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Arctic Aerosol Model Validation and Evidence for Deposition Ice Nucleation over Siberia

Zamora, Lauren M; Kahn, Ralph; Evangeliou, Nikolaos; Zwaaftink, Christine Groot

2021

Changes in black carbon emissions in Europe and China due to COVID-19

Evangeliou, Nikolaos; Jia, M.; Platt, Stephen Matthew; Eckhardt, Sabine; Myhre, Cathrine Lund; Laj, Paolo G.; Alados-Arboledas, Lucas; Backman, J.; Brem, Benjamin T.; Fiebig, Markus; Flentje, H.; Marinoni, A.; Pandolfi, M.; Yus-Diez, Jesus; Prats, N.; Putaud, J. P.; Sellegri, K.; Sorribas, M.; Eleftheriadis, K.; Vratolis, Stergios; Wiedensohler, A.; Stohl, Andreas; Huang, X.; Gao, J.; Ding, A.

2021

Marine Contribution to Antarctic Carbonaceous Aerosol

Rauber, M.; Salazar, G.; Yttri, Karl Espen; Moschos, V.; Haddad, Imad El; Prévôt, A. S. H.; Glasius, M.; Szidat, S.

2021

Black carbon in Siberian Arctic: gas flaring and wildfires impacts

Popovicheva, Olga; Kobelev, Vasily O.; Chichaeva, M. A.; Evangeliou, Nikolaos; Eleftheriadis, K.; Kasimov, Nikolai S.

2021

Atmospheric transport and deposition of road microplastics to remote regions

Evangeliou, Nikolaos; Grythe, Henrik; Klimont, Z.; Heyes, C; Eckhardt, Sabine; Lopez-Aparicio, Susana; Stohl, Andreas

2021

Enhancing chemical schemes accounted in the FLEXPART v10.4 transport model using a kinetic preprocessor

Sousse, Ruben; Daskalakis, Nikos; Evangeliou, Nikolaos; Hilboll, Andreas; Vrekoussis, Mihalis

2021

Safety assessment of titanium dioxide (E171) as a food additive

Younes, Maged; Aquilina, Gabriele; Castle, Laurence; Engel, Karl-Heinz; Fowler, Paul; Fernandez, Maria Jose Frutos; Fürst, Peter; Gundert-Remy, Ursula; Gürtler, Rainer; Husøy, Trine; Manco, Melania; Mennes, Wim; Moldeus, Peter; Passamonti, Sabina; Shah, Romina; Waalkens-Berendsen, Ine; Wölfle, Detlef; Corsini, Emanuela; Cubadda, Francesco; De Groot, Didima; FitzGerald, Rex; Gunnare, Sara; Gutleb, Arno C.; Mast, Jan; Mortensen, Alicja; Oomen, Agnes; Piersma, Aldert; Plichta, Veronika; Ulbrich, Beate; Van Loveren, Henk; Benford, Diane; Bignami, Margherita; Bolognesi, Claudia; Crebelli, Riccardo; Dusinska, Maria; Marcon, Francesca; Nielsen, Elsa; Schlatter, Josef; Vleminckx, Christiane; Barmaz, Stefania; Carfi, Maria; Civitella, Consuelo; Giarola, Alessandra; Rincon, Ana Maria; Serafimova, Rositsa; Smeraldi, Camilla; Tarazona, Jose; Tard, Alexandra; Wright, Matthew

