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On the tuning of atmospheric inverse methods: comparisons with the European Tracer Experiment (ETEX) and Chernobyl datasets using the atmospheric transport model FLEXPART

Tichý, Ondřej; Ulrych, Lukas; Šmídl, Václav; Evangeliou, Nikolaos; Stohl, Andreas

Estimation of the temporal profile of an atmospheric release, also called the source term, is an important problem in environmental sciences. The problem can be formalized as a linear inverse problem wherein the unknown source term is optimized to minimize the difference between the measurements and the corresponding model predictions. The problem is typically ill-posed due to low sensor coverage of a release and due to uncertainties, e.g., in measurements or atmospheric transport modeling; hence, all state-of-the-art methods are based on some form of regularization of the problem using additional information. We consider two kinds of additional information: the prior source term, also known as the first guess, and regularization parameters for the shape of the source term. While the first guess is based on information independent of the measurements, such as the physics of the potential release or previous estimations, the regularization parameters are often selected by the designers of the optimization procedure. In this paper, we provide a sensitivity study of two inverse methodologies on the choice of the prior source term and regularization parameters of the methods. The sensitivity is studied in two cases: data from the European Tracer Experiment (ETEX) using FLEXPART v8.1 and the caesium-134 and caesium-137 dataset from the Chernobyl accident using FLEXPART v10.3.

2020

Legacy and emerging flame retardants (FRs) in the urban atmosphere of Pakistan: Diurnal variations, gas-particle partitioning and human health exposure

Syed, Jabir Hussain; Iqbal, Mehreen; Breivik, Knut; Chaudhry, Muhammad Jamshed Iqbal; Shahnawaz, Muhammad; Abbas, Zaigham; Nasir, Jawad; Rizvi, Syed Hussain Haider; Taqi, Malik Mumtaz Hussain; Li, Jun; Zhang, Gan

2020

Anthropogenic, Direct Pressures on Coastal Wetlands

Newton, Alice; Icely, John; Cristina, Sónia; Perillo, Gerardo M.; Turner, R. Eugene; Ashan, Dewan; Cragg, Simon; Luo, Yongming; Tu, Chen; Li, Yuan; Zhang, Haibo; Ramesh, Ramachandran; Forbes, Donald L.; Solidoro, Cosimo; Béjaoui, Béchir; Gao, Shu; Pastres, Roberto; Kelsey, Heath; Taillie, Dylan; Nhan, Nguyen; Brito, Ana C; Lima, Ricardo de; Kuenzer, Claudia

Coastal wetlands, such as saltmarshes and mangroves that fringe transitional waters, deliver important ecosystem services that support human development. Coastal wetlands are complex social-ecological systems that occur at all latitudes, from polar regions to the tropics. This overview covers wetlands in five continents. The wetlands are of varying size, catchment size, human population and stages of economic development. Economic sectors and activities in and around the coastal wetlands and their catchments exert multiple, direct pressures. These pressures affect the state of the wetland environment, ecology and valuable ecosystem services. All the coastal wetlands were found to be affected in some ways, irrespective of the conservation status. The main economic sectors were agriculture, animal rearing including aquaculture, fisheries, tourism, urbanization, shipping, industrial development and mining. Specific human activities include land reclamation, damming, draining and water extraction, construction of ponds for aquaculture and salt extraction, construction of ports and marinas, dredging, discharge of effluents from urban and industrial areas and logging, in the case of mangroves, subsistence hunting and oil and gas extraction. The main pressures were loss of wetland habitat, changes in connectivity affecting hydrology and sedimentology, as well as contamination and pollution. These pressures lead to changes in environmental state, such as erosion, subsidence and hypoxia that threaten the sustainability of the wetlands. There are also changes in the state of the ecology, such as loss of saltmarsh plants and seagrasses, and mangrove trees, in tropical wetlands. Changes in the structure and function of the wetland ecosystems affect ecosystem services that are often underestimated. The loss of ecosystem services impacts human welfare as well as the regulation of climate change by coastal wetlands. These cumulative impacts and multi-stressors are further aggravated by indirect pressures, such as sea-level rise.

