exploitation of a high-resolution model output in the existing methodology, geostatistical downscaling of the existing spatial maps using fine-resolution proxy datasets and exploitation of existing low-cost sensor networks.
ETC/ATNI
2021
2022
2021
2003
2009
2003
Evaluating a forecast system for long-range atmospheric transport episodes of POPs. NILU PP
Background air measurements of persistent organic pollutants (POPs) within existing monitoring programs are typically conducted by use of active air samplers (AAS), but the high cost of AAS limits their spatial and temporal coverage. Sampling at many such sites furthermore occurs at fixed intervals (e.g. one day per week) without any a priori consideration of air mass transport (i.e., whether the air is likely to be polluted or not). While the current strategy is appropriate for the purpose of assessing long-term trends (years, decades), the fixed interval non-continuous sampling approach is at risk of missing out key long-range atmospheric transport (LRAT) episodes. The objectives of this study have been to (i) develop a forecast system using the Lagrangian transport model FLEXPART to predict long-range atmospheric transport episodes of POPs using PCB-28 as a model compound, (ii) to evaluate the capability of the forecast system to capture specific LRAT events at a background site in southern Norway (Birkenes) through targeted sampling (i.e. when LRAT events are predicted), (iii) to assess whether predicted LRAT events for PCB-28 coincide with elevated concentrations of additional PCBs and other POPs, and (iv) to identify source regions of POPs during individual episodes. The system has been initially evaluated by comparing targeted samples collected over 12 to 25 hours during individual LRAT episodes, with monitoring samples regularly collected over one day per week throughout 2011. The FLEXPART model was clearly successful in identifying LRAT episodes for both PCB-28 and other PCBs. The model fails to accurately reproduce the magnitude of PCB-28 concentrations during individual episodes, but this can be mainly attributed to uncertainties in the absolute emission rates of PCB-28 used to drive simulations. We conclude that forecasting of pollution episodes has the potential to add value to relevant monitoring efforts which are normally collecting active air samples at fixed intervals in a non-continuous manner. Observations targeted at strong pollution episodes (as in this study) or on transport from specific source regions with highly uncertain emissions (as could be done in a very similar forecasting framework) could significantly enhance our understanding of POP sources.
2013
2002
2018
2024
2017
2015
2015
2020
2006
2013
2013
2011
Evaluation and Global-Scale Observation of Nitrous Oxide from IASI on Metop-A
Nitrous oxide (N2O) is a greenhouse gas difficult to estimate by satellite because of its weak spectral signature in the infra-red band and its low variability in the troposphere. Nevertheless, this study presents the evaluation of new tropospheric N2O observations from the Infrared Atmospheric Sounder Interferometer (IASI) on Metop-A using the Toulouse N2O Retrieval Version 2.0 tool. This tool is based on the Radiative Transfer for Tiros Operational Vertical sounder (RTTOV) model version 12.3 coupled to the Levenberg-Marquardt optimal estimation method enabling the simultaneous retrieval of methane, water vapour, temperature profiles together with surface temperature and emissivity within the 1240–1350 cm−1 window. In this study, we focused on the upper troposphere (300 hPa) where the sensitivity of IASI is significant. The IASI N2O data has been evaluated using aircraft N2O observations from the High-performance Instrumented Airborne Platform for Environmental Research Pole-to-Pole Observations (HIPPO) campaigns in 2009, 2010, and 2011 and from the National Oceanic and Atmospheric Administration’s (NOAA) Global Greenhouse Gas Reference Network (GGGRN) in 2011. In addition, we evaluated the IASI N2O using ground-based N2O measurements from 9 stations belonging to the Network for the Detection of Atmospheric Composition Change (NDACC). We found a total random error of ∼2 ppbv (0.6%) for one single retrieval at 300 hPa. Under favorable conditions, this error is also found in the vertical level pressure range 300–500 hPa. It decreases rapidly to ∼0.4 ppbv (0.1%) when we average on a 1° × 1° box. In addition, independent observations allows the estimation of bias with the IASI TN2OR v2.0 N2O. The bias between IASI and aircraft N2O data at 300 hPa is ∼1.0 ppbv (∼0.3%). We found an estimated random error of ∼2.3 ppbv (∼0.75%). This study also shows relatively high correlations between IASI data and aircraft in situ profiles but more varying correlations over the year 2011 depending on the location between IASI and NDACC remote sensing data. Finally, we present daily, monthly, and seasonal IASI N2O horizontal distributions in the upper troposphere as well as cross sections for different seasons that exhibit maxima in the Tropical band especially over Africa and South America.
MDPI
2022
2007
2007
2007
2007
2010