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Assessing Lagrangian inverse modelling of urban anthropogenic CO2 fluxes using in situ aircraft and ground-based measurements in the Tokyo area

Pisso, Ignacio; Patra, Prabir; Takigawa, Masayuki; Machida, Toshinobu; Matsueda, Hidekazu; Sawa, Yousuke

BACKGROUND: In order to use in situ measurements to constrain urban anthropogenic emissions of carbon dioxide (CO2), we use a Lagrangian methodology based on diffusive backward trajectory tracer reconstructions and Bayesian inversion. The observations of atmospheric CO2 were collected within the Tokyo Bay Area during the Comprehensive Observation Network for TRace gases by AIrLiner (CONTRAIL) flights, from the Tsukuba tall tower of the Meteorological Research Institute (MRI) of the Japan Meteorological Agency and at two surface sites (Dodaira and Kisai) from the World Data Center for Greenhouse Gases (WDCGG).
RESULTS: We produce gridded estimates of the CO2 emissions and calculate the averages for different areas within the Kanto plain where Tokyo is located. Using these inversions as reference we investigate the impact of perturbing different elements in the inversion system. We modified the observations amount and location (surface only sparse vs. including aircraft CO2 observations), the background representation, the wind data used to drive the transport model, the prior emissions magnitude and time resolution and error parameters of the inverse model.
CONCLUSIONS: Optimized fluxes were consistent with other estimates for the unperturbed simulations. Inclusion of CONTRAIL measurements resulted in significant differences in the magnitude of the retrieved fluxes, 13% on average for the whole domain and of up to 21% for the spatiotemporal cells with the highest fluxes. Changes in the background yielded differences in the retrieved fluxes of up to 50% and more. Simulated biases in the modelled transport cause differences in the retrieved fluxes of up to 30% similar to those obtained using different meteorological winds to advect the Lagrangian trajectories. Perturbations to the prior inventory can impact the fluxes by ~ 10% or more depending on the assumptions on the error covariances. All of these factors can cause significant differences in the estimated flux, and highlight the challenges in estimating regional CO2 fluxes from atmospheric observations.

2019

Assessing air pollution from wood burning using low-cost sensors and citizen science

Castell, Nuria; Vogt, Matthias; Schneider, Philipp; Grossberndt, Sonja

2021

Ash generation and distribution from the April-May 2010 eruption of Eyjafjallajökull, Iceland.

Gudmundsson, M.T.; Thordarson, T.; Höskuldsson, A.; Larsen, G.; Björnsson, H.; Prata, F.J.; Oddsson, B.; Magnússon, E.; Högnadóttir, T.; Petersen, G.N.; Hayward, C.L.; Stevenson, J.A.; Jónsdóttir, I.

2012

ASCAT/SMOS data assimilation. NILU F

Lahoz, W.A.

2012

Artificial turf. Preliminary study on potential genotoxicity of nanoparticles generated from football pitches. NILU report

Rundén-Pran, E.; Dusinska, M.; El Yamani, N.; Dauge, F.; Knudsen, S.

2017

Artificial intelligence models with multivariate inputs for calibration of low cost PM sensors.

Topalovic, D. B.; Davidovic, M.; Bartonova, A.; Jovaševic-Stojanovic, M.

2017

Artificial intelligence models for calibration of low-cost electrochemical sensors in high-density air pollution monitoring networks.

Topalovic, D.B.; Ristovski, Z.; Bartonova, A.; Castell, N.; Davidovic, M.; Jovaševic-Stojanovic, M.

2016

Artificial cloud test confirms volcanic ash detection using infrared spectral imaging.

Prata, A.J.; Dezitter, F.; Davies, I.; Weber, K.; Birnfeld, M.; Moriano, D.; Bernardo, C.; Vogel, A.; Prata, G.S.; Mather, T.A.; Thomas, H.E.; Cammas, J.; Weber, M.

2016

Arktis brenner! Hvordan kanadiske skogbranner påvirker oss alle.

Stebel, Kerstin; Eckhardt, Sabine; Evangeliou, Nikolaos; Schneider, Philipp

2023

Arealutslipp for Oslo. NILU OR

Sundvor, I.

Arelautslippene som benyttes for spredningsberegninger for Oslo er gjennomgått og endret utifra trender og ny tilgjengelig informasjon. Som resultat ble det flere kildekategorier enn tidligere og totalutslippet har økt.

2014

Are Sterols Useful for the Identification of Sources of Faecal Contamination in Shellfish? A Case Study.

Florini, Styliano; Shahsavari, Esmaeil; Aburto-Medina, Arturo; Khudur, Leadin S.; Mudge, Stephen Michael; Smith, David J.; Ball, Andrew S.

This work aimed to identify the major source(s) of faecal pollution impacting Salcott Creek oyster fisheries in the UK through the examination of the sterol profiles. The concentration of the major sewage biomarker, coprostanol, in water overlying the oysters varied between 0.01 µg L−1 and 1.20 µg L−1. The coprostanol/epicoprostanol ratio ranged from 1.32 (September) to 33.25 (February), suggesting that human sewage represents the key input of faecal material into the estuary. However, a correlation between the sterol profile of water above the oysters with that of water that enters from Tiptree Sewage Treatment Works (r = 0.82), and a sample from a site (Quinces Corner) observed to have a high population of Brent geese (r = 0.82), suggests that both sources contribute to the faecal pollution affecting the oysters. In identifying these key faecal inputs, sterol profiling has allowed targeted management practices to be employed to ensure that oyster quality is optimised.

2020

Are poly(anhydride) nanoparticles really safe?

Alonso, T. I.; El Yamani, N.; Dusinska, M.; Salsamendi, A. L.; Oscoz, A. A.

2016

Are poly(anhydride) nanoparticles really safe?

Alonso, T.I.; El Yamani, N.; Dusinska, M.; Salsamendi, A.L.; Oscoz, A.A.

2016

Are parents driving air pollution at schools?

Grythe, Henrik; Santos, Gabriela Sousa; Castell, Nuria

2024

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