2020

Environmental behaviour and bioaccumulation of chlorinated paraffins, dechloranes and PCBs in northern freshwater ecosystems

Arriola, Aline; Krogseth, Ingjerd Sunde; Warner, Nicholas Alexander; Herzke, Dorte; Evenset, Anita; Möckel, Claudia; Breivik, Knut

2020

SEN4POL – Towards a Sentinel-based pollen information service

Schneider, Philipp; Hamer, Paul David; Vogt, Matthias; Trier, Øivind Due; Solberg, Rune; Skogesal, Hogne; Brobakk, Trond Einar; Ramfjord, Hallvard

2020

Grenseverdier for organiske miljøgifter i gjødselvarer - hvordan etablere det?

Eggen, Trine; Heimstad, Eldbjørg Sofie; Nikiforov, Vladimir; Vogelsang, Christian

2020

Hva skjedde med diesel-forbudet?

Høiskar, Britt Ann Kåstad (intervjuobjekt); Fossum, Øystein B. (journalist)

2020

Nytt, stort hull i ozonlaget

Hansen, Georg H. (intervjuobjekt); Tønset, Arne Egil (journalist)

2020

How to COPE? Contaminant–climate change interactions in the Arctic.

Krogseth, Ingjerd Sunde; Solbakken, Christine Forsetlund; Borch, Trude

2020

Reflecting on Ethics of Nanosafety

Malsch, Ineke; Panagiotis, Isigonis; Bouman, Evert; Afantitis, Antreas; Melagraki, Georgia; Lynch, Iseult; Cimpan, Mihaela-Roxana; Dusinska, Maria

2020

Skogens helsetilstand i Norge. Resultater fra skogskadeovervåkingen i 2019

Timmermann, Volkmar; Andreassen, Kjell; Beachell, Andreas Myki; Børja, Isabella; Brurberg, May Bente; Clarke, Nicholas; Halvorsen, Rune; Hylen, Gro; Jepsen, Jane Uhd; Perminow, Juliana; Solberg, Sverre; Solheim, Halvor; Talgø, Venche; Tollefsrud, Mari Mette; Vindstad, Ole Petter Laksforsmo; Økland, Bjørn; Økland, Tonje; Aas, Wenche

Skogens helsetilstand påvirkes i stor grad av klima og værforhold, enten direkte ved tørke, frost og vind, eller indirekte ved at klimaet påvirker omfanget av soppsykdommer og insektangrep.
Klimaendringene og den forventede økningen i klimarelaterte skogskader gir store utfordringer for forvaltningen av framtidas skogressurser. Det samme gjør invaderende skadegjørere, både allerede etablerte arter og nye som kan komme til Norge i nær framtid. I denne rapporten presenteres
resultater fra skogskadeovervåkingen i Norge i 2019 og trender over tid.....

NIBIO

2020

An optimized comet-based in vitro DNA repair assay to assess base and nucleotide excision repair activity

Vodenkova, Sona; Azqueta, Amaya; Collins, Andrew Richard; Dusinska, Maria; Gaivao, Isabel; Møller, Peter; Opattová, Alena; Vodicka, Pavel; Godschalk, Roger W. L.; Langie, Sabine A.S.

