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2020
2020
Arctic sea-ice loss intensifies aerosol transport to the Tibetan Plateau
The Tibetan Plateau (TP) has recently been polluted by anthropogenic emissions transported from South Asia, but the mechanisms conducive to this aerosol delivery are poorly understood. Here we show that winter loss of Arctic sea ice over the subpolar North Atlantic boosts aerosol transport toward the TP in April, when the aerosol loading is at its climatological maximum and preceding the Indian summer monsoon onset. Low sea ice in February weakens the polar jet, causing decreased Ural snowpack via reduced transport of warm, moist oceanic air into the high-latitude Eurasian interior. This diminished snowpack persists through April, reinforcing the Ural pressure ridge and East Asian trough, segments of a quasi-stationary Rossby wave train extending across Eurasia. These conditions facilitate an enhanced subtropical westerly jet at the southern edge of the TP, invigorating upslope winds that combine with mesoscale updrafts to waft emissions over the Himalayas onto the TP.
2020
The fingerprint of the summer 2018 drought in Europe on ground-based atmospheric CO2 measurements
During the summer of 2018, a widespread drought developed over Northern and Central Europe. The increase in temperature and the reduction of soil moisture have influenced carbon dioxide (CO2) exchange between the atmosphere and terrestrial ecosystems in various ways, such as a reduction of photosynthesis, changes in ecosystem respiration, or allowing more frequent fires. In this study, we characterize the resulting perturbation of the atmospheric CO2 seasonal cycles. 2018 has a good coverage of European regions affected by drought, allowing the investigation of how ecosystem flux anomalies impacted spatial CO2 gradients between stations. This density of stations is unprecedented compared to previous drought events in 2003 and 2015, particularly thanks to the deployment of the Integrated Carbon Observation System (ICOS) network of atmospheric greenhouse gas monitoring stations in recent years. Seasonal CO2 cycles from 48 European stations were available for 2017 and 2018. Earlier data were retrieved for comparison from international databases or national networks. Here, we show that the usual summer minimum in CO2 due to the surface carbon uptake was reduced by 1.4 ppm in 2018 for the 10 stations located in the area most affected by the temperature anomaly, mostly in Northern Europe. Notwithstanding, the CO2 transition phases before and after July were slower in 2018 compared to 2017, suggesting an extension of the growing season, with either continued CO2 uptake by photosynthesis and/or a reduction in respiration driven by the depletion of substrate for respiration inherited from the previous months due to the drought. For stations with sufficiently long time series, the CO2 anomaly observed in 2018 was compared to previous European droughts in 2003 and 2015. Considering the areas most affected by the temperature anomalies, we found a higher CO2 anomaly in 2003 (+3 ppm averaged over 4 sites), and a smaller anomaly in 2015 (+1 ppm averaged over 11 sites) compared to 2018.
This article is part of the theme issue ‘Impacts of the 2018 severe drought and heatwave in Europe: from site to continental scale'.
2020
Understanding nanomaterial (NM)–protein interactions is a key issue in defining the bioreactivity of NMs with great impact for nanosafety. In the present work, the complex phenomena occurring at the bio/nano interface were evaluated in a simple case study focusing on NM–protein binding thermodynamics and protein stability for three representative metal oxide NMs, namely, zinc oxide (ZnO; NM-110), titanium dioxide (TiO2; NM-101), and silica (SiO2; NM-203). The thermodynamic signature associated with the NM interaction with an abundant protein occurring in most cell culture media, bovine serum albumin (BSA), has been investigated by isothermal titration and differential scanning calorimetry. Circular dichroism spectroscopy offers additional information concerning adsorption-induced protein conformational changes. The BSA adsorption onto NMs is enthalpy-controlled, with the enthalpic character (favorable interaction) decreasing as follows: ZnO (NM-110) > SiO2 (NM-203) > TiO2 (NM-101). The binding of BSA is spontaneous, as revealed by the negative free energy, ΔG, for all systems. The structural stability of the protein decreased as follows: TiO2 (NM-101) > SiO2 (NM-203) > ZnO (NM-110). As protein binding may alter NM reactivity and thus the toxicity, we furthermore assessed its putative influence on DNA damage, as well as on the expression of target genes for cell death (RIPK1, FAS) and oxidative stress (SOD1, SOD2, CAT, GSTK1) in the A549 human alveolar basal epithelial cell line. The enthalpic component of the BSA–NM interaction, corroborated with BSA structural stability, matched the ranking for the biological alterations, i.e., DNA strand breaks, oxidized DNA lesions, cell-death, and antioxidant gene expression in A549 cells. The relative and total content of BSA in the protein corona was determined using mass-spectrometry-based proteomics. For the present case study, the thermodynamic parameters at bio/nano interface emerge as key descriptors for the dominant contributions determining the adsorption processes and NMs toxicological effect.
2020
The response of the atmosphere to solar irradiance and geomagnetic activity is analyzed in experiments with the Whole Atmosphere Community Climate Model (WACCM) under idealized forcings. Four experiments are carried out combining high (H) and low (L) solar radiative forcing with high (7) and low (3) geomagnetic activity: H7 (with high radiative forcing and high geomagnetic activity), H3, (high/low), L7 (low/high), and L3 (low/low). The comparison between these experiment is used to assess the effects of solar radiative forcing and geomagnetic activity mainly on the stratosphere. A two-step Monte Carlo-based statistical test, which defines an impact score, is used to assess statistically significant impacts on regional scales, on pressure levels, for a few key model variables, like NOx, ozone, and temperature.
