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EEA-33 Industrial Emissions Country Profiles. Methodology report. Updated July 2020.

Weydahl, Torleif; Young, Katrina; Hampshire, Kathryn; Goodwin, Justin; Granger, Marthe; Zeiger, Bastian

The industrial emissions country profiles summarise key data related to industry: its relevance with respect to economic contributions, energy and water consumption, as well as air and water emissions and waste generation. The country profiles are developed for the EEA-33 countries which includes the 28 EU Member States together with Iceland, Lichtenstein, Norway, Switzerland and Turkey.

The present revision (v. 3.0) of this report includes data available at date of release. This year, a new reporting, the so-called EU-Registry and thematic data reporting, is introduced in order to gather the former E-PRTR, LCP and IED reportings and finally replace them. The 2018 data are not yet readily available. Nevertheless, more quality checks have been performed on the latest E-PRTR database in order to have the cleanest final E-PRTR dataset possible. Hence, the industrial emissions country profiles are enriched with the most up-to-date data sources while still only covering the years up to 2017.

This report describes the underlying methodology to the industrial emissions country profiles that are presented as a Tableau story on the EEA webpages ([1]).

The scope of industry in this respect includes in short all industrial activities reported under the European Pollutant Release and Transfer Register (E-PRTR) excluding agriculture (activity code 7.(a) and 7.(b)). The data sources include Eurostat, the E-PRTR, greenhouse gas (GHG) emissions reported under the Monitoring Mechanism Regulation (MMR) and air pollutant emission inventories reported under the Convention on Long-range Transboundary Air Pollution (CLRTAP), each of which have their own data categories. A recently developed EEA-mapping which align these different categories is used ([2]). The data sources and industry scope is presented in full detail in the Annexes following this report.

The water and air pollutants including greenhouse gases are selected based on criteria related to their relative impact. Emissions of heavy metals to air and water have been combined by weighted averages using both eco toxicology and human toxicology characterisation factors ([3]). The amounts of hazardous and non-hazardous waste reported under Eurostat is presented, but excluding the major mineral waste that dominates the mining and construction sectors.

The data quality is evaluated and gap filling of Eurostat data is performed when needed. A method for E-PRTR outlier handling is proposed and applied where appropriate.

The significance of industry, given by gross value added (GVA), energy consumption and water use, as well as generation of waste are presented in the Tableau story as a sector percentage of EEA-33 gross total as well as percentage of country total. The trend in air and water pollution is presented as totals per pollutants relative to the latest year (2017). For the latest year the emissions are also given as percentage per sector relative to country total. The details on how the presented data is processed and aggregated is described in Annex 2.

The report is to a large extent based on previous methodology reports for “Industrial pollution country profiles”, but is also further developed to reflect feedback received through Eionet review and general requests from EEA and the European Commission.

ETC/ATNI

2020

Monitoring of environmental contaminants in air and precipitation. Annual report 2019.

Bohlin-Nizzetto, Pernilla; Aas, Wenche; Nikiforov, Vladimir

This report presents environmental monitoring data from 2019 and time-trends for the Norwegian programme for Long-range atmospheric transported contaminants. The results cover 200 organic compounds (regulated and non-regulated), 11 heavy metals, and organic chemicals of potential Arctic concern.

NILU

2020

Quantification of microplastic in fillet and organs of farmed and wild salmonids- a comparison of methods for detection and quantification

Gomiero, Alessio; Haave, Marte; Bjorøy, Ørjan; Herzke, Dorte; Kögel, Tanja; Nikiforov, Vladimir; Øysæd, Kjell Birger

Microplastic (MP) is of growing concern to environmental and human health. This study investigated three analytical approaches to measure MP in tissues of salmonids. The study aimed to 1) determine and demonstrate the sensitivity of current analytical methods for MP in salmon tissues for the three different quantitative methods, 2) compare the utility of the different methods in terms of cost, time and sensitivity 3) quantify MP in a relevant selection of tissues of farmed and wild salmon in order to establish likely indicator organs for future documentation purposes. We here present the results, compare the methods and discuss uncertainties and needs for further method development.