The present opinion deals with an updated safety assessment of the food additive titanium dioxide (E 171) based on new relevant scientific evidence considered by the Panel to be reliable, including data obtained with TiO2 nanoparticles (NPs) and data from an extended one-generation reproductive toxicity (EOGRT) study. Less than 50% of constituent particles by number in E 171 have a minimum external dimension < 100 nm. In addition, the Panel noted that constituent particles < 30 nm amounted to less than 1% of particles by number. The Panel therefore considered that studies with TiO2 NPs < 30 nm were of limited relevance to the safety assessment of E 171. The Panel concluded that although gastrointestinal absorption of TiO2 particles is low, they may accumulate in the body. Studies on general and organ toxicity did not indicate adverse effects with either E 171 up to a dose of 1,000 mg/kg body weight (bw) per day or with TiO2 NPs (> 30 nm) up to the highest dose tested of 100 mg/kg bw per day. No effects on reproductive and developmental toxicity were observed up to a dose of 1,000 mg E 171/kg bw per day, the highest dose tested in the EOGRT study. However, observations of potential immunotoxicity and inflammation with E 171 and potential neurotoxicity with TiO2 NPs, together with the potential induction of aberrant crypt foci with E 171, may indicate adverse effects. With respect to genotoxicity, the Panel concluded that TiO2 particles have the potential to induce DNA strand breaks and chromosomal damage, but not gene mutations. No clear correlation was observed between the physico-chemical properties of TiO2 particles and the outcome of either in vitro or in vivo genotoxicity assays. A concern for genotoxicity of TiO2 particles that may be present in E 171 could therefore not be ruled out. Several modes of action for the genotoxicity may operate in parallel and the relative contributions of different molecular mechanisms elicited by TiO2 particles are not known. There was uncertainty as to whether a threshold mode of action could be assumed. In addition, a cut-off value for TiO2 particle size with respect to genotoxicity could not be identified. No appropriately designed study was available to investigate the potential carcinogenic effects of TiO2 NPs. Based on all the evidence available, a concern for genotoxicity could not be ruled out, and given the many uncertainties, the Panel concluded that E 171 can no longer be considered as safe when used as a food additive.

2021

Atmospheric Supply of Nitrogen, Copper, HCB, BDE-99, SCCP and PFOS to the Baltic Sea in 2019

Gauss, Michael; Gusev, Alexey; Aas, Wenche; Shatalov, Victor; Ilyin, Ilia; Rozovskaya, Olga; Klein, Heiko; Nyiri, Agnes; Vulyh, Nadejda

Norwegian Meteorological Institute

2021

Air Quality Plans and Measures. Analysis of data submitted from 2014 to 2020.

Sousa Santos, Gabriela; Clemetsen, Tore; Weydahl, Torleif; Guerreiro, Cristina

The submitted data were analysed with the aim to provide information to the EEA Member countries that can be used to improve their air quality management practices, and to give feedback on data quality and possible use. Previous studies in the framework of the Air Implementation Pilot (published in 2012 and 2013) made assessments of the measures and management practices but were not successful in defining the measures’ effectiveness, so the present report also looks into what kind of information can be obtained from the data.

In the period 2014 – 2020, 23 EEA member countries submitted at least one air quality plan. Most countries focus their plans on pollutants related to traffic: NO2 and/or PM10. Most measures target exceedances of NO2 (62 %), PM10 (26 %) and PM2.5 (10 %), and measures are reported that target exceedances of standards of benzo(a)pyrene, nickel and lead (all in PM10) as well as SO2. In one case, the measure is related to benzene.

« Traffic » is the main sector leading to exceedances, with 64 % of records, followed by « domestic heating » (14 %), « local industry » (10 %) and “Other” (8 %). The « Other » category when given further information could comprise a variety of sources including meteorology, agricultural residue burning, harbour activity or shipping.

The majority of the exceedances occurred in urban areas (65 %) followed by suburban areas (21 %), while 14 % of the exceedances addressed in the plans occurred in rural areas.

The available data consist of a large number of individual records (ranging from several hundreds to over 20 thousand depending on the reporting element) that in theory can be linked using unique identifiers. However, not all the records can be linked. While the basis for analysis can vary depending on which reporting segments are used, the overall results are consistent across the segments, and provide a very good overview of which air pollution abatement measures are taken by national and local authorities.

ETC/ATNI

2021

European air quality interim mapping under ETC/ATNI. Evaluation of AQ mapping using UTD measurement and CAMS forecast modelling data: an approach for more timely European AQ annual maps.

