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Modelling the coupled mercury-halogen-ozone cycle in the central Arctic during spring

Ahmed, Shaddy; Thomas, Jennie L.; Angot, Hélène; Dommergue, Aurélien; Archer, Stephen D.; Bariteau, Ludovic; Beck, Ivo; Benavent, Nuria; Blechschmidt, Anne-Marlene; Blomquist, Byron; Boyer, Matthew; Christensen, Jesper H.; Dahlke, Sandro; Dastoor, Ashu; Helmig, Detlev; Howard, Dean; Jacobi, Hans-Werner; Jokinen, Tuija; Lapere, Rémy; Laurila, Tiia; Quéléver, Lauriane L.J.; Richter, Andreas; Ryjkov, Andrei; Mahajan, Anoop S.; Marelle, Louis; Pfaffhuber, Katrine Aspmo; Posman, Kevin; Rinke, Annette; Saiz-Lopez, Alfonso; Schmale, Julia; Skov, Henrik; Steffen, Alexandra; Stupple, Geoff; Stutz, Jochen; Travnikov, Oleg; Zilker, Bianca

Near-surface mercury and ozone depletion events occur in the lowest part of the atmosphere during Arctic spring. Mercury depletion is the first step in a process that transforms long-lived elemental mercury to more reactive forms within the Arctic that are deposited to the cryosphere, ocean, and other surfaces, which can ultimately get integrated into the Arctic food web. Depletion of both mercury and ozone occur due to the presence of reactive halogen radicals that are released from snow, ice, and aerosols. In this work, we added a detailed description of the Arctic atmospheric mercury cycle to our recently published version of the Weather Research and Forecasting model coupled with Chemistry (WRF-Chem 4.3.3) that includes Arctic bromine and chlorine chemistry and activation/recycling on snow and aerosols. The major advantage of our modelling approach is the online calculation of bromine concentrations and emission/recycling that is required to simulate the hourly and daily variability of Arctic mercury depletion. We used this model to study coupling between reactive cycling of mercury, ozone, and bromine during the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) spring season in 2020 and evaluated results compared to land-based, ship-based, and remote sensing observations. The model predicts that elemental mercury oxidation is driven largely by bromine chemistry and that particulate mercury is the major form of oxidized mercury. The model predicts that the majority (74%) of oxidized mercury deposited to land-based snow is re-emitted to the atmosphere as gaseous elemental mercury, while a minor fraction (4%) of oxidized mercury that is deposited to sea ice is re-emitted during spring. Our work demonstrates that hourly differences in bromine/ozone chemistry in the atmosphere must be considered to capture the springtime Arctic mercury cycle, including its integration into the cryosphere and ocean.

2023

Accurate Lightweight Calibration Methods for Mobile Low-Cost Particulate Matter Sensors

Jørstad, Per Martin; Wojcikowski, Marek; Cao, Tuan-Vu; Lepioufle, Jean-Marie; Wojtkiewicz, Krystian; Ha, Hoai Phuong

2023

Organizing the Indicator Zoo: Can a New Taxonomy Make It Easier for Citizen Science Data to Contribute to the United Nations Sustainable Development Goal Indicators?

Grossberndt, Sonja; Graff, Geir; Bartonova, Alena; Volchkova, Iuliia; Evensen, Thomas

In order to measure progress towards the aims outlined by the United Nations (UN) 2030 Agenda, data are needed for the different indicators that are linked to each UN Sustainable Development Goal (SDG). Where statistical or scientific data are not sufficient or available, alternative data sources, such as data from citizen science (CS) activities, could be used.

Statistics Norway, together with the Norwegian Association of Local and Regional Authorities, have developed a taxonomy for classifying indicators that are intended to measure the SDGs. The purpose of this taxonomy is to sort, evaluate, and compare different SDG indicators and to assess their usefulness by identifying their central properties and characteristics. This is done by organizing central characteristics under the three dimensions of Goal, Perspective, and Quality. The taxonomy is designed in a way that can help users to find the right indicators across sectors to measure progress towards the SDGs depending on their own context and strategic priorities. The Norwegian taxonomy also offers new opportunities for the re-use of data collected through CS activities. This paper presents the taxonomy and demonstrates how it can be applied for an indicator based on a CS data set, and we also suggest further use of CS data.