NORCE Norwegian Research Centre

2020

Record‐Breaking Increases in Arctic Solar Ultraviolet Radiation Caused by Exceptionally Large Ozone Depletion in 2020

Bernhard, Germar H.; Fioletov, Vitali E.; Grooss, Jens-Uwe; Ialongo, Iolanda; Johnsen, Bjørn; Lakkala, Kaisa; Manney, Gloria L.; Müller, Rolf; Svendby, Tove Marit

Measurements of solar ultraviolet radiation (UVR) performed between January and June 2020 at 10 Arctic and subarctic locations are compared with historical observations. Differences between 2020 and prior years are also assessed with total ozone column and UVR data from satellites. Erythemal (sunburning) UVR is quantified with the UV Index (UVI) derived from these measurements. UVI data show unprecedently large anomalies, occurring mostly between early March and mid‐April 2020. For several days, UVIs observed in 2020 exceeded measurements of previous years by up to 140%. Historical means were surpassed by more than six standard deviations at several locations in the Arctic. In northern Canada, the average UVI for March was about 75% larger than usual. UVIs in April 2020 were elevated on average by about 25% at all sites. However, absolute anomalies remained below 3.0 UVI units because the enhancements occurred during times when the solar elevation was still low.

2020

Contaminants, prolactin and parental care in an Arctic seabird: Contrasted associations of perfluoroalkyl substances and organochlorine compounds with egg-turning behavior

Blévin, Pierre; Shaffer, Scott A.; Bustamante, Paco; Angelier, Frédéric; Picard, Baptiste; Herzke, Dorte; Moe, Børge; Gabrielsen, Geir W.; Bustnes, Jan Ove; Chastel, Olivier

2020

Evaluation of climate model aerosol trends with ground-based observations over the last 2 decades – an AeroCom and CMIP6 analysis

Mortier, Augustin; Gliss, Jonas; Schulz, Michael; Aas, Wenche; Andrews, Elisabeth; Bian, Huisheng; Chin, Mian; Ginoux, Paul; Hand, Jenny; Holben, Brent; Zhang, Hua; Kipling, Zak; Kirkevåg, Alf; Laj, Paolo; Lurton, Thibault; Myhre, Gunnar; Neubauer, David; Oliviè, Dirk Jan Leo; Salzen, Knut von; Skeie, Ragnhild Bieltvedt; Takemura, Toshihiko; Tilmes, Simone

This study presents a multiparameter analysis of aerosol trends over the last 2 decades at regional and global scales. Regional time series have been computed for a set of nine optical, chemical-composition and mass aerosol properties by using the observations from several ground-based networks. From these regional time series the aerosol trends have been derived for the different regions of the world. Most of the properties related to aerosol loading exhibit negative trends, both at the surface and in the total atmospheric column. Significant decreases in aerosol optical depth (AOD) are found in Europe, North America, South America, North Africa and Asia, ranging from −1.2 % yr−1 to −3.1 % yr−1. An error and representativity analysis of the spatially and temporally limited observational data has been performed using model data subsets in order to investigate how much the observed trends represent the actual trends happening in the regions over the full study period from 2000 to 2014. This analysis reveals that significant uncertainty is associated with some of the regional trends due to time and space sampling deficiencies. The set of observed regional trends has then been used for the evaluation of 10 models (6 AeroCom phase III models and 4 CMIP6 models) and the CAMS reanalysis dataset and of their skills in reproducing the aerosol trends. Model performance is found to vary depending on the parameters and the regions of the world. The models tend to capture trends in AOD, the column Ångström exponent, sulfate and particulate matter well (except in North Africa), but they show larger discrepancies for coarse-mode AOD. The rather good agreement of the trends, across different aerosol parameters between models and observations, when co-locating them in time and space, implies that global model trends, including those in poorly monitored regions, are likely correct. The models can help to provide a global picture of the aerosol trends by filling the gaps in regions not covered by observations. The calculation of aerosol trends at a global scale reveals a different picture from that depicted by solely relying on ground-based observations. Using a model with complete diagnostics (NorESM2), we find a global increase in AOD of about 0.2 % yr−1 between 2000 and 2014, primarily caused by an increase in the loads of organic aerosols, sulfate and black carbon.