Horálek, Jan; Hamer, Paul David; Schreiberova, Marketa; Schneider, Philipp

Air quality European-wide annual maps based on the Air Quality (AQ) e-Reporting validated (E1a) measurement data, the EMEP modelling data and other supplementary data have been regularly produced, using the Regression – Interpolation – Merging Mapping (RIMM) methodology. However, due to the time schedule of production of the validated AQ measurement and the EMEP modelling data, the RIMM air quality maps of a year Y have typically not been available until May of year Y+2. In this report, we examine the AQ interim mapping, based on the preliminary (E2a) measurement and the CAMS Ensemble Forecast modelling data. Such interim maps could be prepared one year earlier than the validated maps. In order to overcome an obstacle of data gaps of E2a data in several areas, so-called pseudo stations data in areas with no E2a data are estimated, based on regression relation between E2a data from year Y and validated E1a data from year Y-1, together with the ratio of the modelling results from years Y and Y-1. The analysis have been performed for the PM10 annual average, the NO2 annual average and the ozone indicator SOMO35, based on the 2017 data. We evaluate these maps using the validated E1a data. Based on the results, we recommend the regular production of the interim AQ maps for the examined indicators, in addition to the regular AQ maps.

ETC/ATNI

2021

Ett år uten et av Norges største miljøproblem: – Mer insekter, null svovelstank

Berglen, Tore Flatlandsmo; Aspholm, Paul Eric (intervjuobjekter); Andreassen, Erik; Kalinina, Kristina (journalister)

2021

Sea Spray Aerosol (SSA) as a Source of Perfluoroalkyl Acids (PFAAs) to the Atmosphere: Field Evidence from Long-Term Air Monitoring

Sha, Bo; Johansson, Jana H.; Tunved, Peter; Bohlin-Nizzetto, Pernilla; Cousins, Ian T.; Salter, Matthew E.

The effective enrichment of perfluoroalkyl acids (PFAAs) in sea spray aerosols (SSA) demonstrated in previous laboratory studies suggests that SSA is a potential source of PFAAs to the atmosphere. In order to investigate the influence of SSA on atmospheric PFAAs in the field, 48 h aerosol samples were collected regularly between 2018 and 2020 at two Norwegian coastal locations, Andøya and Birkenes. Significant correlations (p < 0.05) between the SSA tracer ion, Na+, and PFAA concentrations were observed in the samples from both locations, with Pearson’s correlation coefficients (r) between 0.4–0.8. Such significant correlations indicate SSA to be an important source of atmospheric PFAAs to coastal areas. The correlations in the samples from Andøya were observed for more PFAA species and were generally stronger than in the samples from Birkenes, which is located further away from the coast and closer to urban areas than Andøya. Factors such as the origin of the SSA, the distance of the sampling site to open water, and the presence of other PFAA sources (e.g., volatile precursor compounds) can have influence on the contribution of SSA to PFAA in air at the sampling sites and therefore affect the observed correlations between PFAAs and Na+.

2021

Plastic ingestion by the northern fulmar Fulmarus glacialis from Kongsfjorden

Collard, France; Tulatz, Felix; Gabrielsen, Geir W.; Herzke, Dorte; Krapp, Rupert; Langset, Magdalene; Bourgeon, Sophie

2021

Why is the city's responsibility for its air pollution often underestimated? A focus on PM2.5

Thunis, Philippe; Clappier, Alain; de Meij, Alexander; Pisoni, Enrico; Bessagnet, Bertrand; Tarrasón, Leonor

While the burden caused by air pollution in urban areas is well documented, the origin of this pollution and therefore the responsibility of the urban areas in generating this pollution are still a subject of scientific discussion. Source apportionment represents a useful technique to quantify the city's responsibility, but the approaches and applications are not harmonized and therefore not comparable, resulting in confusing and sometimes contradicting interpretations. In this work, we analyse how different source apportionment approaches apply to the urban scale and how their building elements and parameters are defined and set. We discuss in particular the options available in terms of indicator, receptor, source, and methodology. We show that different choices for these options lead to very large differences in terms of outcome. For the 150 large EU cities selected in our study, different choices made for the indicator, the receptor, and the source each lead to an average difference of a factor of 2 in terms of city contribution. We also show that temporal- and spatial-averaging processes applied to the air quality indicator, especially when diverging source apportionments are aggregated into a single number, lead to the favouring of strategies that target background sources while occulting actions that would be efficient in the city centre. We stress that methodological choices and assumptions most often lead to a systematic and important underestimation of the city's responsibility, with important implications. Indeed, if cities are seen as a minor actor, plans will target the background as a priority at the expense of potentially effective local actions.