Ubiquity Press

2023

Circular economy for aquatic food systems: insights from a multiscale phosphorus flow analysis in Norway

Pandit, Avijit Vinayak; Dittrich, Nils Maximilian; Strand, Andrea Viken; Lozach, Loïs; Las Heras Hernandez, Miguel; Reitan, Kjell Inge; Mueller, Daniel Beat

As wild-caught fish become scarce, feed ingredients for farming fish, such as salmon, are increasingly sourced from agricultural plants that depend on mineral fertilizers. Since these fish are naturally carnivorous, they have difficulty digesting the phosphorus in plant-based feed. So additional phosphorus supplements are added to the feed, resulting in a disproportionate increase in mineral phosphorus use and emission. Aquatic food production is increasingly relying on agriculture and mineral phosphorus resources. The feed surplus and the excreta are seldom collected and recycled, leading to a massive loss of nutrients to water bodies and the seafloor, resulting in local risk for eutrophication. Norway currently produces more than half of the world’s Atlantic salmon, and it is set to increase production from currently 1.5 to 5 Mt. in 2050. This has large implications for feed supply and emissions globally. There is a lack of studies that analyze the phosphorus system in aquatic food production at a sufficient spatial and temporal granularity to effectively inform interventions for a more circular use of phosphorus. Here, we present a multi-scale phosphorus flow analysis at monthly resolution ranging between 2005 and 2021 for aquatic food production in Norway and quantitatively discuss the effectiveness of alternative strategies for improving resource efficiency. The results indicate that P emissions from aquaculture have nearly doubled in the period between 2005 and 2021. The P use efficiency (PUE) in Norwegian aquaculture was 19% in 2021. The addition of phytase to the feed could improve the PUE by 8% by reducing P supplements and emissions by 7 kt/y. The use of Integrated Multi-Trophic Aquaculture close to fish farming sites could absorb emissions by 4 kt/y by creating new marine food products. Sludge collection systems could reduce P emissions by 4 to 11 kt/y, depending on the technology. Using the sludge in local agriculture would exacerbate the current P accumulation in soils close to the coastline, given that the animal density in this region is already high. Hence, a large and sophisticated processing infrastructure will be needed to create transportable, high-quality secondary fertilizers for effective sludge recycling in regions with a P deficit.

Frontiers Media S.A.

2023

Skogens helsetilstand i Norge. Resultater fra skogskadeovervåkingen i 2022

Timmermann, Volkmar; Børja, Isabella; Clarke, Nicholas; Gohli, Jostein; Hietala, Ari Mikko; Jepsen, Jane Uhd; Krokene, Paal; Lislegård, Harald Haga; Nagy, Nina Elisabeth; Nyeggen, Hans; Solberg, Sverre; Solheim, Halvor; Solvin, Thomas Mørtvedt; Svensson, Arvid; Tollefsrud, Mari Mette; Vindstad, Ole Petter Laksforsmo; Økland, Bjørn; Aas, Wenche

Skogens helsetilstand påvirkes i stor grad av klima og værforhold, enten direkte ved tørke, frost og vind, eller indirekte ved at klimaet påvirker omfanget av soppsykdommer og insektangrep. Klimaendringene og den forventede økningen i klimarelaterte skogskader gir store utfordringer for forvaltningen av framtidas skogressurser. Det samme gjør invaderende skadegjørere, både allerede etablerte arter og nye som kan komme til Norge i nær framtid. I denne rapporten presenteres resultater fra skogskadeovervåkingen i Norge i 2022 og trender over tid for følgende temaer:
(i) Landsrepresentativ skogovervåking;
(ii) Intensiv skogovervåking;
(iii) Overvåking av bjørkemålere i Troms og Finnmark;
(iv) Barkbilleovervåkingen;
(v) Furuvednematode;
(vi) Askeskuddsyke;
(vii) Andre spesielle skogskader i 2022.

NIBIO

2023

The Impacts of Third Pole Snow Assimilation on Seasonal Meteorology Predictions

Li, Wei; Li, Lu; Jie, Chen; Orsolini, Yvan Joseph Georges Emile G.; de Rosnay, Patricia; Senan, Retish

2023

Røyk fra Canada kommer fortsatt inn over Norge

Solbakken, Christine Forsetlund

Norges forskningsråd

2023

Forecast products for BC and dust

Evangeliou, Nikolaos; Eckhardt, Sabine; Zwaaftink, Christine Groot; Sollum, Espen

2023

Observations and Retrievals of Volcanic Ash Clouds Using Ground- and Satellite-Based Sensors

Mereu, Luigi; Scollo, Simona; Bonadonna, Costanza; Corradini, Stefano; Donnadieu, Franck; Montopoli, Mario; Vulpiani, Gianfranco; Barsotti, Sara; Freret-Lorgeril, Valentin; Gudmundsson, Magnús Tumi; Kylling, Arve; Ripepe, Maurizio

2023

Accurate Lightweight Calibration Methods for Mobile Low-Cost Particulate Matter Sensors