2020

Changes in black carbon emissions over Europe due to COVID-19 lockdowns

Evangeliou, Nikolaos; Platt, Stephen Matthew; Eckhardt, Sabine; Myhre, Cathrine Lund; Laj, P.; Alados-Arboledas, Lucas; Backman, J; Brem, Benjamin T.; Fiebig, Markus; Flentje, H.; Marinoni, A.; Pandolfi, M.; Yus-Diez, Jesus; Prats, N.; Putaud, J. P.; Sellegri, K.; Sorribas, Mar; Eleftheriadis, K.; Vratolis, Sterios; Wiedensohler, A.; Stohl, Andreas

2020

2020

New particle formation characteristics in the Arctic (Zeppelin, Svalbard)

Lee, Haebum; Lee, KwangYul; Krejci, Radovan; Aas, Wenche; Park, Jiyeon; Park, Ki-Tae; Lee, Bang-Yong; Yoon, Young-Jun; Park, Kihong

2020

Microplastics catch an atmospheric ride to the oceans and the Arctic

Evangeliou, Nikolaos (intervjuobjekt); Bourzac, Katherine (journalist)

2020

Environmental Contaminants in an Urban Fjord, 2019

Ruus, Anders; Bæk, Kine; Rundberget, Thomas; Allan, Ian; Beylich, Bjørnar; Vogelsang, Christian; Schlabach, Martin; Götsch, Arntraut; Borgå, Katrine; Helberg, Morten

This programme, “Environmental Contaminants in an Urban Fjord” has covered sampling and analyses of sediment and organisms in a marine food web of the Inner Oslofjord, in addition to samples of blood and eggs from herring gull. The programme also included inputs of pollutants via surface water (storm water), and effluent water and sludge from a sewage treatment plant. The bioaccumulation potential of the contaminants in the Oslo fjord food web was evaluated. The exposure to/accumulation of the contaminants was also assessed in birds. A vast number of chemical parameters have been quantified, in addition to some biological effect parameters in cod, and the report serves as a status description of the concentrations of these chemicals in different compartments of the Inner Oslofjord marine ecosystem.

Norsk institutt for vannforskning (NIVA)

2020

Mapping urban air quality using low-cost sensor networks

Schneider, Philipp; Castell, Nuria; Bartonova, Alena

2020

Non-target and suspect characterisation of organic contaminants in Arctic air – Part 2: Application of a new tool for identification and prioritisation of chemicals of emerging Arctic concern in air

Röhler, Laura; Schlabach, Martin; Haglund, Peter; Breivik, Knut; Kallenborn, Roland; Bohlin-Nizzetto, Pernilla

The Norwegian Arctic possesses a unique environment for the detection of new potential chemicals of emerging Arctic concern (CEACs) due to remoteness, sparse population and the low number of local contamination sources. Hence, a contaminant present in Arctic air is still considered a priority indication for its environmental stability and environmental mobility. Today, legacy persistent organic pollutants (POPs) and related conventional environmental pollutants are already well-studied because of their identification as Arctic pollutants in the 1980s. Many of them are implemented and reported in various national and international monitoring activities including the Arctic Monitoring and Assessment Programme (AMAP). These standard monitoring schemes, however, are based on compound-specific quantitative analytical methods. Under such conditions, the possibility for the identification of hitherto unidentified contaminants is limited and random at best. Today, new and advanced technological developments allow a broader, unspecific analytical approach as either targeted multicomponent analysis or suspect and non-target screening strategies. In order to facilitate such a wide range of compounds, a wide-scope sample clean-up method for high-volume air samples based on a combination of adsorbents was applied, followed by comprehensive two-dimensional gas chromatography separation and low-resolution time-of-flight mass spectrometric detection (GC × GC-LRMS). During the study reported here, simultaneous non-target and suspect screening were applied. The detection of over 700 compounds of interest in the particle phase and over 1200 compounds in the gaseous phase is reported. Of those, 62 compounds were confirmed with reference standards and 90 compounds with a probable structure (based upon mass spectrometric interpretation and library spectrum comparison). These included compounds already detected in Arctic matrices and compounds not detected previously (see also Fig. 1). In addition, 241 compounds were assigned a tentative structure or compound class. Hitherto unknown halogenated compounds, which are not listed in the mass spectral libraries used, were also detected and partly identified.