2021

Magnitude and Uncertainty of Nitrous Oxide Emissions From North America Based on Bottom-Up and Top-Down Approaches: Informing Future Research and National Inventories

Xu, Rongting; Tian, Hanqin; Pan, N.; Thompson, Rona Louise; Canadell, Josep G. ; Davidson, Eric A.; Nevison, Cynthia; Winiwarter, Wilfried; Shi, H.; Pan, Shufen; Chang, J.; Ciais, Philippe; Dangal, Shree R. S.; Ito, Akihiko; Jackson, Robert B.; Joos, Fortunat; Lauerwald, Ronny; Lienert, Sebastian; Maavara, Taylor; Millet, Dylan B.; Raymond, Peter A.; Regnier, P.; Tubiello, Francesco N; Vuichard, Nicolas; Wells, Kelley C.; Wilson, Chris; Yang, J.; Yao, Y; Zaehle, Sönke; Zhou, Feng

American Geophysical Union (AGU)

2021

Luftkvalitet i Ny-Ålesund. Målinger av lokal luftkvalitet 2019 og 2020.

Johnsrud, Mona; Hermansen, Ove; Krejci, Radovan; Tørnkvist, Kjersti Karlsen

De målte konsentrasjonene var generelt lave for alle komponenter og under nasjonale grenseverdier for beskyttelse av menneskets helse og økosystemet. Vind fra nordlige sektorer ga de høyeste gjennomsnittskonsentrasjonene av nitrogenoksider og svoveldioksid, noe som peker på kraftstasjonen og havnen som mulige kilder. Vi ser også enkelte episoder med langtransport av svoveldioksid.

NILU

2021

Datarapport: Analyse av Gadolinium, Komp-540 og Ioheksol i miljøprøver. DNV-prosjekt: Overvåking utenfor Ramslandsvågen 2021.

Vik, Aasmund Fahre; Pfaffhuber, Katrine Aspmo; Davanger, Kirsten; Rostkowski, Pawel; Gundersen, Hans; Bjørklund, Morten; Uggerud, Hilde Thelle; Vadset, Marit; Bjørneby, Stine Marie

NILU

2021

Seasonality of the particle number concentration and size distribution: a global analysis retrieved from the network of Global Atmosphere Watch (GAW) near-surface observatories

Rose, Clemence; Coen, Martine Collaud; Andrews, Elisabeth; Lin, Yong; Bossert, Isaline; Myhre, Cathrine Lund; Tuch, Thomas; Wiedensohler, Alfred; Fiebig, Markus; Aalto, Pasi; Alastuey, Andrés; Alonso-Blanco, Elisabeth; Andrade, Marcos; Artiñano, Begoña; Arsov, Todor; Baltensprenger, Urs; Bastian, Susanne; Bath, Olaf; Beukes, Johan Paul; Brem, Benjamin T.; Bukowiecki, Nicolas; Casquero-Vera, Juan Andres; Conil, Sébastien; Eleftheriadis, Konstantinos; Favez, Olivier; Flentje, Harald; Gini, Maria I.; Gómez-Moreno, Francisco Javier; Gysel-Beer, Martin; Hallar, Anna Gannet; Kalapov, Ivo; Kalivitis, Nikos; Kasper-Giebl, Anne; Keywood, Melita; Kim, Jeong Eun; Kim, Sang-Woo; Kristensson, Adam; Kulmala, Markku; Lihavainen, Heikki; Lin, Neng-Huei; Lyamani, Hassan; Marinoni, Angela; Dos Santos, Sebastiao Martins; Mayol-Bracero, Olga; Meinhardt, Frank; Merkel, Maik; Metzger, Jean-Marc; Mihalopoulos, Nikolaos; Ondráček, Jakub; Pandolfi, Marco; Pérez, Noemi; Petäjä, Tuukka; Petit, Jean-Eudes; Picard, David; Pichon, Jean-Marc; Pont, Veronique; Putaud, Jean-Philippe; Reisen, Fabienne; Sellegri, Karine; Sharma, Sangeeta; Schauer, Gerhard; Sheridan, Patrick; Sherman, James Patrick; Schwerin, Andreas; Sohmer, Ralf; Sorribas, Mar; Sun, Junying; Tulet, Pierre; Vakkari, Ville; van Zyl, Pieter Gideon; Velarde, Fernando; Villani, Paolo; Vratolis, Stergios; Wagner, Zdenek; Wang, Sheng-Hsiang; Weinhold, Kay; Weller, Rolf; Yela, Margarita; Ždímal, Vladimir; Laj, Paolo G.