Jørstad, Per Martin; Wojcikowski, Marek; Cao, Tuan-Vu; Lepioufle, Jean-Marie; Wojtkiewicz, Krystian; Ha, Hoai Phuong

2023

Long-term observations of aerosol optical depth and their relation to in-situ aerosol properties in the Svalbard region (LOAD-RIS)

Hansen, Georg H.; Kouremeti, Natalia; Gilardoni, Stefania; Stebel, Kerstin; Evangeliou, Nikolaos; Ritter, Christoph; Zielinski, Tymon; Herrero, Sara; Kazadzis, Stelios; Mateos, David; Mazzola, Mauro; Pakszys, Paulina; Eleftheriadis, Konstantinos

Aerosols are an important constituent of the atmosphere both influencing the climate system and contributing to increasing pollution of the Arctic. At the same time, their adequate monitoring is a big challenge, as instruments on the ground only can sample aerosols in the lowermost atmosphere. For this reason, these measurements are complemented with observations of aerosol optical depth (AOD) which quantify the total amount of aerosols throughout the atmosphere from the attenuation of direct sunlight (and moonlight). This procedure requires extremely careful instrument calibration and removal of cloud contaminated data. In Svalbard, such measurements have been performed by several research groups with different instruments, mostly in Ny-Ålesund and in Hornsund, but also on research vessels offshore. In the framework of the SSF Strategic Grant project ReHearsol, all AOD data from the Svalbard region since 2002 have been collected and made available to the SIOS research community. They indicate that number and intensity of Arctic haze episodes occurring in late winter and spring have decreased consistently and significantly in the last 20 years, while pollution events in summer/early autumn, caused by boreal biomass burning, are on the rise, though not as consistently. Comparison between in-situ measurements at Gruvebadet Atmosphere Laboratory in Ny-Ålesund and AOD measurements indicate that most (more than 65%) of the episodes with high aerosol load are not captured by surface measurements. This finding does not change when one includes in-situ measurements at Zeppelin Observatory (475 m a.s.l.). Studying extensive high-AOD episodes such as those in summer 2019 requires a multi-tool approach including in-situ and remote-sensing measurements combined with model tools.

2023

Gigant-skogbranner kan ses fra verdensrommet – røykpartikler har nådd Norge

Evangeliou, Nikolaos (intervjuobjekt); Berger, Nina Dayana (journalist)

2023

Emerging pollutants in the Arctic environment

Kallenborn, Roland; Ali, Aasim Musa Mohamed; Drotikova, Tatiana; Hartz, William Frederik

2023

Renere luft i Longyearbyen

Grythe, Henrik (intervjuobjekt); Krüger, Louise (journalist)

2023

Impacts of a warming climate on concentrations of organochlorines in a fasting high arctic marine bird: Direct vs. indirect effects?

Bustnes, Jan Ove; Bårdsen, Bård-Jørgen; Moe, Børge; Herzke, Dorte; Ballesteros, Manuel; Fenstad, Anette; Borgå, Katrine; Krogseth, Ingjerd Sunde; Eulaers, Igor; Skogeng, Lovise Pedersen; Gabrielsen, Geir Wing; Hanssen, Sveinn Are

The present study examined how climate changes may impact the concentrations of lipophilic organochlorines (OCs) in the blood of fasting High Arctic common eiders (Somateria mollissima) during incubation. Polychlorinated biphenyls (PCBs), 1-dichloro-2,2-bis (p-chlorophenyl) ethylene (p,p′-DDE), hexachlorobenzene (HCB) and four chlordane compounds (oxychlordane, trans-chlordane and trans- and cis-nonachlor) were measured in females at chick hatching (n = 223) over 11 years (2007–2017). Firstly, median HCB and p,p′-DDE concentrations increased ~75 % over the study period, whereas median chlordane concentrations doubled (except for oxychlordane). PCB concentrations, in contrast, remained stable over the study period. Secondly, both body mass and clutch size were negatively associated with OC levels, suggesting that females with high lipid metabolism redistributed more OCs from adipose tissue, and that egg production is an important elimination route for OCs. Thirdly, the direct climate effects were assessed using the mean effective temperature (ET: air temperature and wind speed) during incubation, and we hypothesized that a low ET would increase redistribution of OCs. Contrary to expectation, the ET was positively correlated to most OCs, suggesting that a warmer climate may lead to higher OCs levels, and that the impact of ET may not be direct. Finally, potential indirect impacts were examined using the Arctic Oscillation (AO) in the three preceding winters (AOwinter 1–3) as a proxy for potential long-range transport of OCs, and for local spring climate conditions. In addition, we used chlorophyll a (Chla) as a measure of spring primary production. There were negative associations between AOwinter 1 and HCB, trans-chlordane and trans-nonachlor, whereas oxychlordane and cis-chlordane were negatively associated with Chla. This suggests that potential indirect climate effects on eiders were manifested through the food chain and not through increased long-range transport, although these relationships were relatively weak.