2020

Field- and model-based calibration of polyurethane foam passive air samplers in different climate regions highlights differences in sampler uptake performance

Bohlin-Nizzetto, Pernilla; Melymuk, Lisa; White, Kevin B.; Kalina, Jiří; Madadi, Vincent O.; Adu-Kumi, Sam; Prokeš, Roman; Pribylova, Petra; Klanova, Jana

2020

On the robustness of field calibration for smart air quality monitors

Vito, Saverio De; Esposito, Elena; Castell, Nuria; Schneider, Philipp; Bartonova, Alena

The robustness of field calibrated Air Quality Multi-sensors (AQM) performances to long term and/or mobile operation is still debated. Though accuracy generally exceeds the one of laboratory calibrations models, experimental results show that field calibration models cannot sustain optimal field performances due to changes occurring in operative conditions. Among them, the relocation of calibrated multi-sensors platforms and sensor drift are considered as the most relevant. In this work, we want to provide an answer to the general issue of field calibration robustness assessement. Analysing theoretical foundations and providing tools for determining the calibration model validity domain. In particular, by leveraging the probability distribution of target and interferent gas as well as environmental variables, measures of dissimilarity between calibration and operative phase conditions are considered to quantitatively capture the occurring change. A 6 months multiple nodes dataset including node relocations events in several sites have been processed for deriving nonlinear multivariate field calibrations whose robustness to changing conditions have been analysed. Kullback-Leibler, Euclidean and Hellinger dissimilarity measurements have been correlated with recorded performance degradation. Results show that quantifying relevant factors probability distribution changes allows to explain and predict performances of in field data driven calibration models. They also highlight the role of concept drift in explaining field performances ameliorating our capability to select optimal conditions in which a field calibration should be derived. Finally, smart air quality monitors could now autonomously detect the need for re-calibration.

2020

Changes in Net Ecosystem Exchange over Europe During the 2018 Drought

Thompson, Rona Louise; Broquet, G; Gerbig, C.; Koch, T; Lang, M.; Monteil, G.; Munassar, S; Nickless, A; Scholze, M.; Ramonet, M.; Karstens, U.; Schaik, E van; Wu, Z.; Rödenbeck, C.

2020

Validation practices for satellite soil moisture retrievals: What are (the) errors?

Gruber, Alexander; Lannoy, Gabriëlle J.M de; Albergel, Clément; Al-Yaari, Amen; Brocca, Luca; Calvet, Jean-Christophe; Colliander, Andreas; Cosh, Michael H.; Crow, Wade T.; Dorigo, Wouter Arnaud; Draper, Clara Sophie; Hirschi, Martin; Kerr, Yann H.; Konings, Alexandra G.; Lahoz, William A.; McColl, Kaighin Alexander; Montzka, Carsten; Muñoz-Sabater, Joaquín; Peng, Jian; Reichle, Rolf H.; Richaume, Philippe; Rüdiger, Christoph; Scanlon, Tracy; Schalie, Robin van der; Wigneron, Jean Pierre; Wagner, Wolfgang

This paper presents a community effort to develop good practice guidelines for the validation of global coarse-scale satellite soil moisture products. We provide theoretical background, a review of state-of-the-art methodologies for estimating errors in soil moisture data sets, practical recommendations on data pre-processing and presentation of statistical results, and a recommended validation protocol that is supplemented with an example validation exercise focused on microwave-based surface soil moisture products. We conclude by identifying research gaps that should be addressed in the near future.