Aerosol particles are a complex component of the atmospheric system which influence climate directly by interacting with solar radiation, and indirectly by contributing to cloud formation. The variety of their sources, as well as the multiple transformations they may undergo during their transport (including wet and dry deposition), result in significant spatial and temporal variability of their properties. Documenting this variability is essential to provide a proper representation of aerosols and cloud condensation nuclei (CCN) in climate models. Using measurements conducted in 2016 or 2017 at 62 ground-based stations around the world, this study provides the most up-to-date picture of the spatial distribution of particle number concentration (Ntot) and number size distribution (PNSD, from 39 sites). A sensitivity study was first performed to assess the impact of data availability on Ntot's annual and seasonal statistics, as well as on the analysis of its diel cycle. Thresholds of 50 % and 60 % were set at the seasonal and annual scale, respectively, for the study of the corresponding statistics, and a slightly higher coverage (75 %) was required to document the diel cycle.

Although some observations are common to a majority of sites, the variety of environments characterizing these stations made it possible to highlight contrasting findings, which, among other factors, seem to be significantly related to the level of anthropogenic influence. The concentrations measured at polar sites are the lowest (∼ 102 cm−3) and show a clear seasonality, which is also visible in the shape of the PNSD, while diel cycles are in general less evident, due notably to the absence of a regular day–night cycle in some seasons. In contrast, the concentrations characteristic of urban environments are the highest (∼ 103–104 cm−3) and do not show pronounced seasonal variations, whereas diel cycles tend to be very regular over the year at these stations. The remaining sites, including mountain and non-urban continental and coastal stations, do not exhibit as obvious common behaviour as polar and urban sites and display, on average, intermediate Ntot (∼ 102–103 cm−3). Particle concentrations measured at mountain sites, however, are generally lower compared to nearby lowland sites, and tend to exhibit somewhat more pronounced seasonal variations as a likely result of the strong impact of the atmospheric boundary layer (ABL) influence in connection with the topography of the sites. ABL dynamics also likely contribute to the diel cycle of Ntot observed at these stations. Based on available PNSD measurements, CCN-sized particles (considered here as either >50 nm or >100 nm) can represent from a few percent to almost all of Ntot, corresponding to seasonal medians on the order of ∼ 10 to 1000 cm−3, with seasonal patterns and a hierarchy of the site types broadly similar to those observed for Ntot.

Overall, this work illustrates the importance of in situ measurements, in particular for the study of aerosol physical properties, and thus strongly supports the development of a broad global network of near surface observatories to increase and homogenize the spatial coverage of the measurements, and guarantee as well data availability and quality. The results of this study also provide a valuable, freely available and easy to use support for model comparison and validation, with the ultimate goal of contributing to improvement of the representation of aerosol–cloud interactions in models, and, therefore, of the evaluation of the impact of aerosol particles on climate.

2021

A Bad Start in Life? Maternal Transfer of Legacy and Emerging Poly- And Perfluoroalkyl Substances to Eggs in an Arctic Seabird.

Jouanneau, William; Leándri-Breton, Don-Jean; Corbeau, Alexandre; Herzke, Dorte; Moe, Børge; Nikiforov, Vladimir; Gabrielsen, Geir W.; Chastel, Olivier

2021

Vedfyring ga høy luftforurensning

Grythe, Henrik (intervjuobjekt)

2021

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