Under low solar forcing (L7/L3), a statistically significant relationship between geomagnetic activity and NOx is found in both hemispheres and for all seasons. An equally strong relationship is lacking for ozone and temperature when analyzing these fields on isobaric levels. A statistically significant impact on stratospheric ozone is only seen in austral winter and spring. However, vertical cross sections show statistically significant impact on temperature and ozone mainly in the southern hemisphere (SH) during austral winter and the following spring.
Significant and persistent signals in both SH NOx and ozone concentrations are only produced when the effect of high solar forcing is added to high geomagnetic activity (H7). In this case, statistically significant differences are also found for mesospheric temperatures, ozone and NOx. This latter result appears also under low geomagnetic activity as a result of solar forcing alone, suggesting that solar irradiance significantly affects NOx, ozone and stratospheric temperatures and, in some seasons, even tropospheric temperature.
In summary, geomagnetic activity primarily affects NOx and ozone concentrations in the SH. Solar maximum conditions can reduce the amount of NOx in the stratosphere because of higher ozone production. Thus, we conclude that correlations between changes in solar irradiance and geomagnetic activity are important with respect to their effects on the atmosphere. In particular, geomagnetic activity can modulate atmospheric ozone concentrations and other associated stratospheric and tropospheric variables under conditions of high solar activity.
2020
Embedding Ethical Impact Assessment in Nanosafety Decision Support
Nanotechnology is a key enabling technology, which is developing fast and influences many aspects of life. Nanomaterials are already included in a broad range of products and industrial sectors. Nanosafety issues are still a matter of concern for policy makers and stakeholders, but currently, there is no platform where all stakeholders can meet and discuss these issues. A comprehensive overview of all the issues in one single dashboard presenting the output of a decision support system is also lacking. This article outlines a strategy for developing one innovative part of a modular decision support system, designed to support the work of a new Risk Governance Council (RGC) for nanomaterials which will be established through the combined efforts of the GOV4NANO, NANORIGO, and RiskGONE H2020 projects. This new module will consist of guidelines for Ethical Impact Assessment (EIA) for nanomaterials and nanoenabled products. This article offers recommendations for adapting the European Committee for Standardization (CEN) prestandard on Ethical Impact Assessment CWA (CEN Workshop Agreement) 17145‐2:2017 (E), to fit into the more‐encompassing decision support system for risk governance of nanomaterials within the RiskGONE project.
2020
2020
Monitoring of greenhouse gases and aerosols at Svalbard and Birkenes in 2019. Annual report.
The report summarizes the activities and results of the greenhouse gas monitoring at the Zeppelin Observatory, situated on Svalbard in Arctic Norway, during the period 2001-2019, and the greenhouse gas monitoring and aerosol observations from Birkenes for 2009-2019.
NILU
2020
2020
2020
Organic contaminants (polycyclic aromatic hydrocarbons (PAHs), polybrominated diphenyl ethers (PBDEs), polychlorinated biphenyls (PCBs), and chlorinated paraffins (CPs)) and heavy metals and metalloids (Ag, Cd, Co, Cr, Cu, Hg, Ni, Pb, Sb, Zn) were analysed in surface soil samples from the Agbogbloshie e-waste processing and dumping site in Accra (Ghana). In order to identify which of the pollutants are likely to be linked specifically to handling of e-waste, samples were also collected from the Kingtom general waste site in Freetown (Sierra Leone). The results were compared using principal component analyses (PCA). PBDE congeners found in technical octa-BDE mixtures, highly chlorinated PCBs and several heavy metals (Cu, Pb, Ni, Cd, Ag and Hg) showed elevated concentrations in the soils that are likely due to contamination by e-waste. PCAs associated those compounds with pyrogenic PAHs, suggesting that burning of e-waste, a common practice to isolate valuable metals, may cause this contamination. Moreover, other contamination pathways, especially incorporation of waste fragments into the soil, also appeared to play an important role in determining concentrations of some of the pollutants in the soil. Concentrations of several of these compounds were extremely high (especially PBDEs, heavy metals and SCCPs) and in some cases exceeded action guideline levels for soil. This indicates that exposure to these contaminants via the soil alone is potentially harmful to the recyclers and their families living on waste sites. Many organic contaminants and other exposure pathways such as inhalation are not yet included in such guidelines but may also be significant, given that deposition from the air following waste burning was identified as a major pollutant source.
2020
Emissions outsourcing in the EU. A review of potential effects on industrial pollution.
This study reviews potential evidence for emissions outsourcing in the European Union as the reduction in industrial emissions in Europe may be linked to the relocation of industry abroad (i.e. away from Europe). Emission trends of selected industrial pollutants to air (PAH, SOx, B(a)P, PCB, Pb, Zn and Ni) were established for both domestic emissions and embodied emissions in imports using available data in the EXIOBASE environmentally extended multiregional input-output system. Despite the overall decreasing trends of domestic emissions in Europe, a great variation was observed in the decrease rate of direct emissions and the increase rates in embodied emissions, due to increasing import of associated products. In addition to the analysis of data in EXIOBASE, a review of literature shows that industries’ responses to environmental regulations differ greatly based on the nature of industrial activities. Despite imposing higher costs to industries, no evidence was found in the reviewed literature that European environmental regulations caused industries to relocate. However, once industries aim to relocate outside of Europe to benefit from economic factors, such as lowering their production cost, the degree by which environmental regulations are enforced in the country of relocation can play a significant role in selecting their new location.
ETC/ATNI
2020
2020
2020