2020

Bedre luftkvalitet, men fortsatt mye svevestøv

Høiskar, Britt Ann Kåstad (intervjuobjekt); Jonassen, Andreas de Brito (journalist)

2020

Målte skyhøyt forurensningsnivå – her er forklaringen

Tønnesen, Dag; Tørnkvist, Kjersti Karlsen (intervjuobjekter); Holterhuset, Martin (journalist)

2020

Nitrogen fertilisers are incredibly efficient, but they make climate change a lot worse

Canadell, P.; Tian, Hanqin; Patra, Prabir; Thompson, Rona Louise

2020

Forslag til norsk overvåkingsnettverk for å oppfylle NEC‐direktivets krav om å overvåke effekter av luftforurensing

Garmo, Øyvind Aaberg; Bakkestuen, Vegar; Solberg, Sverre; Timmermann, Volkmar; Simpson, David; Vollsnes, Ane Victoria; Aarrestad, Per Arild; Ranneklev, Sissel Brit

Norge har et eksisterende overvåkingsnettverk for å måle effekter av luftforurensninger som forsuring, overgjødsling og
ozoneksponering i økosystemer. Ved eventuell implementering av nytt NEC‐direktiv «takdirektiv» (2016/2284/EU) må Norge
rapportere inn overvåkingsnettverk og resultater fra overvåking av effekter av luftforurensninger i økosystemer.
I denne rapporten er dagens overvåkingsnettverk vurdert med hensyn til de krav som stilles i nytt NEC‐direktiv. Resultater viste
at for innsjøer og elver er dagens overvåkingsnettverk relatert til forsuring tilfredsstillende. For overgjødsling av skog, skogsjord
og terrestrisk natur er det behov for oppgraderinger av overvåkingsnettverket. I forhold til ozonskader i vegetasjon er det behov
for oppgraderinger av dagens overvåkingsnettverk.
Det vil påløpe kostnader for opprettelse av nye overvåkingsstasjoner og oppgraderinger av dagens overvåkingsnettverk.
Estimerte kostnader for å dekke mangler i eksisterende overvåkingsnettverk er angitt i rapporten.

Norsk institutt for vannforskning (NIVA)

2020

ClairCity: Citizen-led air pollution reduction in cities. D7.4 Final City Policy Package – Ljubljana.

Slingerland, Stephan; Artola, Irati; Bolscher, Hans; Barnes, Jo; Boushel, Corra; Fogg-Rogers, Laura; Hayes, Enda; Rodrigues, Vera; Oliveira, Kevin; Lopes, Myriam; Vanherle, Kris; Csobod, Eva; Trozzi, Carlo; Piscitello, Enzo; Knudsen, Svein; Soares, Joana

The ClairCity Horizon2020 project aims to contribute to citizen-inclusive air quality and carbon policy making in middle-sized European cities. It does so by investigating citizens’ current behaviours as well as their preferred future behaviours and policy measures in six European cities1 through an extensive citizen and stakeholder engagement process. The project also models the possible future impacts of citizens’ policy preferences and examines implementation possibilities for these measures in the light of the existing institutional contexts in each city (Figure 0-1). This report summarises the main policy results for Ljubljana.

ClairCity Project

2020

Source Quantification of South Asian Black Carbon Aerosols with Isotopes and Modeling

Dasari, Sanjeev; Andersson, August; Stohl, Andreas; Evangeliou, Nikolaos; Bikkina, Srinivas; Holmstrand, Henry; Budhavant, Krishnakant; Salam, Abdus; Gustafsson, Örjan

