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Applications of low-cost sensing technologies for air quality monitoring and exposure assessment: How far have they gone?

Morawska, Lidia; Thai, Phong K.; Liu, Xiaoting; Asumadu-Sakyi, Akwasi; Ayoko, Godwin; Bartonova, Alena; Bedini, Andrea; Chai, Fahe; Christensen, Bryce; Dunbabin, Matthew; Gao, Jian; Hagler, Gayle S. W.; Jayaratne, Rohan; Kumar, Prashant; Lau, Alexis K. H.; Louie, Peter K. K.; Mazaheri, Mandana; Ning, Zhi; Motta, Nunzio; Mullins, Ben; Rahman, Md Mahmudur; Ristovski, Zoran; Shafiei, Mahnaz; Tjondronegoro, Dian; Westerdahl, Dane; Williams, Ron

2018

Webcrawling and machine learning as a new approach for the spatial distribution of atmospheric emissions

Lopez-Aparicio, Susana; Grythe, Henrik; Vogt, Matthias; Pierce, Matthew; Vallejo, Islen

In this study we apply two methods for data collection that are relatively new in the field of atmospheric science. The two developed methods are designed to collect essential geo-localized information to be used as input data for a high resolution emission inventory for residential wood combustion (RWC). The first method is a webcrawler that extracts openly online available real estate data in a systematic way, and thereafter structures them for analysis. The webcrawler reads online Norwegian real estate advertisements and it collects the geo-position of the dwellings. Dwellings are classified according to the type (e.g., apartment, detached house) they belong to and the heating systems they are equipped with. The second method is a model trained for image recognition and classification based on machine learning techniques. The images from the real estate advertisements are collected and processed to identify wood burning installations, which are automatically classified according to the three classes used in official statistics, i.e., open fireplaces, stoves produced before 1998 and stoves produced after 1998. The model recognizes and classifies the wood appliances with a precision of 81%, 85% and 91% for open fireplaces, old stoves and new stoves, respectively. Emission factors are heavily dependent on technology and this information is therefore essential for determining accurate emissions. The collected data are compared with existing information from the statistical register at county and national level in Norway. The comparison shows good agreement for the proportion of residential heating systems between the webcrawled data and the official statistics. The high resolution and level of detail of the extracted data show the value of open data to improve emission inventories. With the increased amount and availability of data, the techniques presented here add significant value to emission accuracy and potential applications should also be considered across all emission sectors.

2018

Temporal variability in surface water pCO2 in Adventfjorden (West Spitsbergen) with emphasis on physical and biogeochemical drivers

Ericson, Ylva; Falck, Eva; Chierici, Melissa; Fransson, Agneta Ingrid; Kristiansen, Svein; Platt, Stephen Matthew; Hermansen, Ove; Myhre, Cathrine Lund

Seasonal and interannual variability in surface water partial pressure of CO2 (pCO2) and air‐sea CO2 fluxes from a West Spitsbergen fjord (IsA Station, Adventfjorden) are presented, and the associated driving forces are evaluated. Marine CO2 system data together with temperature, salinity, and nutrients, were collected at the IsA Station between March 2015 and June 2017. The surface waters were undersaturated in pCO2 with respect to atmospheric pCO2 all year round. The effects of biological activity (primary production/respiration) followed by thermal forcing on pCO2 were the most important drivers on a seasonal scale. The ocean was a sink for atmospheric CO2 with annual air‐sea CO2 fluxes of −36 ± 2 and −31 ± 2 g C·m−2·year−1 for 2015–2016 and 2016–2017, respectively, as estimated from the month of April. Waters of an Arctic origin dominated in 2015 and were replaced in 2016 by waters of a transformed Atlantic source. The CO2 uptake rates over the period of Arctic origin waters were significantly higher (2 mmol C·m−2·day−1) than the rates of the Atlantic origin waters of the following year.