2020

Development of an Adverse Outcome Pathway for Chronic and Multi-Generational Impacts of Nanomaterials in the Environmental Indicator Species Daphnia Magna

Lynch, Iseult; Reilly, Katie; Cimpan, Mihaela Roxana; Drønen, Anne-Marthe; Rios-Mondragon, Ivan; Cambier, Sébastien; Gutleb, Arno; Serchi, Tommaso; Dusinska, Maria; Rundén-Pran, Elise; Mariussen, Espen; Longhin, Eleonora Marta; Murugadoss, Sivakumar; Hoet, Peter; Willihagen, Egon; Martens, Marvin; Afantitis, Antreas; Melargakis, Georgia; Vrcek, Ivana Vincovik

2020

The Lagrangian particle dispersion model FLEXPART version 10.4

Pisso, Ignacio; Sollum, Espen; Grythe, Henrik; Kristiansen, Nina Iren; Cassiani, Massimo; Eckhardt, Sabine; Arnold, Delia; Morton, Don; Thompson, Rona Louise; Zwaaftink, Christine Groot; Evangeliou, Nikolaos; Sodemann, Harald; Haimberger, Leopold; Henne, Stephan; Brunner, Dominik; Burkhart, John; Fouilloux, Anne Claire; Brioude, Jerome; Philipp, Anne; Seibert, Petra; Stohl, Andreas

2020

Dropp vedfyring når du har hjemmekontor

Guerreiro, Cristina (intervjuobjekt); Pedersen, Lars Håkon (journalist)

2020

MetVed v.2.0. Improvement and update of the MetVed emission model for residential wood combustion

Grythe, Henrik; Lopez-Aparicio, Susana

This report presents the update of the MetVed-model (Grythe et al., 2019). Among the updates are new emission factors and several new species that include climate gases (CO2, CH4 and N2O). There is now a new parameter that describes the emission altitude and a new and improved time variation. Activity data has been updated to the most recent year (2019), which also has required updates to the model and model input variables. The largest update has been the holiday cabin emission module, which is an entirely new addition. Emissions from cabins differ in several ways from residential emissions. The most notable difference is that cabins are spread over more rural areas and are more dispersed than the residential dwellings. The model differentiates alpine and coastal cabins, which is an important distinction as a high density of cabins exists along the coast and they are mainly used during summer.

NILU

2020

A life cycle perspective on the benefits of renewable electricity generation – Methodology and assumptions

Bouman, Evert

This report details the methodology and assumptions for the ETC/CME report: A life cycle perspective on the benefits of renewable electricity generation. In that report, gross avoided potential environmental impacts are estimated for electricity production in the EU-27 in the period 2005-2018. Avoided potential impacts are calculated by comparing the actual data with a counterfactual scenario where electricity production from Renewable Energy Sources is frozen at 2005 levels.

The overall methodological approach to the study is described in this report together with a short mathematical treatment of the calculation of life cycle indicators and subsequent scaling up to produce the two scenarios required to estimate gross avoided potential impacts. A short overview of data sources used in the study is included as well as a discussion and recommendations for the future.

ETC/CME

2020

Atmospheric Supply of Nitrogen, Cadmium, Lead, Mercury, PCDD/Fs, PCB-153, and B(a)P to the Baltic Sea EMEP/MSC-W Report for HELCOM

Gauss, Michael; Gusev, Alexey; Aas, Wenche; Hjellbrekke, Anne-Gunn; Ilyin, Ilia; Klein, Heiko; Nyiri, Agnes; Rozovskaya, Olga; Shatalov, Victor; Strijkina, Irina; Travnikov, Oleg

Norwegian Meteorological Institute

2020

Cyclic and Linear Siloxanes in Indoor Environments: Occurence and Human Exposure

Cincinelli, A.; Martellini, T.; Scodellini, R.; Scopetani, C.; Guerranti, C.; Katsoyiannis, Athanasios A.

2020

Final report, on-going key comparison BIPM.QM-K1, ozone at ambient level, comparison with NILU, January 2018

Viallon, Joële; Idrees, Faraz; Moussay, Philippe; Wielgosz, Robert; Marsteen, Leif

As part of the ongoing key comparison BIPM.QM-K1, a comparison has been performed between the ozone standard of Norway maintained by the Norwegian Institute for Air Research (NILU) and the common reference standard of the key comparison, maintained by the Bureau International des Poids et Mesures (BIPM). The instruments have been compared over a nominal ozone amount-of-substance fraction range from 0 nmol/mol to 500 nmol/mol.