Black carbon (BC) aerosols perturb climate and impoverish air quality/human health—affecting ∼1.5 billion people in South Asia. However, the lack of source-diagnostic observations of BC is hindering the evaluation of uncertain bottom-up emission inventories (EIs) and thereby also models/policies. Here, we present dual-isotope-based (Δ14C/δ13C) fingerprinting of wintertime BC at two receptor sites of the continental outflow. Our results show a remarkable similarity in contributions of biomass and fossil combustion, both from the site capturing the highly populated highly polluted Indo-Gangetic Plain footprint (IGP; Δ14C-fbiomass = 50 ± 3%) and the second site in the N. Indian Ocean representing a wider South Asian footprint (52 ± 6%). Yet, both sites reflect distinct δ13C-fingerprints, indicating a distinguishable contribution of C4-biomass burning from peninsular India (PI). Tailored-model-predicted season-averaged BC concentrations (700 ± 440 ng m–3) match observations (740 ± 250 ng m–3), however, unveiling a systematically increasing model-observation bias (+19% to −53%) through winter. Inclusion of BC from open burning alone does not reconcile predictions (fbiomass = 44 ± 8%) with observations. Direct source-segregated comparison reveals regional offsets in anthropogenic emission fluxes in EIs, overestimated fossil-BC in the IGP, and underestimated biomass-BC in PI, which contributes to the model-observation bias. This ground-truthing pinpoints uncertainties in BC emission sources, which benefit both climate/air-quality modeling and mitigation policies in South Asia.

2020

Satellite validation strategy assessments based on the AROMAT campaigns

Merlaud, Alexis; Belegante, Livio; Constantin, Daniel-Eduard; Hoed, Mirjam Den; Meier, Andreas Carlos; Allaart, Marc; Ardelean, Magdalena; Arseni, Maxim; Bösch, Tim; Brenot, Hugues; Calcan, Andreea; Dekemper, Emmanuel; Donner, Sebastian; Dörner, Steffen; Dragomir, Mariana Carmelia Balanica; Georgescu, Lucian; Nemuc, Anca; Nicolae, Doina; Pinardi, Gaia; Richter, Andreas; Rosu, Adrian; Ruhtz, Thomas; Schönhardt, Anja; Schuettemeyer, Dirk; Shaiganfar, Reza; Stebel, Kerstin; Tack, Frederik; Vajaiac, Sorin Nicolae; Vasilescu, Jeni; Vanhamel, Jurgen; Wagner, Thomas; Roozendael, Michel Van

The Airborne ROmanian Measurements of Aerosols and Trace gases (AROMAT) campaigns took place in Romania in September 2014 and August 2015. They focused on two sites: the Bucharest urban area and large power plants in the Jiu Valley. The main objectives of the campaigns were to test recently developed airborne observation systems dedicated to air quality studies and to verify their applicability for the validation of space-borne atmospheric missions such as the TROPOspheric Monitoring Instrument (TROPOMI)/Sentinel-5 Precursor (S5P). We present the AROMAT campaigns from the perspective of findings related to the validation of tropospheric NO2, SO2, and H2CO. We also quantify the emissions of NOx and SO2 at both measurement sites.

We show that tropospheric NO2 vertical column density (VCD) measurements using airborne mapping instruments are well suited for satellite validation in principle. The signal-to-noise ratio of the airborne NO2 measurements is an order of magnitude higher than its space-borne counterpart when the airborne measurements are averaged at the TROPOMI pixel scale. However, we show that the temporal variation of the NO2 VCDs during a flight might be a significant source of comparison error. Considering the random error of the TROPOMI tropospheric NO2 VCD (σ), the dynamic range of the NO2 VCDs field extends from detection limit up to 37 σ (2.6×1016 molec. cm−2) and 29 σ (2×1016 molec. cm−2) for Bucharest and the Jiu Valley, respectively. For both areas, we simulate validation exercises applied to the TROPOMI tropospheric NO2 product. These simulations indicate that a comparison error budget closely matching the TROPOMI optimal target accuracy of 25 % can be obtained by adding NO2 and aerosol profile information to the airborne mapping observations, which constrains the investigated accuracy to within 28 %. In addition to NO2, our study also addresses the measurements of SO2 emissions from power plants in the Jiu Valley and an urban hotspot of H2CO in the centre of Bucharest. For these two species, we conclude that the best validation strategy would consist of deploying ground-based measurement systems at well-identified locations.

2020

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