2018

Emerging pollutants in the EU: 10 years of NORMAN in support of environmental policies and regulations

Dulio, Valeria; Bavel, Bert van; Broström-Lundén, Eva; Harmsen, Joop; Hollender, Juliane; Schlabach, Martin; Slobodnik, Jaroslav; Thomas, Kevin; Koschorreck, Jan

In 2005, the European Commission funded the NORMAN project to promote a permanent network of reference laboratories and research centers, including academia, industry, standardization bodies, and NGOs. Since then, NORMAN has (i) facilitated a more rapid and wide-scope exchange of data on the occurrence and effects of contaminants of emerging concern (CECs), (ii) improved data quality and comparability via validation and harmonization of common sampling and measurement methods (chemical and biological), (iii) provided more transparent information and monitoring data on CECs, and (iv) established an independent and competent forum for the technical/scientific debate on issues related to emerging substances. NORMAN plays a significant role as an independent organization at the interface between science and policy, with the advantage of speaking to the European Commission and other public institutions with the “bigger voice” of more than 70 members from 20 countries. This article provides a summary of the first 10 years of the NORMAN network. It takes stock of the work done so far and outlines NORMAN’s vision for a Europe-wide collaboration on CECs and sustainable links from research to policy-making. It contains an overview of the state of play in prioritizing and monitoring emerging substances with reference to several innovative technologies and monitoring approaches. It provides the point of view of the NORMAN network on a burning issue—the regulation of CECs—and presents the positions of various stakeholders in the field (DG ENV, EEA, ECHA, and national agencies) who participated in the NORMAN workshop in October 2016. The main messages and conclusions from the round table discussions are briefly presented.

2018

Higher plasma oxidative damage and lower plasma antioxidant defences in an Arctic seabird exposed to longer perfluoroalkyl acids

Costantini, David; Blévin, Pierre; Herzke, Dorte; Moe, Børge; Gabrielsen, Geir W.; Bustnes, Jan Ove; Chastel, Olivier

2018

Organic micropollutants in the riverine sedimentsalong the lower stretch of the River Ganga: Occurrences, sources and risk assessment

Chakraborty, Paromita; Mukhopadhyay, Moitraiyee; Sampath, Srimurali; Ramaswamy, BabuRajendran; Katsoyiannis, Athanasios A.; Cincinelli, Alessandra; Snow, Daniel

2018

The comet assay applied to cells of the eye

Azqueta, Amaya; Rundén-Pran, Elise; Elje, Elisabeth; Nicolaissen, Bjørn; Haug, Kristiane; Smeringaiova, Ingrida; Jirsova, Katerina; Collins, Andrew Richard

2018

A satellite-based estimate of combustion aerosol cloud microphysical effects over the Arctic Ocean

Zamora, Lauren M; Kahn, Ralph A.; Huebert, Klaus B; Stohl, Andreas; Eckhardt, Sabine

Climate predictions for the rapidly changing Arctic are highly uncertain, largely due to a poor understanding of the processes driving cloud properties. In particular, cloud fraction (CF) and cloud phase (CP) have major impacts on energy budgets, but are poorly represented in most models, often because of uncertainties in aerosol–cloud interactions. Here, we use over 10 million satellite observations coupled with aerosol transport model simulations to quantify large-scale microphysical effects of aerosols on CF and CP over the Arctic Ocean during polar night, when direct and semi-direct aerosol effects are minimal. Combustion aerosols over sea ice are associated with very large (∼ 10Wm−2) differences in longwave cloud radiative effects at the sea ice surface. However, co-varying meteorological changes on factors such as CF likely explain the majority of this signal. For example, combustion aerosols explain at most 40% of the CF differences between the full dataset and the clean-condition subset, compared to between 57% and 91% of the differences that can be predicted by co-varying meteorology. After normalizing for meteorological regime, aerosol microphysical effects have small but significant impacts on CF, CP, and precipitation frequency on an Arctic-wide scale. These effects indicate that dominant aerosol–cloud microphysical mechanisms are related to the relative fraction of liquid-containing clouds, with implications for a warming Arctic.

2018

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