2020

Strategies for grouping per- and polyfluoroalkyl substances (PFAS) to protect human and environmental health

Cousins, Ian T.; DeWitt, Jamie C.; Glüge, Juliane; Goldenman, Gretta; Herzke, Dorte; Lohmann, Rainer; Miller, Mark; Ng, Carla A.; Scheringer, Martin; Vierke, Lena; Wang, Zhanyun

Grouping strategies are needed for per- and polyfluoroalkyl substances (PFAS), in part, because it would be time and resource intensive to test and evaluate the more than 4700 PFAS on the global market on a chemical-by-chemical basis. In this paper we review various grouping strategies that could be used to inform actions on these chemicals and outline the motivations, advantages and disadvantages for each. Grouping strategies are subdivided into (1) those based on the intrinsic properties of the PFAS (e.g. persistence, bioaccumulation potential, toxicity, mobility, molecular size) and (2) those that inform risk assessment through estimation of cumulative exposure and/or effects. The most precautionary grouping approach of those reviewed within this article suggests phasing out PFAS based on their high persistence alone (the so-called “P-sufficient” approach). The least precautionary grouping approach reviewed advocates only grouping PFAS for risk assessment that have the same toxicological effects, modes and mechanisms of action, and elimination kinetics, which would need to be well documented across different PFAS. It is recognised that, given jurisdictional differences in chemical assessment philosophies and methodologies, no one strategy will be generally acceptable. The guiding question we apply to the reviewed grouping strategies is: grouping for what purpose? The motivation behind the grouping (e.g. determining use in products vs. setting guideline levels for contaminated environments) may lead to different grouping decisions. This assessment provides the necessary context for grouping strategies such that they can be adopted as they are, or built on further, to protect human and environmental health from potential PFAS-related effects.

2020

Reducing sampling artifacts in active air sampling methodology for remote monitoring and atmospheric fate assessment of cyclic volatile methylsiloxanes

Warner, Nicholas Alexander; Nikiforov, Vladimir; Krogseth, Ingjerd Sunde; Bjørneby, Stine Marie; Kierkegaard, Amelie; Bohlin-Nizzetto, Pernilla

Active sampling methodology for atmospheric monitoring of cyclic volatile methylsiloxanes (cVMS) was improved to reduce sampling artifacts. A new sorbent, ABN Express (ABN), was evaluated for storage stability and measurement accuracy. Storage stability of cVMS on ABN showed less than 1% degradation of the individual 13C-labelled octamethylcyclotetrasiloxane (13C4-D4), decamethylcyclopentasiloxane (13C5-D5) and dodecamethylcyclohexasiloxane (13C6-D6) after 14 days storage at room temperature and at −20 °C whereas significant degradation was observed on ENV+ sorbent at room temperature (37–62 %) and −20 °C (9–16 %). 13C4-D4 formed on ENV+ spiked with 13C5-D5, and both 13C4-D4 and 13C5-D5 formed on ENV+ spiked with 13C6-D6. However, this was not observed on the ABN sorbent. Performance of ABN was compared to ENV+ through an 8-month Arctic sampling campaign at the Zeppelin Observatory (Ny Ålesund, Svalbard). Good agreement between ABN and ENV+ was observed for D4 in the spring/summer months. However, D5 and D6 was found to be consistently higher on the ABN sorbent during this time period with D6 showing the greatest deviation. During the winter months, larger deviations were observed between ABN and ENV+ sorbents with a factor of 4 times higher atmospheric concentrations of both D5 and D6 found on ABN; indicating sorbent related degradation on ENV+. Our findings show that the ABN sorbent provides greater stability and accuracy for atmospheric monitoring of cVMS. Implications of these improvements towards atmospheric fate processes will be discussed.

2020

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