Elsevier

2023

Hierarchical Clustering and Dissimilarity Polygon Analyses. Optimizing the Polish Deposition Network.

Soares, Joana; Aas, Wenche; Eckhardt, Sabine; Guerreiro, Cristina

The potential re-design of the current deposition monitoring network in Poland was assessed by hierarchical clustering analysis. This statistical method determines the inherent or natural groupings of datasets, and/or to provide a summarization of data into groups using different metrics to assess the (di)similarity. The metrics are based on the correlation, to assess the temporal similarity, the Euclidean distance, to assess the magnitude similarity, and the combination of both. This method was used to assess the areas with similar deposition patters across the country based on measurement and model data for acidic compounds and heavy metals. The analysis clearly identified stations potentially redundant or measuring unique deposition patters and regions that represent the potential location of a single station.

NILU

2023

Sources and atmospheric dispersion of microplastics in the Norwegian territory

Gossmann, Isabel; Herzke, Dorte; Held, Andreas; Schulz, Janina; Nikiforov, Vladimir; Georgi, Christoph; Evangeliou, Nikolaos; Eckhardt, Sabine; Gerdts, Gunnar; Wurl, Oliver; Scholz-Böttcher, Barbara

2023

Fate of Anthropogenic Particles in Arctic Waters around Svalbard

Philipp, Carolin; Collard, France; Husum, Katrine; Herzke, Dorte; Halsband, Claudia; Gabrielsen, Geir Wing; Hallanger, Ingeborg G.

2023

Copernicus Atmosphere Monitoring Service. Interim Annual Assessment Report on European Air Quality in 2022

Hamer, Paul David; Fjæraa, Ann Mari; Tarrasón, Leonor; Soares, Joana; Meleux, Frédérik; Colette, Augustin; Ung, Anthony; Raux, Blandine; Kuenen, Jeroen

Copernicus Atmosphere Monitoring Service

2023

Genotoxic effects of occupational exposure to glass fibres - A human biomonitoring study.

Ceppi, Marcello; Smolkova, Bozena ; Staruchova, Marta; Kazimirova, Alena; Barancokova, Magdalena; Volkovova, Katarina; Collins, Andrew Richard; Kocan, Anton; Dzupinkova, Zuzana; Horska, Alexandra; Buocikova, Verona; Tulinska, Jana; Liskova, Aurelia; Mikusova, Miroslava Lehotska; Krivosikova, Zora; Wsolova, Ladislava; Kuba, Daniel; Rundén-Pran, Elise; El Yamani, Naouale; Longhin, Eleonora Marta; Halasova, Erika; Kyrtopoulos, Soterios; Bonassi, Stefano ; Dusinska, Maria

As part of a large human biomonitoring study, we conducted occupational monitoring in a glass fibre factory in Slovakia. Shopfloor workers (n = 80), with a matched group of administrators in the same factory (n = 36), were monitored for exposure to glass fibres and to polycyclic aromatic hydrocarbons (PAHs). The impact of occupational exposure on chromosomal aberrations, DNA damage and DNA repair, immunomodulatory markers, and the role of nutritional and lifestyle factors, as well as the effect of polymorphisms in metabolic and DNA repair genes on genetic stability, were investigated.

The (enzyme-modified) comet assay was employed to measure DNA strand breaks (SBs) and apurinic sites, oxidised and alkylated bases. Antioxidant status was estimated by resistance to H2O2-induced DNA damage. Base excision repair capacity was measured with an in vitro assay (based on the comet assay).

Exposure of workers to fibres was low, but still was associated with higher levels of SBs, and SBs plus oxidised bases, and higher sensitivity to H2O2. Multivariate analysis showed that exposure increased the risk of high levels of SBs by 20%. DNA damage was influenced by antioxidant enzymes catalase and glutathione S-transferase (measured in blood). DNA repair capacity was inversely correlated with DNA damage and positively with antioxidant status. An inverse correlation was found between DNA base oxidation and the percentage of eosinophils (involved in the inflammatory response) in peripheral blood of both exposed and reference groups. Genotypes of XRCC1 variants rs3213245 and rs25487 significantly decreased the risk of high levels of base oxidation, to 0.50 (p = 0.001) and 0.59 (p = 0.001), respectively.

Increases in DNA damage owing to glass fibre exposure were significant but modest, and no increases were seen in chromosome aberrations or micronuclei. However, it is of concern that even low levels of exposure to these fibres can cause significant genetic damage.

2023

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